Related papers: A Multi-Harmonic NIR-UV Dual-Comb Spectrometer
The optical frequency comb has made a significant impact in precision spectroscopy and on our ability to probe atomic, molecular and, recently, nuclear transitions to further our understanding of their fundamental properties and how their…
Broadband and high-resolution spectroscopy in the visible and ultraviolet is central to advances in multiple fields, including fundamental quantum physics, biology, atmospheric science and astronomy. Traditionally, these measurements are…
We perform dual-comb spectroscopy in two UV bands: 325-342 nm and 372-410 nm, corresponding to the 7th and 6th harmonics of a dual-comb 2.35-{\mu}m laser source, and simultaneously resolve ~500,000 and ~1,000,000 comb lines spaced by 80 MHz…
Dual-comb spectroscopy enables broadband analysis of key molecules with unparalleled frequency resolution and exceptional signal-to-noise ratios across various spectral regions. However, fully harnessing its potential for broadband…
Dual Comb Spectroscopy proved its versatile capabilities in molecular fingerprinting in different spectral regions, but not yet in the ultraviolet (UV). Unlocking this spectral window would expand fingerprinting to the electronic energy…
Ultrabroadband electro-optic sampling with few-cycle optical pulses is known to be an extremely sensitive technique to detect electric field amplitudes. By combining this method with dual-comb spectroscopy and with a new class of ultrafast…
Ultraviolet spectroscopy provides unique insights into the structure of matter with applications ranging from fundamental tests to photochemistry in the earth's atmosphere and astronomical observations from space telescopes. At longer…
We describe an electro-optic dual-comb system that operates in the near-infrared (near-IR) region to generate optical frequency combs in the near-UV by sum frequency generation in two configurations. The near-IR frequency combs are…
The highly energetic photons of ultraviolet light drive electronic and rovibronic transitions in all molecular species. This radiation is thus a prime tool for strongly selective spectroscopic fingerprinting and real-time environmental…
Mid-infrared (mid-IR) spectroscopy offers unparalleled sensitivity for the detection of trace gases, solids and liquids, which is based on the existence of strong telltale vibrational bands in this part of the spectrum. It was shown more…
We introduce a novel ultra-broadband ultraviolet and visible frequency comb light source covering more than 240 THz by resonant dispersive wave emission in a gas-filled hollow-core fiber waveguide. The light source allows tuning from ~340…
High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb…
Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…
Optical frequency combs emit narrow pulses of light with a stable repetition rate. Equivalently, the generated light spectrum consists of many discrete frequencies spaced by this same repetition rate. These precision light sources have…
Dual-comb interferometry is a measurement technique that uses two laser frequency combs to retrieve complex spectra in a line-by-line basis. This technique can be implemented with electro-optic frequency combs, offering intrinsic mutual…
Dual-comb spectroscopy utilizes two sets of comb lines with slightly different comb-tooth-spacings, and optical spectral information is acquired by measuring the radio-frequency beat notes between the sets of comb lines. It holds the…
Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…
Ultraviolet frequency combs enable applications ranging from precision spectroscopy to atomic clocks by addressing the electronic transitions of atoms and molecules. Access to ultraviolet light via integrated nonlinear optics is usually…
With the advent of laser frequency combs, coherent light sources that offer equally-spaced sharp lines over a broad spectral bandwidth have become available. One decade after revolutionizing optical frequency metrology, frequency combs hold…
Dual-comb spectroscopy has demonstrated remarkable capabilities for rapid and sensitive measurements; however, significant challenges still exist in generating high-power, mutually coherent mid-infrared combs. Here we demonstrate that a…