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The packing geometry of macromolecules in complex mesophases is of key importance to self-organization in synthetic and biological soft materials. While approximate or heuristic models rely on often-untested assumptions about how flexible…

Soft Condensed Matter · Physics 2023-10-05 Benjamin R. Greenvall , Michael S. Dimitriyev , Gregory M. Grason

Molecular simulations provide an effective route for investigating morphology evolution and structure-property relationship in polymer-clay nanocomposites (PCNCs) incorporating layered silicates like montmorillonite (MMT), an important…

Soft Condensed Matter · Physics 2025-06-27 Parvez Khana , Ankit Patidara , Gaurav Goel

Electron-electron interactions in topological p-n junctions consisting of vertically stacked topological insulators are investigated. n-type Bi2Te3 and p-type Sb2Te3 of varying relative thicknesses are deposited using molecular beam epitaxy…

Microfluidic channels are integral to biomedical technology and process engineering, offering versatility in handling fluids with complex properties, often a combination of viscous and elastic attributes. Despite significant advancements in…

Soft Condensed Matter · Physics 2025-09-29 Sampad Laha , Siddhartha Mukherjee , Suman Chakraborty

Almost all the polymer crystals have several polymorphic modifications. Their structure and existence conditions, as well as transitions between them are not understood even in the case of the 'model' polymer polyethylene (PE). For analysis…

Materials Science · Physics 2011-09-06 Elena A. Zubova , Alexander V. Savin , Nikolay K. Balabaev

Theoretical aspects of polymers in mixed solvents are considered using the Edwards Hamiltonian formalism. Thermodynamic and structural properties are investigated and some predictions are made when the mixed solvent approaches criticality.…

Soft Condensed Matter · Physics 2007-05-23 A. Negadi , A. Sans-Penninckx , M. Bemouna , T. A. Vilgis

The behavior of polyampholytes near a charged planar surface is studied by means of Monte Carlo simulations. The investigated polyampholytes are overall electrically neutral and made up of oppositely charged units (called blocks) that are…

Soft Condensed Matter · Physics 2009-11-11 Rene Messina

Despite their considerable practical and biological applications, the link between molecular properties, assembly conditions and self-organized structure in confined polymer solutions remains elusive. Here, we explore the lyotropic nematic…

Soft Condensed Matter · Physics 2023-03-21 Maxime M. C. Tortora , Daniel Jost

The advent of solid state nanodevices allows for interrogating the physico-chemical properties of a polyelectrolyte chain by electrophoretically driving it through a nanopore. Salient dynamical aspects of the translocation process have been…

Soft Condensed Matter · Physics 2015-06-05 A. Rosa , M. Di Ventra , C. Micheletti

We investigate the presence of topological twistons in crystalline polyethylene. We describe crystalline polyethylene with a model that couples the torsional and longitudinal degrees of freedom of the polymeric chain by means of a system of…

Chemical Physics · Physics 2009-11-06 E. Ventura , A. M. Simas , D. Bazeia

Molecular dynamics simulation methods are used to study the folding of polymer chains into packed cubic states. The polymer model, based on a chain of linked sites moving in the continuum, includes both excluded volume and torsional…

Soft Condensed Matter · Physics 2009-11-10 D. C. Rapaport

We apply monomer-resolved computer simulations of supercoiled ring polymers under shear, taking full account of the hydrodynamic interactions, accompanied, in parallel, by simulations in which these are switched off. The combination of…

Soft Condensed Matter · Physics 2024-04-17 Christoph Schneck , Jan Smrek , Christos N. Likos , Andreas Zöttl

We present a detailed study of the static and dynamic behavior of long semiflexible polymer chains in a melt. Starting from previously obtained fully equilibrated high molecular weight polymer melts [{\it Zhang et al.} ACS Macro Lett. 3,…

Soft Condensed Matter · Physics 2016-05-25 Hsiao-Ping Hsu , Kurt Kremer

The equations for strands of rigid charge configurations interacting nonlocally are formulated on the special Euclidean group, SE(3), which naturally generates helical conformations. Helical stationary shapes are found by minimizing the…

Mathematical Physics · Physics 2011-01-06 Steve Benoit , Darryl D. Holm , Vakhtang Putkaradze

Understanding how entanglements affect the behaviour of polymeric complex fluids is an open challenge in many fields. To elucidate the nature and consequence of entanglements in dense polymer solutions, we propose a novel method: a…

Soft Condensed Matter · Physics 2021-01-01 Davide Michieletto , Takahiro Sakaue

We present a novel, self-consistent and robust theoretical model to investigate elastic interactions between topological defects in liquid crystal shells. Accounting for the non-concentric nature of the shell in a simple manner, we are able…

Soft Condensed Matter · Physics 2016-12-14 Alexandre Darmon , Olivier Dauchot , Teresa Lopez-Leon , Michael Benzaquen

A living polymers transition is found in molecular dynamics simulations of a charge-symmetric size-asymmetric electrolyte with no anisotropic interactions. The fluid has strong polymeric character at low temperatures, where it consists of…

Statistical Mechanics · Physics 2007-05-23 Sorin Bastea

The order parameter of the smectic liquid crystal phase is the same as that of a superfluid or superconductor, namely a complex scalar field. We show that the essential difference in boundary conditions between these systems leads to a…

Soft Condensed Matter · Physics 2017-02-08 Randall D. Kamien , Ricardo A. Mosna

We present results of molecular dynamics simulations of strong, flexible polyelectrolyte chains in solution with added salt. The effect of added salt on the polyelectrolyte chain structure is fully treated for the first time as a function…

Soft Condensed Matter · Physics 2008-02-03 Mark J. Stevens , Steve Plimpton

The structural properties of fluids whose molecules interact via potentials with a hard core plus two piece-wise constant sections of different widths and heights are presented. These follow from the more general development previously…

Soft Condensed Matter · Physics 2013-08-27 Andrés Santos , Santos B. Yuste , Mariano López de Haro , Mariana Bárcenas , Pedro Orea