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We report on the creation of ultracold 84Sr2 molecules in the electronic ground state. The molecules are formed from atom pairs on sites of an optical lattice using stimulated Raman adiabatic passage (STIRAP). We achieve a transfer…

Quantum Gases · Physics 2012-09-18 Simon Stellmer , Benjamin Pasquiou , Rudolf Grimm , Florian Schreck

In this work we model and realize stimulated Raman adiabatic passage (STIRAP) in the diatomic $\mathrm{^{23}Na^{40}K}$ molecule from weakly bound Feshbach molecules to the rovibronic ground state via the…

We report the creation of ultracold samples of $^{39}$K$^{133}$Cs molecules in their rovibrational ground state. By investigating potentially suitable excited states using one- and two-photon spectroscopy, we have identified a pathway to…

A quantum gas of ultracold polar molecules, with long-range and anisotropic interactions, would not only enable explorations of a large class of many-body physics phenomena, but could also be used for quantum information processing. We…

We suggest and analyze a novel technique for efficient and robust creation of dense ultracold molecular ensembles in their ground rovibrational state. In our approach a molecule is brought to the ground state through a series of…

Quantum Physics · Physics 2009-11-13 Elena Kuznetsova , Philippe Pellegrini , Robin Côté , M. D. Lukin , S. F. Yelin

We develop a complete theoretical description of photoassociative Stimulated Raman Adiabatic Passage (STIRAP) near a Feshbach resonance in a thermal atomic gas. We show that it is possible to use low intensity laser pulses to directly…

Quantum Physics · Physics 2015-05-13 Elena Kuznetsova , Susanne F. Yelin , Marko Gacesa , Philippe Pellegrini , Robin Côté

We produce ultracold dense trapped samples of 87Rb133Cs molecules in their rovibrational ground state, with full nuclear hyperfine state control, by stimulated Raman adiabatic passage (STIRAP) with efficiencies of 90%. We observe the onset…

We report efficient all-optical creation of an ultracold gas of alkaline-earth-metal dimers, $^{88}\rm{Sr}_2$, in their absolute ground state. Starting with weakly bound singlet molecules formed by narrow-line photoassociation in an optical…

Atomic Physics · Physics 2021-11-01 K. H. Leung , E. Tiberi , B. Iritani , I. Majewska , R. Moszynski , T. Zelevinsky

Using the technique of stimulated Raman adiabatic passage (STIRAP) we have coherently transferred ultracold 87Rb2 Feshbach molecules into a more deeply bound vibrational quantum level. Our measurements indicate a high transfer efficiency of…

Other Condensed Matter · Physics 2009-11-11 K. Winkler , F. Lang , G. Thalhammer , P. v. d. Straten , R. Grimm , J. Hecker Denschlag

A narrow-linewidth, dual-wavelength laser system is vital for the creation of ultracold ground state molecules via stimulated Raman adiabatic passage (STIRAP) from a weakly bound Feshbach state. Here we describe how a relatively simple…

Atomic Physics · Physics 2015-05-21 P. D. Gregory , P. K. Molony , M. P. Köppinger , A. Kumar , Z. Ji , B. Lu , A. L. Marchant , S. L. Cornish

Ultracold LiCs molecules in the absolute ground state X$^1\Sigma^+$, v"=0, J"=0 are formed via a single photo-association step starting from laser-cooled atoms. The selective production of v"=0, J"=2 molecules with a 50-fold higher rate is…

Quantum Physics · Physics 2010-08-09 J. Deiglmayr , A. Grochola , M. Repp , K. Mörtlbauer , C. Glück , J. Lange , O. Dulieu , R. Wester , M. Weidemüller

One possibility for the creation of ultracold, high-phase-space-density quantum gases of molecules in the rovibrational ground state relies on first associating weakly-bound molecules from quantum-degenerate atomic gases on a Feshbach…

We create fermionic dipolar $^{23}$Na$^6$Li molecules in their triplet ground state from an ultracold mixture of $^{23}$Na and $^6$Li. Using magneto-association across a narrow Feshbach resonance followed by a two-photon STIRAP transfer to…

We associate Sr atom pairs on sites of a Mott insulator optically and coherently into weakly-bound ground-state molecules, achieving an efficiency above 80\%. This efficiency is 2.5 times higher than in our previous work [S. Stellmer, B.…

Quantum Gases · Physics 2017-07-25 Alessio Ciamei , Alex Bayerle , Chun-Chia Chen , Benjamin Pasquiou , Florian Schreck

We report on a resonantly coupled 2(1) - 4 (1) photoassociation resonance in LiRb. This pair of states displays interesting decay physics that hint at interference-like effects caused by two different decay paths. We observe decay to…

Atomic Physics · Physics 2016-12-28 I. C. Stevenson , D. Blasing , Y. P. Chen , D. S. Elliott

Ultracold ground state dipolar 40K-87Rb molecules have recently been produced in a loose harmonic trap by employing a magnetic field sweep across a Feshbach resonance followed by stimulated Raman adiabatic passage [K.-K. Ni et al., Science…

We discuss the production of ultracold molecules in their electronic ground state by photoassociation employing electronically excited states with ion-pair character and strong spin-orbit interaction. A short photoassociation laser pulse…

Chainwise stimulated Raman adiabatic passage (C-STIRAP) in M-type molecular system is a good alternative in creating ultracold deeply-bound molecules when the typical STIRAP in {\Lambda}-type system does not work due to weak Frank-Condon…

Quantum Physics · Physics 2024-08-06 Jiahui Zhang , Li Deng , Yueping Niu , Shangqing Gong

We propose an improved photoassociation scheme to produce ultracold molecules in their vibronic ground state for the generic case where non-adiabatic effects facilitating transfer to deeply bound levels are absent. Formation of molecules is…

Atomic Physics · Physics 2008-10-28 Christiane P. Koch , Robert Moszynski

In this study, we investigate the structure of the polar alkali-Strontium diatomic molecules as possible candidates for the realization of samples of new species of ultracold polar molecules. Using a quantum chemistry approach based on…

Atomic and Molecular Clusters · Physics 2015-05-19 Romain Guérout , Mireille Aymar , Olivier Dulieu
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