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Direct laser excitation of the lowest known nuclear excited state in $^{229}$Th has been a longstanding objective. It is generally assumed that reaching this goal would require a considerably reduced uncertainty of the isomer's excitation…

$^{229}$Th with a low-lying nuclear isomeric state is an essential candidate for a nuclear clock as well as many other applications. Laser excitation of the isomeric state has been a long-standing goal. With relativistic $^{229}$Th ions in…

$^{229}$Th is the only known nucleus with an excited state that offers the possibility for a direct laser excitation using existing laser technology. Its excitation energy has been measured indirectly to be 7.8(5) eV ($\approx$160 nm). The…

Instrumentation and Detectors · Physics 2018-12-14 Benedict Seiferle , Lars von der Wense , Ines Amersdorffer , Nicolas Arlt , Benjamin Kotulski , Peter G. Thirolf

The results of experimental studies of the low-energy isomeric state in the $^{229}$Th nucleus are presented. The work is consisted of several stages. During the first stage $^{229}$Th nuclei were excited with the inverse internal…

Thorium-229 is a unique case in nuclear physics: it presents a metastable first excited state Th-229m, just a few electronvolts above the nuclear ground state. This so-called isomer is accessible by VUV lasers, which allows transferring the…

We investigate the process of nuclear excitation via a two-photon electron transition (NETP) for the case of the doubly charged thorium. The theory of the NETP process has been devised originally for heavy helium-like ions. In this work, we…

Atomic Physics · Physics 2019-05-17 Robert A. Müller , Andrey V. Volotka , Andrey Surzhykov

Excitation of the isomeric nuclear state 229m Th in the process of thorium atom irradiation by two-color femtosecond pulse of Ti: Sa laser at the fundamental wavelength and second harmonic is analyzed. It is shown that the rate of isomeric…

Optics · Physics 2019-01-23 A. V. Andreev , A. B. Savelyev , S. Yu. Stremoukhov , O. A. Shoutova

The nuclear isomeric state $^{229m}$Th with an exceptionally low excitation energy makes the $^{229}$Th isotope a crucial candidate for nuclear clocks and many other applications. Efficient and controllable production of $^{229m}$Th is…

Nuclear Theory · Physics 2024-06-19 Jingyan Zhao , Adriana Pálffy , Christoph H. Keitel , Yuanbin Wu

The first excited isomeric state of Th-229 has an exceptionally low energy of only a few eV and could form the gateway to high-precision laser spectroscopy of nuclei. The excitation energy of the isomeric state has been inferred from…

We consider the excitation of the nuclear transition ^{229g}Th - ^{229m}Th near 7.6 eV in singly ionized thorium via an electronic bridge process. The process relies on the excitation of the electron shell by two laser photons whose sum…

Atomic Physics · Physics 2010-10-27 S. G. Porsev , V. V. Flambaum , E. Peik , Chr. Tamm

Thorium-229 possesses the lowest nuclear first excited state with an energy of about 8 eV. The extremely narrow linewidth of the nuclear first excited state with the uncertainty of 53 THz prevents the direct laser excitation and the…

Atomic Physics · Physics 2024-05-14 Lin Li , Zi Li , Chen Wang , Wen-Ting Gan , Xia Hua , Xin Tong

The isomeric first excited state of the isotope 229Th exhibits the lowest nuclear excitation energy in the whole landscape of known atomic nuclei. For a long time this energy was reported in the literature as 3.5(5) eV, however, a new…

Nuclear Experiment · Physics 2015-06-12 L. v. d. Wense , P. G. Thirolf , D. Kalb , M. Laatiaoui

Theoretical considerations are made for the nuclear excitation from the ground state to the 8 eV $^{229m}$Th isomer via near-resonant electron transitions in Sb-like ($q=39+$) thorium ions. The energy of the first excited atomic state…

Atomic Physics · Physics 2025-04-17 Karol Kozioł , Jacek Rzadkiewicz

The electronic excitation of molecules triggers diverse phenomena such as luminescence and photovoltaic effects, which are the bases of various energy-converting devices. Understanding and control of the excitations at the single-molecule…

Chemical Physics · Physics 2017-07-12 Hiroshi Imada , Kuniyuki Miwa , Miyabi Imai-Imada , Shota Kawahara , Kensuke Kimura , Yousoo Kim

A possibility of the two-photon excitation of an isomeric state in a nucleus of thorium-229 has been discussed. The fluorescence intensity of the excitation is demonstrated to be identical for the irradiation of nuclei with either…

A scanning tunneling microscope (STM) can do more than atomic imaging and manipulation. Its tunneling current can also be used for the excitation of light, converting electron energy to photon energy. STM based single-molecule…

Optics · Physics 2019-01-01 Yao Zhang , Yang Zhang , Zhenchao Dong

$^{229}$Th, a crucial candidate for nuclear clocks and many other applications, is a typical heavy nucleus with an extremely low-energy isomeric state $^{229m}$Th. A detailed study of the nuclear structure of $^{229}$Th is performed here by…

Nuclear Theory · Physics 2025-08-28 Zi-Rui Chen , Long-Jun Wang , Yuanbin Wu

In-source resonance ionization spectroscopy was used to identify an efficient and selective three step excitation/ionization scheme of thorium, suitable for titanium:sapphire (Ti:sa) lasers. The measurements were carried out in preparation…

The molecular dark state participates in many important photon-induced processes, yet is typically beyond the optical-spectroscopic measurement due to the forbidden transition dictated by the selection rule. In this work, we propose to use…

Quantum Physics · Physics 2021-11-09 Guohui Dong , Zhubin Hu , Xiang Sun , Hui Dong

The low-lying isomeric state of $^{229}$Th provides unique opportunities for high-resolution laser spectroscopy of the atomic nucleus. We determine the energy of this isomeric state by taking the absolute energy difference between the…

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