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Highly efficient terahertz (THz) wave sources based on difference frequency generation (DFG) process in nonlinear optical crystals play an important role for the applications of THz wave. In order to find more novel nonlinear crystals, here…
We report a theoretical design analysis of domain-engineered periodically poled lithium niobate (PPLN) for wavelength conversion of near-infrared sources to generate coherent light in the visible spectral range. Our analysis on the spectral…
Coherent nonlinear optical micro-spectroscopy is a frequently used tool in modern material science, as it is sensitive to many different local observables, which comprise, among others, crystal symmetry and vibrational properties. The…
The optimization of nonlinear optical processes at the nanoscale is a crucial step for the development of nanoscale photon sources for quantum-optical networks. The development of innovative plasmonic nanoantenna designs and hybrid…
Providing quantitative interpretation of coherent nonlinear microscopy images, such as third-harmonic generation (THG), is generally hampered by the complex phase-matching conditions, especially in the presence of sample linear…
We present a combined experimental and theoretical study of enhanced third-harmonic generation (THG) in silicon nitride metasurfaces. These structures exhibit strong resonant nonlinear responses, enabling up to two orders of magnitude…
Quadratic optical parametric processes form the foundation for a variety of applications related to classical and quantum frequency conversion, which have attracted significant interest recently in on-chip implementation. These processes…
We report the successful design and experimental implementation of three coincident nonlinear interactions, namely ZZZ ("type-0"), ZYY (type-I), and YYZ/YZY (type-II) second harmonic generation of 780 nm light from a 1560 nm pump beam in a…
Second-harmonic generation (SHG) is a fundamental tool in modern laser technology, enabling coherent frequency conversion to remote optical bands, serving as the basis for self-referenced femtosecond lasers and quadrature-squeezed light…
High harmonic generation (HHG) from semiconductors and insulators has become a very active area of research due to its great potential for developing compact HHG devices. Here we show that by growing monolayers (ML) of insulators on…
Quasi-phase-matching (QPM) is a widely adopted technique for mitigating stringent momentum conservation in nonlinear optical processes such as second-harmonic generation (SHG). It effectively compensates for the phase velocity mismatch…
Thin-film lithium niobate (TFLN) based frequency doublers have been widely recognized as essential components for both classical and quantum optical communications. Nonetheless, the efficiency of these devices is hindered by imperfections…
Periodically poled thin-film lithium niobate (TFLN) waveguides, which enable efficient quadratic nonlinear processes, serve as crucial foundation for classical and quantum signal processing. To expand their application scope, we provide the…
Possible squeezed states generated in a three-waveguide nonlinear coupler operating with second harmonic generation is discussed. This study is carried out using two well-known techniques; the phase space method (based on positive…
We report on a direct generation of efficient and wavelength-tunable third-harmonic generation (THG) from ultrapure electronic-grade (EG) diamond crystals. Under an ultrafast infrared excitation at 1280 nm, the considerably high optical…
The generalization of quasi-phase-matching using polarization beating and of multimode quasi-phase-matching (MMQPM) for the generation of high-order harmonics is explored, and a method for achieving polarization beating is proposed. If two…
Second harmonic generation in a two dimensional nonlinear quasi-crystal is demonstrated for the first time. Temperature and wavelength tuning of the crystal reveal the uniformity of the pattern while angle tuning reveals the dense nature of…
Lithium niobate (LN) thin film has recently emerged as an important platform for nonlinear optical investigations for its large $\chi^{(2)}$ nonlinear coefficients and ability of light localization. In this paper, we report the first…
This work is the second in the series "On the performance of QTP functionals applied to second-order response properties." In the first paper (J. Chem. Phys. 162, 054105, 2025), we demonstrated the good performance of Quantum Theory Project…
A new scheme for non-destructive characterization of quasi-phase-matching grating structures and temperature gradients via inverse Fourier theory using second-harmonic-generation experiments is proposed. We show how it is possible to…