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We successfully synthesized ($p$-Py-V)[Cu(hfac)$_2$], a verdazyl-based complex. Molecular orbital calculations revealed five types of intermolecular interactions between the radical spins and two types of intramolecular interactions between…

We present a new model compound with the S = 1/2 frustrated square lattice composed of the charge-transfer salt (o-MePy-V)PF6. Ab initio calculations indicate the formation of an S = 1/2 square lattice, in which six types of…

Strongly Correlated Electrons · Physics 2018-09-26 H. Yamaguchi , Y. Sasaki , T. Okubo , M. Yoshida , T. Kida , M. Hagiwara , Y. Kono , S. Kittaka , T. Sakakibara , M. Takigawa , Y. Iwasaki , Y. Hosokoshi

We investigated the isotropic spin-1/2 Heisenberg model on an anisotropic square lattice with competing exchange interactions, motivated by the unconventional magnetic behavior observed in the verdazyl-based compound (o-MePy-V)PF6. Using a…

Strongly Correlated Electrons · Physics 2025-11-21 L. M. Ramos , M. Schmidt , F. M. Zimmer

We present a model compound with a spin-1/2 frustrated square lattice, in which three ferromagnetic (F) interactions and one antiferromagnetic (AF) compet. Considering the effective spin-1 formed by the dominant F dimer, this square lattice…

Strongly Correlated Electrons · Physics 2021-08-31 H. Yamaguchi , N. Uemoto , T. Okubo , Y. Kono , S. Kittaka , T. Sakakibara , T. Yajima , S. Shimono , Y. Iwasaki , Y. Hosokoshi

The magnetization process of a frustrated spin-1/2 spin-dimer model on a square lattice is investigated by means of a sign-problem-free quantum Monte Carlo algorithm developed recently. Rich field-induced quantum phases are discovered. We…

Strongly Correlated Electrons · Physics 2017-03-02 Kwai-Kong Ng , Min-Fong Yang

We present Quantum Monte-Carlo simulations of an exchange-anisotropic spin-1/2 Heisenberg model on a square lattice with nearest and next-nearest neighbor interactions. The ground state phase diagram shows two classical magnetically ordered…

Strongly Correlated Electrons · Physics 2012-12-20 A. Kalz , A. Honecker , S. Fuchs , T. Pruschke

By means of the recently developed algorithm based on the tensor product states, the magnetization process of frustrated spin-1/2 spin-dimer models on a square lattice is investigated. Various field-induced quantum phases are discovered. In…

Strongly Correlated Electrons · Physics 2010-01-26 Pochung Chen , Chen-Yen Lai , Min-Fong Yang

We introduce a model compound featuring a spin-1/2 frustrated square lattice partially coupled by spin-5/2. A significant magnetization plateau exceeding 60 T could be observed, indicating a quantum state formed by $S$ = 1/2 spins in the…

Motivated by theoretical and experimental studies reported by Yamaguchi et al. (Phys. Rev. B 98, 094402 (2018)), we performed a cluster mean-field analysis of an anisotropic Heisenberg model with six competing exchange interactions. We…

Strongly Correlated Electrons · Physics 2025-07-04 L. M. Ramos , F. M. Zimmer , M. Schmidt

We study the impact of the diagonal frustrating couplings on the quantum phase diagram of a two-leg ladder composed of alternating spin-1 and spin-1/2 rungs. As the coupling strength is increased the system successively exhibits two gapped…

Strongly Correlated Electrons · Physics 2015-05-14 V. Ravi Chandra , N. B. Ivanov , J. Richter

We present a model compound with a spin-1/2 spatially anisotropic frustrated square lattice, in which three antiferromagnetic interactions and one ferromagnetic interaction are competing. We observe an unconventional gradual increase in the…

Strongly Correlated Electrons · Physics 2021-06-24 H. Yamaguchi , Y. Iwasaki , Y. Kono , T. Okubo , S. Miyamoto , Y. Hosokoshi , A. Matsuo , T. Sakakibara , T. Kida , M. Hagiwara

We report on high-field magnetization measurements for a number of layered vanadium phosphates that were recently recognized as spin-1/2 frustrated square lattice compounds with ferromagnetic nearest-neighbor couplings (J_1) and…

Strongly Correlated Electrons · Physics 2010-10-28 Alexander A. Tsirlin , Burkhard Schmidt , Yurii Skourski , Ramesh Nath , Christoph Geibel , Helge Rosner

A mixed Heisenberg spin chain with frustrated side chains is investigated by numerical and perturbational calculations. A frustration-induced quantum partially polarized ferrimagnetic phase and a nonmagnetic spin quadrupolar phase are found…

Strongly Correlated Electrons · Physics 2008-08-12 Kazuo Hida , Ken'ichi Takano

We investigate quantum phase transitions among the spin-gap phases and the magnetically ordered phases in a two-dimensional frustrated antiferromagnetic spin system, which interpolates several important models such as the orthogonal-dimer…

Strongly Correlated Electrons · Physics 2009-11-07 Yoshihiro Takushima , Akihisa Koga , Norio Kawakami

We study the frustrated dimer-plaquette quantum spin chain for ferromagnetic dimer bonds. This quantum system undergoes a series of first-order ground-state phase transitions driven by frustration or by a magnetic field. We find that the…

Strongly Correlated Electrons · Physics 2009-11-07 J. Schulenburg , J. Richter

We report magnetocaloric and magnetic-torque evidence that in Cs$_{2}$CuBr$_{4}$ -- a geometrically frustrated Heisenberg $S=1/2$ triangular-lattice antiferromagnet -- quantum fluctuations stabilize a series of spin states at simple…

Strongly Correlated Electrons · Physics 2015-05-13 N. A. Fortune , S. T. Hannahs , Y. Yoshida , T. E. Sherline , T. Ono , H. Tanaka , Y. Takano

Although the frustrated spin chain (zigzag chain) is a Drosophila of frustrated magnetism, the understanding of a pair of coupled zigzag chains (frustrated spin ladder) in a magnetic field is incomplete. We address this problem through…

Strongly Correlated Electrons · Physics 2021-10-05 M. Pikulski , T. Shiroka , F. Casola , A. P. Reyes , P. L. Kuhns , S. Wang , H. -R. Ott , J. Mesot

We propose a new type of magnetically disordered ground state for a frustrated quantum antiferromagnet. This disordered state is an array of spin singlets spontaneously formed on four spin plaquettes. Both perturbation results and…

Condensed Matter · Physics 2009-10-28 M. E. Zhitomirsky , Kazuo Ueda

Frustrated spin ladders show magnetization plateaux depending on the rung-exchange interaction and frustration defined by the ratio of first and second neighbor exchange interactions in each chain. This paper is the first report on its…

Strongly Correlated Electrons · Physics 2018-05-09 T. Sugimoto , M. Mori , T. Tohyama , S. Maekawa

We study the zero-temperature phase diagram of the frustrated square-lattice S=1/2 antiferromagnet in an external magnetic field numerically with the Lanczos algorithm. For strong frustration, we find disordered phases at high (and low)…

Strongly Correlated Electrons · Physics 2009-10-31 A. Honecker
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