Related papers: Numerical investigation of effective nonlinear coe…
State-of-the-art experiments employ strong ultrafast optical fields to study the nonlinear response of electrons in solids on an attosecond time-scale. Notably, a recent experiment retrieved a 3rd order nonlinear susceptibility by comparing…
In this work, the nonlinear optical response, and in particular, the high harmonic generation of semiconductors is addressed by using the Wannier gauge. One of the main problems in the time evolution of the Semiconductor Bloch equations…
A scheme for quasi-phase-matching high-harmonic generation is proposed in which polarization beating within a hollow core birefringent waveguide modulates the generation of harmonics. The evolution of the polarization of a laser pulse…
We report the simultaneous quasi-phase-matching of all three possible nonlinearities for propagation along the X axis of periodocally poled (PP) KTiOPO4 (KTP) for second-harmonic generation of 745 nm pulsed light from 1490nm subpicosecond…
An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…
The emerging all-dielectric platform exhibits high-quality ($Q$) resonances governed by the physics of bound states in the continuum (BIC) that drives highly efficient nonlinear optical processes. Here we demonstrate the robust enhancement…
As one of the two types of backward second-harmonic generation (SHG), symmetric SHG exhibits some physical characteristics and application prospects that are distinct from those of forward SHG. It is generally realized through quasi-phase…
We carried out second-harmonic generation in quasi-phase-matched \alpha-phase lithium niobate channel waveguides realized by proton exchange and surface periodic poling. Owing to a limited ferroelectric domain depth, we could observe the…
Non-congruent gas-liquid phase transition (NCPT) have been studied in modified Coulomb model of a binary ionic mixture C(+6) + O(+8) on a \textit{uniformly compressible} ideal electronic background /BIM($\sim$)/. The features of NCPT in…
High-quality crystals without inversion symmetry are the conventional platform to achieve optical frequency conversion via three wave-mixing. In bulk crystals, efficient wave-mixing relies on phase-matching configurations, while at the…
In this paper we analyze and implement a second-order-in-time numerical scheme for the three-dimensional phase field crystal (PFC) equation. The numerical scheme was proposed in [46], with the unique solvability and unconditional energy…
Efficient generation of high-quality photon pairs is essential for modern quantum technologies. Micro-ring resonator is an ideal platform for studying on-chip photon sources due to strong nonlinear effect, resonant-enhanced optical fields,…
Harmonic generation in underdense spatially homogeneous plasma is generally expected to be inefficient: in an unmagnetized uniform plasma the fundamental and its harmonics cannot be phase-matched, resulting in third-harmonic generation…
In this paper, we have investigated the interplay between the second and third-order nonlinearities in lithium-niobate waveguides with strong waveguide dispersion using uniform and linearly-chirped poling patterns at input powers in the…
We report a new approach to phase matching of nonlinear materials based on the free space multipass cells. This concept quasi-phase matches crystalline quartz and increases the second harmonic generation efficiency by a factor 40.
The nonlinear frequency conversion of low-temporal-coherent light holds a variety of applications and has attracted considerable interest. However, its physical mechanism remains relatively unexplored, and the conversion efficiency and…
Nonlinear frequency conversion provides essential tools for light generation, photon entanglement, and manipulation. Transition metal dichalcogenides (TMDs) possess huge nonlinear susceptibilities and 3R-stacked TMD crystals further combine…
Terahertz nonlinear optics is a viable method to interrogate collective phenomena in quantum materials spanning ferroelectrics, charge-density waves, and superconductivity. In superconductors this includes the Higgs amplitude and Josephson…
We derive general conditions for 100 percent frequency conversion in any doubly resonant nonlinear cavity, for both second- and third-harmonic generation via chi2 and chi3 nonlinearities. We find that conversion efficiency is optimized for…
High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…