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The study and prediction of chemical reactivity is one of the most important application areas of molecular quantum chemistry. Large-scale, fully error-tolerant quantum computers could provide exact or near-exact solutions to the underlying…

Quantum Physics · Physics 2019-09-12 Michael Kühn , Sebastian Zanker , Peter Deglmann , Michael Marthaler , Horst Weiß

Recent experiments have revealed the profound effect of strong light-matter interactions in optical cavities on the electronic ground state of molecular systems. This phenomenon, known as vibrational strong coupling (VSC), can modify…

Quantum Physics · Physics 2023-12-19 Thomas Schnappinger , Markus Kowalewski

We develop a microscopic quantum theory of surface plasmon polaritons valid for arbitrary metal-dielectric geometries. Our framework is based on the Power-Zienau-Woolley representation of quantum electrodynamics, which provides an optimal…

Classical-quantum computational complexity separations are an important motivation for the long-term development of digital quantum computers, but classical-quantum complexity equivalences are just as important in our present era of noisy…

Quantum Physics · Physics 2020-03-10 Jonathan E. Moussa

Variational quantum eigensolvers (VQEs) are successful algorithms for studying physical systems on quantum computers. Recently, they were extended to the measurement-based model of quantum computing, bringing resource graph states and their…

Quantum Physics · Physics 2024-06-27 Albie Chan , Zheng Shi , Luca Dellantonio , Wolfgang Dür , Christine A. Muschik

Large-scale variational quantum algorithms are widely recognized as a potential pathway to achieve practical quantum advantages. However, the presence of quantum noise might suppress and undermine these advantages, which blurs the…

Quantum Physics · Physics 2024-09-20 Yuguo Shao , Fuchuan Wei , Song Cheng , Zhengwei Liu

A coupled quantum dot--nanocavity system in the weak coupling regime of cavity quantumelectrodynamics is dynamically tuned in and out of resonance by the coherent elastic field of a $f_{\rm SAW}\simeq800\,\mathrm{MHz}$ surface acoustic…

State-of-the-art noisy digital quantum computers can only execute short-depth quantum circuits. Variational algorithms are a promising route to unlock the potential of noisy quantum computers since the depth of the corresponding circuits…

Solid-state quantum emitters, such as quantum dots, color centers, rare-earth dopants, and organic molecules, offer qubit systems that integrate well with chip-scale photonic and electronic devices. To fully harness their potential for…

Quantum Physics · Physics 2024-12-16 Kinfung Ngan , Shuo Sun

A semiclassical simulation approach is presented for studying quantum noise in large-scale photonic circuits incorporating an ideal Kerr nonlinearity. A circuit solver is used to generate matrices defining a set of stochastic differential…

Quantum Computing is believed to be the ultimate solution for quantum chemistry problems. Before the advent of large-scale, fully fault-tolerant quantum computers, the variational quantum eigensolver~(VQE) is a promising heuristic quantum…

Quantum Physics · Physics 2023-12-06 Chu Guo , Yi Fan , Zhiqian Xu , Honghui Shang

The variational quantum eigensolver (VQE) is an algorithm to compute ground and excited state energy of quantum many-body systems. A key component of the algorithm and an active research area is the construction of a parametrized trial…

The paradigm of $N$ quantum emitters coupled to a single cavity mode appears in many situations ranging from quantum technologies to polaritonic chemistry. The ideal case of identical emitters is elegantly modeled in terms of symmetric…

We present a quantum-analogous experimental demonstration of variational quantum process tomography using an optical processor. This approach leverages classical one-hot encoding and unitary decomposition to perform the variational quantum…

Quantum Physics · Physics 2025-07-14 Vladlen Galetsky , Paul Kohl , Janis Nötzel

This work studies pulse based variational quantum algorithms (VQAs), which are designed to determine the ground state of a quantum mechanical system by combining classical and quantum hardware. In contrast to more standard gate based…

Quantum Physics · Physics 2023-02-01 Robert de Keijzer , Oliver Tse , Servaas Kokkelmans

With the aim of establishing a framework to efficiently perform the practical application of quantum chemistry simulation on near-term quantum devices, we envision a hybrid quantum--classical framework for leveraging problem decomposition…

We introduce a generalization of the quantum electrodynamic coupled cluster (QED-CC)wave function ansatz, to describe the strongly coupled light-matter system in an unpolarized optical Fabry-P\'erot cavity. This is achieved by explicitly…

Quantum Physics · Physics 2025-07-28 Laurenz Monzel , Stella Stopkowicz

Variational quantum algorithms (VQA) are considered as some of the most promising methods to determine the properties of complex strongly correlated quantum many-body systems, especially from the perspective of devices available in the near…

Quantum Physics · Physics 2022-12-07 Saad Yalouz , Bruno Senjean , Filippo Miatto , Vedran Dunjko

In this article, we introduce a framework for entanglement quantification of photon pairs represented by two-qubit Werner states. The measurement scheme is based on the symmetric informationally complete POVM. To make the framework…

Quantum Physics · Physics 2021-06-22 Artur Czerwinski

The challenge of building a scalable quantum processor requires consolidation of the conflicting requirements of achieving coherent control and preservation of quantum coherence in a large scale quantum system. Moreover, the system should…

Quantum Physics · Physics 2007-05-23 A. Andre , D. DeMille , J. M. Doyle , M. D. Lukin , S. E. Maxwell , P. Rabl , R. Schoelkopf , P. Zoller
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