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The alignment of the frontier orbital energies of an adsorbed molecule with the substrate Fermi level at metal-organic interfaces is a fundamental observable of significant practical importance in nanoscience and beyond. Typical density…

Mesoscale and Nanoscale Physics · Physics 2017-03-07 Zhenfei Liu , David A. Egger , Sivan Refaely-Abramson , Leeor Kronik , Jeffrey B. Neaton

Adding porosity to battery electrodes is believed to be universally useful for adding space to accommodate volumetric expansion, electrolyte access to all active materials, helping to mitigate poor C-rate performance for thicker electrodes…

Applied Physics · Physics 2020-08-26 Sally O'Hanlon , David McNulty , Ruiyuan Tian , Jonathan Coleman , Colm O'Dwyer

Ether-based electrolytes exhibit excellent compatibility with Li metal anodes, but their instability at high voltages limits their use in high-voltage Li metal batteries. To address this issue, we introduce an alternative perfluorobutane…

Materials Science · Physics 2024-09-30 Jian He , Shihan Qi , Jianmin Ma , Nongnuch Artrith

In 2D materials, the quantum confinement and van der Waals-type interlayer interactions largely govern the fundamental electronic and optical properties, and the dielectric screening plays a dominant role in the excitonic properties. This…

Mesoscale and Nanoscale Physics · Physics 2021-02-19 Guowei Zhang , Shenyang Huang , Fanjie Wang , Hugen Yan

In perovskite solar cells, photovoltaic action is created by charge transport layers (CTLs) either side of the light-absorbing metal halide perovskite semiconductor. Hence, the rates for desirable charge extraction and unwanted interfacial…

Designing molecular organic semiconductors with distinct frontier orbitals is key for the development of devices with desirable properties. Generating defined organic nanostructures with atomic precision can be accomplished by on-surface…

The rapid development of modern energy applications drives an urgent need to enhance the dielectric strength of energy storage dielectrics for higher power density. Interface design is a promising strategy to regulate the crucial charge…

Materials Science · Physics 2024-11-05 Haoxiang Zhao , Lixuan An , Daning Zhang , Xiong Yang , Huanmin Yao , Guanjun Zhang , Haibao Mu , Björn Baumeier

This study comprehensively examined the structural, electronic, electrochemical, and energy storage properties of boron-vacancy induced porous boron nitride monolayers (BN:VB) as multifunctional materials, anodes for MIBs and H2 storage…

Materials Science · Physics 2026-05-06 Wadha Alfalasi , Wael Othman , Tanveer Hussain , Nacir Tit

The large Land\'{e} g-factor, high spin-orbit coupling, and low effective mass of the two-dimensional electron gas in InSb quantum wells combined with proximal superconductivity may realize a scalable platform for topological quantum…

The integrated device of a perovskite solar cell with a Li-ion battery is an innovative solution for decentralized energy storage in smart electronic devices. In this study, we examine the stability of Li ions intercalated in a CsPbI$_3$…

Materials Science · Physics 2025-12-02 Wei Wei , Julian Gebhardt , Daniel F. Urban , Christian Elsässer

The magnetic sublayers introduced by intercalation into the host transition-metal dichalcogenide (TMD) are known to produce various magnetic states. The magnetic sublayers and their magnetic ordering strongly modify the electronic coupling…

We present an investigation of the microscopic interplay between excitons and charge carriers by means of combined photoluminescence (PL) and charge carrier transport measurements on organic thin film transistors (OTFT). For this purpose,…

Materials Science · Physics 2015-06-15 N. H. Hansen , C. Wunderlich , A. K. Topczak , J. Pflaum

We have investigated the electronic structure of charged bilayer and trilayer phoshporene using first-principles, density-functional-theory calculations. We find that the effective dielectric constant for an external electric field applied…

Mesoscale and Nanoscale Physics · Physics 2017-08-09 Bukyoung Jhun , Cheol-Hwan Park

Graphene intercalation materials are potentially promising for the implementation of the ultra-low power, excitonic-condensate-based Bilayer pseudoSpin Field-Effect Transistor (BiSFET) concept, as well as other novel device concepts…

Mesoscale and Nanoscale Physics · Physics 2013-08-13 Priyamvada Jadaun , Hema C. P. Movva , Leonard F. Register , Sanjay K. Banerjee

We study a capacitor made of three monolayers of transition metal dichalcogenide (TMD) separated by hexagonal Boron Nitride (hBN). We assume that the structure is symmetric with respect to the central layer plane. The symmetry includes the…

Mesoscale and Nanoscale Physics · Physics 2019-04-10 M. Sammon , B. I. Shklovskii

We use molecular dynamics simulations to explore the impact of a non-ionic solvent on the structural and capacitive properties of supercapacitors based on an ionic liquid electrolyte and carbon electrodes. The study is focused on two pure…

Materials Science · Physics 2013-08-27 Céline Merlet , Mathieu Salanne , Benjamin Rotenberg , Paul A Madden

Atomically thin layered black phosphorous (BP) has recently appeared as an alternative to the transitional metal di chalcogenides for future channel material in a MOS transistor due to its lower carrier effective mass. Investigation of the…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Anuja Chanana , Santanu Mahapatra

A tandem GaAsP/SiGe solar cell has been developed employing group-IV reverse buffer layers grown on silicon substrates with a subsurface porous layer. Reverse buffer layers facilitate a reduction in the threading dislocation density with…

In graphene moir\'e superlattices, electronic interactions between layers are mostly hidden as band structures get crowded because of folding, making their interpretation cumbersome. Here, the evolution of the electronic band structure as a…

Mesoscale and Nanoscale Physics · Physics 2021-09-01 Francisco Sanchez-Ochoa , Andres Botello-Mendez , Cecilia Noguez

The formation of interface dipoles in self-assembled monolayers (SAMs) of --CH$_3$ and --CF$_3$ terminated short-chain alkanethiolates on Ag(111) is studied by means of density functional theory calculations. The interface dipoles are…

Materials Science · Physics 2011-11-09 Paul C. Rusu , Gianluca Giovannetti , Geert Brocks