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Related papers: Nonlinear opto-vibronics in molecular systems

200 papers

Here we present theoretical studies of the effect of vibronic coupling on nonlinear transport characteristics (current-voltage and conductance-voltage) in molecular electronic devices. Considered device is composed of molecular quantum dot…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Kamil Walczak

The emergence of confined structures and pattern formation are exceptional manifestations of concurring nonlinear interactions found in a variety of physical, chemical and biological systems[1]. Optical solitons are a hallmark of extreme…

Optics · Physics 2020-01-29 Felix Kurtz , Claus Ropers , Georg Herink

We study the quantum dynamics of the cavity optomechanical system formed by a Fabry-Perot cavity with a thin vibrating membrane at its center. We first derive the general multimode Hamiltonian describing the radiation pressure interaction…

Quantum Physics · Physics 2011-09-14 C. Biancofiore , M. Karuza , M. Galassi , R. Natali , P. Tombesi , G. Di Giuseppe , D. Vitali

The interaction between electronic and vibrational degrees of freedom is an important mechanism in nonequilibrium charge transport through molecular nanojunctions. While adiabatic polaron-type coupling has been studied in great detail, new…

Mesoscale and Nanoscale Physics · Physics 2022-06-10 Christoph Kaspar , André Erpenbeck , Jakob Bätge , Christian Schinabeck , Michael Thoss

We investigate optical nonlinear interactions in a dynamic environment by studying generation of photons in spontaneous parametric down conversion inside a nonlinear cavity where the optical path length is periodically modulated in time. We…

Optics · Physics 2019-10-16 Usman A. Javid , Qiang Lin

By mapping the strong interaction between Rydberg excitations in ultra-cold atomic ensembles onto single photons via electromagnetically induced transparency, it is now possible to realize a nonlinear optical medium which exhibits a strong…

Quantum Physics · Physics 2016-07-08 Ofer Firstenberg , Charles S. Adams , Sebastian Hofferberth

We propose a new model suitable for a nonequilibrium molecular dynamics (MD) simulation of electrical conductors. The model consists of classical electrons and atoms. The atoms compose a lattice vibration system. The electrons are scattered…

Statistical Mechanics · Physics 2015-05-30 Fan Lee , Tatsuro Yuge , Akira Shimizu

Linear spectra of molecular polaritons formed by $N$ molecules coupled to a microcavity photon mode are usually well described by classical linear optics, raising the question of where the expected nonlinear effects in these strongly…

Quantum Physics · Physics 2024-11-19 Arghadip Koner , Joel Yuen-Zhou

We consider theoretically the optomechanical interaction of several mechanical modes with a single quantized cavity field mode for linear and quadratic coupling. We focus specifically on situations where the optical dissipation is the…

Quantum Physics · Physics 2014-10-24 H. Seok , L. F. Buchmann , S. Singh , P. Meystre

The study of non-equilibrium physics from the perspective of the quantum limits of thermodynamics and fluctuation relations can be experimentally addressed with linear optical systems. We discuss recent experimental investigations in this…

Enhancing optical nonlinearities so that they become appreciable on the single photon level and lead to nonclassical light fields has been a central objective in quantum optics for many years. After this has been achieved in individual…

Quantum Physics · Physics 2016-09-20 Michael J. Hartmann

The quantum dynamics of optomechanical systems was mostly studied for their fluctuations around classical steady states. We present a theoretical approach to determining the system observables of optomechanical systems as genuine quantum…

Quantum Physics · Physics 2012-06-21 Bing He

Few-photon transport via waveguide-coupled local quantum systems has attracted extensive theoretical and experimental studies. Most of the study has focused on atomic or atomic-like local quantum systems due to their strong light-matter…

Quantum Physics · Physics 2022-09-09 Yunkai Wang , Kejie Fang

The observation that materials can change their properties when placed inside or near an optical resonator, has sparked a fervid interest in understanding the effects of strong light-matter coupling on molecular dynamics, and several…

Chemical Physics · Physics 2024-03-20 Ilia Sokolovskii , Gerrit Groenhof

Nonlinear optical phenomena are typically local. Here we predict the possibility of highly nonlocal optical nonlinearities for light propagating in atomic media trapped near a nano-waveguide, where long-range interactions between the atoms…

Quantum Physics · Physics 2016-07-08 Ephraim Shahmoon , Pjotrs Grisins , Hans Peter Stimming , Igor Mazets , Gershon Kurizki

We studied the interaction of a two-level atom with a frequency modulated cavity mode in an ideal optical cavity. The system, described by a Jaynes-Cumming Hamiltonian, gave rise to a set of stiff nonlinear first order equations solved…

Quantum Physics · Physics 2013-01-22 U. Pishipati , I. Almakremi , Amitabh Joshi , Juan D. Serna

We extend the model of exciton-plasmon materials to include a ro-vibrational structure of molecules using wave-packet propagations on electronic potential energy surfaces. The new model replaces conventional two-level emitters with more…

Mesoscale and Nanoscale Physics · Physics 2017-08-18 Maxim Sukharev , Eric Charron

We show that coupling ultracold atoms in optical lattices to quantized modes of an optical cavity leads to quantum phases of matter, which at the same time posses properties of systems with both short- and long-range interactions. This…

Quantum Gases · Physics 2016-07-06 Santiago F. Caballero-Benitez , Gabriel Mazzucchi , Igor B. Mekhov

A rigorous quantum description of molecular dynamics with a particular emphasis on internal observables is developed accounting explicitly for kinetic couplings between nuclei and electrons. Rotational modes are treated in a genuinely…

Chemical Physics · Physics 2015-07-07 Sylvain D. Brechet , Francois A. Reuse , Klaus Maschke , Jean-Philippe Ansermet

In this book chapter we analyze the high excitation nonlinear response of the Jaynes-Cummings model in quantum optics when the qubit and cavity are strongly coupled. We focus on the parameter ranges appropriate for transmon qubits in the…

Mesoscale and Nanoscale Physics · Physics 2012-07-20 Eran Ginossar , Lev S. Bishop , S. M. Girvin