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The optical excitations in $\rug$ and higher fullerenes, including isomers of C$_{76}$, C$_{78}$, and C$_{84}$, are theoretically investigated. We use a tight binding model with long-range Coulomb interactions, treated by the Hartree-Fock…

Condensed Matter · Physics 2008-02-03 Kikuo Harigaya

We present a simple measurement and analysis technique to determine the fraction of optical loss due to both radiation (scattering) and linear absorption in microphotonic components. The method is generally applicable to optical materials…

Optics · Physics 2009-11-13 Matthew Borselli , Thomas J. Johnson , Oskar Painter

Exciton effects on soliton and bipolaron lattice states are investigated using an electron-lattice Peierls model with long-range Coulomb interactions. The Hartree-Fock (HF) approximation and the single-excitation configuration-interaction…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya , Yukihiro Shimoi , Shuji Abe

Optical information processing and computing can potentially offer enhanced performance, scalability and energy efficiency. However, achieving nonlinearity-a critical component of computation-remains challenging in the optical domain. Here…

In this paper we present an approach aimed at calculating the optical dielectric constant of crystalline insulators both at the Hartree-Fock, and correlated levels. Our scheme employs a real-space methodology, employing Wannier functions as…

Materials Science · Physics 2010-01-14 Priya Sony , Alok Shukla

We have performed first principles electron-correlated calculations employing large basis sets to optimize the geometries, and to compute linear optical absorption spectra of various low-lying conformers of silicon hydrides:…

Atomic and Molecular Clusters · Physics 2019-10-16 Pritam Bhattacharyya , Deepak Kumar Rai , Alok Shukla

In this work we propose a method to perform optimization on manifolds. We assume to have an objective function $f$ defined on a manifold and think of it as the potential energy of a mechanical system. By adding a momentum-dependent kinetic…

Numerical Analysis · Mathematics 2023-08-30 Marta Ghirardelli

The electronic structure of solids can routinely be calculated by standard methods like density functional theory. However, in complicated situations like interfaces, grain boundaries or contact geometries one needs to resort to more…

Materials Science · Physics 2025-11-18 Henrik Dick , Thomas Dahm

A theoretical model of resonant hyper-Raman scattering by an ensemble of spherical semiconductor quantum dots has been developed. The electronic intermediate states are described as Wannier-Mott excitons in the framework of the envelope…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 E. Menendez-Proupin , C. Trallero-Giner , A. Garcia-Cristobal

A procedure is presented that combines density functional theory computations of bulk semiconductor alloys with the semiconductor Bloch equations, in order to achieve an ab initio based prediction of the optical properties of semiconductor…

Materials Science · Physics 2017-06-08 L. C. Bannow , P. Rosenow , P. Springer , E. W. Fischer , J. Hader , J. V. Moloney , R. Tonner , S. W. Koch

A first-principles study on the quasiparticles energy and optical absorption spectrum of fluorographene is presented by employing the GW + Bethe-Salpeter Equation (BSE) method with many-electron effects included. The calculated band gap is…

Mesoscale and Nanoscale Physics · Physics 2019-06-05 Yufeng Liang , Li Yang

Optical properties of materials related to light absorption and scattering are explained by the excitation of electrons. The Bethe-Salpeter equation is the state-of-the-art approach to describe these processes from first principles (ab…

Numerical Analysis · Mathematics 2020-08-21 Peter Benner , Carolin Penke

We present a method to measure the vector-field light scattering of individual microscopic objects. The polarization-dependent optical field images are measured with quantitative phase imaging at the sample plane, and then numerically…

Optics · Physics 2018-04-04 Jaehwang Jung , Jinhyung Kim , Min-kyo Seo , YongKeun Park

One of the challenges of excitonic materials is the accurate determination of the exciton binding energy and bandgap. The difficulty arises from the overlap of the discrete and continuous excitonic absorption at the band edge. Many…

Optimal sampling of non band-limited functions is an issue of great importance that has attracted considerable attention. We propose to tackle this problem through the use of a frequency warping: First, by a nonlinear shrinking of…

Classical Analysis and ODEs · Mathematics 2017-03-07 Stefan Lafon , Jacques Lévy Véhel , Jacques Peyrière

The effect of the non-linear interaction between the high density Wannier excitons is analysed. We use the Fokker-Planck equation in the positive P presentation and the corresponding stochastic differential equation to study the composite…

Quantum Physics · Physics 2015-06-26 Liu Yu-Xi , Cao Chang-Qi

Excitons, Coulomb-bound electron-hole pairs, are the fundamental excitations governing the optoelectronic properties of semiconductors. While optical signatures of excitons have been studied extensively, experimental access to the excitonic…

Many developments in science and engineering depend on tackling complex optimizations on large scales. The challenge motivates intense search for specific computing hardware that takes advantage from quantum features, nonlinear dynamics, or…

Electromagnetic waves propagating in a layered superconductor with arbitrary momentum with respect to the main crystallographic directions display an unavoidable mixing between longitudinal and transverse degrees of freedom. Here we show…

Superconductivity · Physics 2024-06-14 Niccolò Sellati , Jacopo Fiore , Claudio Castellani , Lara Benfatto

In insulators, the method of Marzari and Vanderbilt [Phys. Rev. B {\bf 56}, 12847 (1997)] can be used to generate maximally localized Wannier functions whose centers are related to the electronic polarization. In the case of layered…

Materials Science · Physics 2009-12-17 Xifan Wu , Oswaldo Diéguez , Karin M. Rabe , David Vanderbilt