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This paper discusses the elastic behavior of a single polyelectrolyte chain. A simple scaling analysis as in self avoiding walk chains are not possible, because three interplaying relevant length scales are involved, i.e., the Debye…

Statistical Mechanics · Physics 2009-10-30 P. Haronska , J. Wilder , T. A. Vilgis

We investigate the thermodynamic properties of a polyelectrolyte solution in a presence of {\it multivalent} salts. The polyions are modeled as rigid cylinders with the charge distributed uniformly along the major axis. The solution,…

Condensed Matter · Physics 2015-06-25 Paulo S. Kuhn , Yan Levin , Marcia C. Barbosa

The behavior of polyelectrolytes and polyampholytes in semi-dilute solutions is investigated theoretically. Various statistical charge distributions along the polyelectrolyte chains are considered: smeared, annealed, permuted and quenched.…

Soft Condensed Matter · Physics 2007-05-23 I. Borukhov , D. Andelman , H. Orland

The structures of dilute electrolyte solutions close to non-uniformly charged planar substrates are systematically studied within the entire spectrum of microscopic to macroscopic length scales by means of a unified classical density…

Soft Condensed Matter · Physics 2022-11-23 Markus Bier , Maximilian Mußotter , S. Dietrich

The success of topological insulators (TI) in creating devices with unique functionalities is directly connected to the ability of coupling their helical spin states to well defined perturbations. However, up to now, TI-based…

Mesoscale and Nanoscale Physics · Physics 2015-03-12 Thomas Bathon , Paolo Sessi , Konstantin Kokh , Oleg Tereshchenko , Matthias Bode

Light scattering and viscometric measurements on weak polyelectrolytes show two important aspects of counterion condensation, namely, non-monotonic variation in the polyelectrolyte size with the increase in the electrostatic strength, and,…

Statistical Mechanics · Physics 2014-08-12 Prasanta Kundu , Arti Dua

We present a braided circuit topology framework for investigating topology and structural phase transitions in aggregates of semiflexible polymers. In the conventional approach to circuit topology, which specifically applies to single…

Soft Condensed Matter · Physics 2024-02-27 Jonas Berx , Alireza Mashaghi

Studies of the thermodynamics of complex coacervation of pairs of symmetric, strongly ionizable, oppositely charged polyelectrolyte chains are abundant. To generalize such understanding to asymmetric chain lengths and variable ionizability…

Soft Condensed Matter · Physics 2023-06-07 Souradeep Ghosh , Soumik Mitra , Arindam Kundagrami

We study a minimal extension of the worm-like chain to describe polypeptides having alpha-helical secondary structure. In this model presence/absence of secondary structure enters as a scalar variable that controls the local chain bending…

Statistical Mechanics · Physics 2009-11-10 Buddhapriya Chakrabarti , Alex J. Levine

Polyelectrolyte multilayers (PEM) in combination with good electrolyte solvents, e.g., ionic liquids (ILs) are potential candidates for the new generation of electrochemical separators. Swelling PEM with aqueous IL solutions is one way to…

Chemical Physics · Physics 2018-11-20 Nagma Parveen , Pritam Kumar Jana , Monika Schoenhoff

We present an experimentally guided, multi-phase, multi-species polyelectrolyte gel model to make quantitative predictions on the electro-chemical properties of articular cartilage. The mixture theory consists of two different types of…

Tissues and Organs · Quantitative Biology 2013-08-22 Sarthok Sircar , Elizabeth Aisenbrey , Stephanie J. Bryant , David M. Bortz

Strong coupling phenomena, such as the like charged macroions attraction, opposite charged macroions repulsion, charge renormalization or charge inversion, are known to be mediated by multivalent counterions. Most theories treat the…

Soft Condensed Matter · Physics 2016-02-03 Sandipan Dutta , Y. S. Jho

The addition of filler particles to polymer electrolytes is known to increment their ionic conductivity (IC). A detailed understanding of how the interactions between the constituent materials are responsible for the enhancement, remains to…

Materials Science · Physics 2021-03-19 Andres Villa , Juan Carlos Verduzco , Joseph A. Libera , Ernesto E. Marinero

We consider the phase behavior of polymeric systems by calculating the structure factors beyond the Random Phase Approximation. The effect of this correction to the mean-field RPA structure factor is shown to be important in the case of…

Soft Condensed Matter · Physics 2007-05-23 Martin Castelnovo , Jean-Francois Joanny

We investigate theoretically the phase diagram of an insoluble charged surfactant monolayer in contact with a semi-dilute polyelectrolyte solution (of opposite charge). The polyelectrolytes are assumed to have long-range and attractive…

Soft Condensed Matter · Physics 2012-07-19 Adi Shafir , David Andelman

In polymer physics it is typically assumed that excluded volume interactions are effectively screened in polymer melts. Hence, chains could be described by an effective random walk without excluded volume interactions. In this letter, we…

Soft Condensed Matter · Physics 2017-10-31 Hendrik Meyer , Eric Horwath , Peter Virnau

We study the influence of truncating the electrostatic interactions in a fully hydrated pure dipalmitoylphosphatidylcholine (DPPC) bilayer through 20 ns molecular dynamics simulations. The computations in which the electrostatic…

Soft Condensed Matter · Physics 2009-11-07 M. Patra , M. Karttunen , M. Hyvonen , E. Falck , P. Lindqvist , I. Vattulainen

Sliding-induced topological transitions in biphenylene bilayers are investigated, considering various stacking configurations which are analyzed from a symmetry perspective and described in detail,highlighting the intricate patterns of…

Mesoscale and Nanoscale Physics · Physics 2025-12-01 L. L. Lage , S. Bravo , O. Arroyo-Gascón , Leonor Chico , A. Latgé

The effect of chain topology on the statics and dynamics of chain at the interface of two immiscible fluids is studied by means of molecular dynamics simulations. For three topologically different chains, namely, linear, ring, and…

Soft Condensed Matter · Physics 2024-08-01 Jenis Thongam , Lenin S. Shagolsem

We investigate the influence of a non-ionic surfactant like polymer on phospholipid vesicles. Our results from cryogenic transmission electron microscopy (cryo-TEM), dynamic light scattering (DLS), small angle neutron and X-ray scattering…