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Achieving multiferroic two-dimensional (2D) materials should enable numerous functionalities in nanoscale devices. Until now, however, predicted 2D multiferroics are very few and with coexisting yet only loosely coupled (type-I)…

Materials Science · Physics 2019-07-11 Jun-Jie Zhang , Linfang Lin , Yang Zhang , Menghao Wu , Boris I. Yakobson , Shuai Dong

Two-dimensional (2D) multiferroics exhibit cross-control capacity between magnetic and electric responses in reduced spatial domain, making them well suited for next-generation nanoscale devices; however, progress has been slow in…

Materials Science · Physics 2020-05-15 Jing Shang , Chun Li , Aijun Du , Ting Liao , Yuantong Gu , Yandong Ma , Liangzhi Kou , Changfeng Chen

The structurally related compounds NiI$_2$ and CoI$_2$ are multiferroic van der Waals materials, in which helimagnetic orders exist simultaneously with electric polarization. Here, we report on the evolution of the crystal structure and of…

A reduced dimensionality of multiferroic materials is highly desired for device miniaturization, but the coexistence of ferroelectricity and magnetism at the two-dimensional limit is yet to be conclusively demonstrated. Here, we used a…

Magnetic ordering in the two-dimensional limit has been one of the most important issues in condensed matter physics for the past several decades. The recent discovery of new magnetic van der Waals materials heralds a much-needed easy route…

We present a computational search for spin spiral ground states in two-dimensional transition metal halides that are experimentally known as van der Waals bonded bulk materials. Such spin spirals break the rotational symmetry of the lattice…

Materials Science · Physics 2023-06-14 Joachim Sødequist , Thomas Olsen

The realization of multiferroics in nanostructures, combined with a large electric dipole and ferromagnetic ordering, could lead to new applications, such as high-density multi-state data storage. Although multiferroics have been broadly…

Materials Science · Physics 2018-04-18 Chengxi Huang , Yongping Du , Haiping Wu , Hongjun Xiang , Kaiming Deng , Erjun Kan

Magnetoelectric coupling in insulating multiferroic materials is invaluable for both fundamental research and multifunctional device applications. However, material realization remains a significant challenge. We employ first-principles…

Materials Science · Physics 2025-07-08 Xilong Xu , Li Yang

Nowadays, designing and searching for materials with multiple functional characteristics are the key to achieving high-performance electronic devices. Among many candidates, two-dimensional multiferroic materials have great potential to be…

Materials Science · Physics 2020-11-03 Hai-Peng You , Ning Ding , Jun Chen , Shuai Dong

The coexistence of multiple ferroic orders, i.e. multiferroicity, is a scarce property to be found in materials. Historically, this state has been found mainly in 3-dimensional complex oxides, but so far this state has still been elusive…

Contribution of d-electron to ferroelectricity of type-II multiferroics causes strong magneto-electric coupling and distinguishes them from the conventional type-I multiferroics. However, their therein polarization is too small because the…

Materials Science · Physics 2019-06-05 Hengxin Tan , Menglei Li , Haitao Liu , Zhirong Liu , Yuanchang Li , Wenhui Duan

The realization of two-dimensional multiferroics offers significant potential for nanoscale device functionality. However, type-I two-dimensional multiferroics with strong magnetoelectric coupling, enabling electric field control of spin,…

Materials Science · Physics 2025-01-24 Wei Li , Dongyang Zhu , Shuai Dong , Jun-Jie Zhang

Since the discovery of graphene, two-dimensional materials with atomic level thickness have rapidly grown to be a prosperous field of physical science with interdisciplinary interests, for their fascinating properties and broad…

Materials Science · Physics 2020-11-20 Ming An , Shuai Dong

Low-dimensional multiferroicity, though highly scarce in nature, has attracted great attention due to both fundamental and technological interests. Using first-principles density functional theory, we show that ferromagnetism and…

Materials Science · Physics 2018-07-26 Jingshan Qi , Hua Wang , Xiaofang Chen , Xiaofeng Qian

Layered van der Waals materials have risen as powerful platforms to artificially engineer correlated states of matter. Here we show the emergence of a multiferroic order in a twisted dichalcogenide bilayer superlattice at quarter-filling.…

Strongly Correlated Electrons · Physics 2022-09-07 Mikael Haavisto , J. L. Lado , Adolfo O. Fumega

Much is known about the magnetoelectric effect of multiferroic insulators, yet little is understood about multiferroic metals. In this work, we employ first-principles calculations to identify the sliding van der Waals bilayer $1T$-NbTe$_2$…

Materials Science · Physics 2025-10-28 Zefei Han , Haojin Wang , Yuanchang Li

The family of monolayer two-dimensional (2D) materials hosts a wide range of interesting phenomena, including superconductivity, charge density waves, topological states and ferromagnetism, but direct evidence for antiferromagnetism in the…

Materials Science · Physics 2021-10-12 Zhuoliang Ni , A. V. Haglund , H. Wang , B. Xu , C. Bernhard , D. G. Mandrus , X. Qian , E. J. Mele , C. L. Kane , Liang Wu

Two-dimensional antiferromagnetism has long attracted significant interest in many areas of condensed matter physics, but only recently has experimental exploration become feasible due to the isolation of van der Waals antiferromagnetic…

Mesoscale and Nanoscale Physics · Physics 2025-11-21 Cheol-Yeon Cheon , Volodymyr Multian , Kenji Watanabe , Takashi Taniguchi , Alberto F. Morpurgo , Dmitry Lebedev

Stacking order can significantly influence the physical properties of two-dimensional (2D) van der Waals materials. The recent isolation of atomically thin magnetic materials opens the door for control and design of magnetism via stacking…

Two-dimensional (2D) van der Waals (vdW) multiferroics offer an attractive platform for four-state nonvolatile memory by combining switchable ferroelectric polarization and magnetization within a single material system. However, their…

Materials Science · Physics 2026-05-15 Zhibin Tan , Tao Wang , Hao Jin