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Magnetic materials have been applied in a large variety of technologies, from data storage to quantum devices. The development of 2D materials has opened new arenas for magnetic compounds, even when classical theories discourage their…

Materials Science · Physics 2022-02-11 Carlos Mera Acosta , Elton Ogoshi , Jose Antonio Souza , Gustavo M. Dalpian

We present a perspective on the status of antiferromagnetism in two-dimensional (2D) materials. Various types of spin-compensated orders are discussed and include non-collinear order, spin spirals and altermagnetism. Spin-orbit effects…

Materials Science · Physics 2024-08-09 Thomas Olsen

The recent observation of ferromagnetic order in two-dimensional (2D) materials has initiated a booming interest in the subject of 2D magnetism. In contrast to bulk materials, 2D materials can only exhibit magnetic order in the presence of…

Materials Science · Physics 2020-02-18 Daniele Torelli , Kristian S. Thygesen , Thomas Olsen

Magnetic materials often exhibit complex energy landscapes with multiple local minima, each corresponding to a self-consistent electronic structure solution. Finding the global minimum is challenging, and heuristic methods are not always…

We present a computational search for spin spiral ground states in two-dimensional transition metal halides that are experimentally known as van der Waals bonded bulk materials. Such spin spirals break the rotational symmetry of the lattice…

Materials Science · Physics 2023-06-14 Joachim Sødequist , Thomas Olsen

The magnetic properties of the pyrochlore iridate material Eu$_2$Ir$_2$O$_7$ (5$d^5$) have been studied based on the first principle calculations, where the crystal field splitting $\Delta$, spin-orbit coupling (SOC) $\lambda$ and Coulomb…

Strongly Correlated Electrons · Physics 2017-11-08 Yilin Wang , Hongming Weng , Liang Fu , Xi Dai

We calculate the orbital magnetization of 822 two-dimensional magnetic materials from the Computational 2D Materials Database (C2DB). For compounds containing 5$d$ elements we find orbital moments of the order of 0.3-0.5 $\mu_\mathrm{B}$,…

Materials Science · Physics 2024-11-11 Martin Ovesen , Thomas Olsen

Stabilization of unusual spin-orbit driven magnetic orderings are achieved for chains of Mn atoms deposited on a W(110) substrate. First-principles electronic structure calculations show that the ground state spin configuration is…

We present a high throughput computational search for altermagnetism in two-dimensional (2D) materials based on the Computational 2D Materials Database (C2DB). We start by showing that the symmetry requirements for altermagnetism in 2D are…

Materials Science · Physics 2024-08-09 Joachim Sødequist , Thomas Olsen

Magnetic ordering phenomena have a profound influence on the macroscopic properties of correlated-electron materials, but their realistic prediction remains a formidable challenge. An archetypical example is the ternary nickel oxide system…

We present the results of a muon-spin relaxation (muSR) investigation into magnetic ordering in several families of layered quasi-two-dimensional molecular antiferromagnets based on transition metal ions such as S=1/2 Cu2+ bridged with…

We employ density functional theory within a non-collinear framework to investigate the magnetic properties of the octanuclear molecular rings Cr$_8$ and V$_8$. Our aim is to generalize the evaluation of the effective magnetic interactions…

Materials Science · Physics 2026-04-28 Maria Barbara Maccioni , Elia Stocco , Luca Binci , Andrea Floris , Matteo Cococcioni

We investigate the chiral magnetic order in free-standing planar 3$d$-5$d$ bi-atomic metallic chains (3$d$: Fe, Co; 5$d$: Ir, Pt, Au) using first-principles calculations based on density functional theory. We found that the antisymmetric…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Vikas Kashid , Timo Schena , Bernd Zimmermann , Yuriy Mokrousov , Stefan Blügel , Vaishali Shah , H. G. Salunke

Two-dimensional metallic altermagnets are rare, and no correlated 2D material has been established to host large nonrelativistic spin splitting. Here we show that spontaneous orbital order, driven by electronic correlations and Fermi…

Mesoscale and Nanoscale Physics · Physics 2026-03-27 Nirmalya Jana , Atasi Chakraborty , Anamitra Mukherjee , Amit Agarwal

The realization of long-range spin order in two-dimensions (2D) has catapulted the search for layered materials with magnetic ordering above room temperature. These efforts aim to understand and enhance the spin spin interactions in 2D. An…

Materials Science · Physics 2025-12-23 Rabindra Basnet , Ramesh C. Budhani

We investigate the necessary conditions for the emergence of complex, noncoplanar magnetic configurations in a Kondo lattice model with classical local moments on the geometrically frustrated Shastry-Sutherland lattice and their evolution…

Strongly Correlated Electrons · Physics 2017-12-05 Munir Shahzad , Pinaki Sengupta

Altermagnetism, as an unconventional antiferromagnetism, exhibits collinear-compensated magnetic order in real space and spin-splitting band structure in reciprocal space. In this work, we propose a general approach to generating…

Materials Science · Physics 2025-05-15 Hongjie Peng , Sike Zeng , Ji-Hai Liao , Chang-Chun He , Xiao-Bao Yang , Yu-Jun Zhao

Density-functional calculations are carried out to investigate incommensurate magnetic structures and ferroelectric polarization in newly discovered multiferroic material MnI$_2$. The exchange interactions among local moments on Mn are…

Strongly Correlated Electrons · Physics 2013-05-30 Xianxin Wu , Yingxiang Cai , Qing Xie , Hongming Weng , Heng Fan , Jiangping Hu

Within the framework of the $s$-$d(f)$ exchange model in the mean-field approximation for square, simple cubic, body-centered and face-centered cubic lattices, the formation of a ferromagnetic, spiral, and commensurate antiferromagnetic…

Strongly Correlated Electrons · Physics 2021-07-14 A. K. Pankratova , P. A. Igoshev , V. Yu. Irkhin

The terminology "altermagnetism" has recently been adopted to describe collinear magnetic order with no net magnetization and non-relativisitic, momentum-dependent spin-splitting. The archetypal material used to theoretically explore…

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