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Correlation-Driven Orbital Order Realizes 2D Metallic Altermagnetism

Mesoscale and Nanoscale Physics 2026-03-27 v1 Materials Science Strongly Correlated Electrons

Abstract

Two-dimensional metallic altermagnets are rare, and no correlated 2D material has been established to host large nonrelativistic spin splitting. Here we show that spontaneous orbital order, driven by electronic correlations and Fermi surface nesting, provides a general microscopic route to two-dimensional metallic altermagnetism. Antiferro-orbital ordering between the dxz_{xz} and dyz_{yz} orbitals breaks the equivalence of magnetic sublattices with opposite spins and generates a symmetry-enforced altermagnetic spin texture. As a concrete realization, we identify monolayer YbMn2_2Ge2_2 as a stable correlated metallic altermagnet exhibiting giant nonrelativistic spin splitting of order 1 eV. The resulting phase supports an exceptionally large and gate-tunable transverse spin conductivity. These results establish correlation-driven orbital order as a robust and general mechanism for designing correlated altermagnets with large spin splitting.

Keywords

Cite

@article{arxiv.2603.25426,
  title  = {Correlation-Driven Orbital Order Realizes 2D Metallic Altermagnetism},
  author = {Nirmalya Jana and Atasi Chakraborty and Anamitra Mukherjee and Amit Agarwal},
  journal= {arXiv preprint arXiv:2603.25426},
  year   = {2026}
}

Comments

8 pages, 5 figures, comments and suggestions are welcome

R2 v1 2026-07-01T11:39:14.203Z