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The Hilbert space for an interacting electron system increases exponentially with electron number $N$. This limits the concept of wavefunctions $\psi$ based on solutions of the Schr\"odinger equation to $N \leq N_0$ with $N_0 \simeq 10^3$…

Chemical Physics · Physics 2020-05-13 Peter Fulde

An alternative to Density Functional Theory are wavefunction based electronic structure calculations for solids. In order to perform them the Exponential Wall (EW) problem has to be resolved. It is caused by an exponential increase of the…

Chemical Physics · Physics 2017-06-07 Peter Fulde , Hermann Stoll

Wavefunctions for large electron numbers suffer from an exponential growth of the Hilbert space which is required for their description. In fact, as pointed out by W. Kohn, for electron numbers $N > N_0$ where $N_0 \approx 10^3$ they become…

Chemical Physics · Physics 2017-05-31 Peter Fulde

Wavefunctions for large electron numbers $N$ are plagued by the Exponential Wall Problem (EWP), i.e., an exponential increase in the dimensions of Hilbert space with $N$. Therefore they loose their meaning for macroscopic systems, a point…

Other Condensed Matter · Physics 2019-02-20 Peter Fulde

Electronic structure calculations for solids based on many-electron wavefunctions have been hampered by the argument that for large electron numbers wavefunctions are not a legitimate scientific concept, because they face an exponential…

Materials Science · Physics 2015-09-30 Peter Fulde

The electronic Schr\"odinger equation describes the motion of N electrons under Coulomb interaction forces in a field of clamped nuclei. The solutions of this equation, the electronic wavefunctions, depend on 3N variables, three spatial…

Numerical Analysis · Mathematics 2017-01-16 Stephan Scholz , Harry Yserentant

New method for ab initio calculations of the properties of large size system based on phase-amplitude functional is presented. It is shown that Schrodinger equation for many electrons complex system including large size molecules, or…

Computational Physics · Physics 2019-10-10 Pawel Strak , Konrad Sakowski , Pawel Kempisty , Stanislaw Krukowski

For a given many-electron molecule, it is possible to define a corresponding one-electron Schr\"odinger equation, using potentials derived from simple atomic densities, whose solution predicts fairly accurate molecular orbitals for single-…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten

The Schr\"odinger equation relates the electron wavefunction and the electric potential, which are emergent physical quantities. At that emergent level, the Schr\"odinger equation is either postulated as a principle of quantum physics or…

Quantum Physics · Physics 2022-12-27 Spyros Efthimiades

The Bloch wavefunction leads either to mathematically impossible consequences or suggests that the ground state energy is a function of size and shape when the geometry of large crystals is considered in detail. It is incompatible with the…

Materials Science · Physics 2008-06-20 T. R. S. Prasanna

The electronic Schr\"odinger equation describes the motion of $N$ electrons under Coulomb interaction forces in a field of clamped nuclei. It is proved that its solutions for eigenvalues below the essential spectrum lie in the spectral…

Analysis of PDEs · Mathematics 2026-04-10 Harry Yserentant

For a given many-electron molecule, it is possible to define a corresponding one-electron Schr\"odinger equation, using potentials derived from simple atomic densities, whose solution predicts fairly accurate molecular orbitals for single-…

Chemical Physics · Physics 2022-05-16 Fariba Nazari , Jerry L. Whitten

How does charge density constrain many-body wavefunctions in nature? The Hohenberg-Kohn theorem for non-relativistic, interacting many-body Schr\"odinger systems is well-known and was proved using \emph{reductio-ad-absurdum}; however, the…

Computational Physics · Physics 2022-04-28 Purnima Ghale

A method is proposed to find the wave function of an electron moving infinitely in the field of an arbitrary 1D layer structure with two different homogeneous semi-infinite boundaries. It is shown that in general the problem reduces to…

Quantum Physics · Physics 2009-11-10 A. Zh. Khachatrian

Wave functions and electron potentials of laterally-confined surface states are determined experimentally by means of photoemission from stepped Au(111) surfaces. Using an iterative formalism borrowed from x-ray diffraction, we retrieve the…

Materials Science · Physics 2012-11-13 A. Mugarza , J. E. Ortega , F. J. Himpsel , F. J. Garcia de Abajo

We develop a new density functional theory (DFT) and formalism for correlated electron systems by taking as reference an interacting electron system that has a ground state wavefunction which obeys exactly the Gutzwiller approximation for…

Superconductivity · Physics 2009-11-13 K. M. Ho , J. Schmalian , C. Z. Wang

We examine the deformation quantization of a single particle moving in one dimension (i) in the presence of an infinite potential wall, (ii) confined by an infinite square well, and (iii) bound by a delta function potential energy. In…

Quantum Physics · Physics 2009-11-10 S. Kryukov , M. A. Walton

The theoretical foundations of quantum mechanics and de Broglie--Bohm mechanics are analyzed and it is shown that both theories employ a formal approach to microphysics. By using a realistic approach it can be established that the internal…

Quantum Physics · Physics 2015-06-26 W. A. Hofer

Following Max Planck's hypothesis of quanta (quant-ph/0012069) and the matter wave idea of Louis de Broglie (quant-ph/9911107), Erwin Schroedinger proposed, at the beginning of 1926, the concept of wavefunction and wave equation for it.…

Quantum Physics · Physics 2007-05-23 Andrei P. Kirilyuk

We develop a new envelope-function formalism to describe electrons in slowly-varying inhomogeneously strained semiconductor crystals. A coordinate transformation is used to map a deformed crystal back to geometrically undeformed structure…

Materials Science · Physics 2014-10-29 Wenbin Li , Xiaofeng Qian , Ju Li
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