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We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…

By employing a pump-probe technique for enhanced spectral mapping of the dynamics in nonlinear frequency conversion, we demonstrate that photo-induced second-harmonic generation (SHG) in silicon nitride (Si3N4) microresonators can persist…

We show that the divergence of extreme ultraviolet pulses from high harmonic generation, which is directly linked to the shape and size of the refocused beam, can be controlled by the relative delay between the fundamental and its intense…

Since the new millennium coherent extreme ultra-violet and soft x-ray radiation has revolutionized the understanding of dynamical physical, chemical and biological systems at the electron's natural timescale. Unfortunately, coherent…

We demonstrate a 1.4 W continuous wavelength (CW) laser at 243.1 nm. The radiation is generated through frequency quadrupling the output of a ytterbium-doped fiber amplifier system which produces $>$ 10 W of CW power at 972.5 nm. We…

Atomic Physics · Physics 2018-11-27 Z. Burkley , A. D. Brandt , C. Rasor , S. F. Cooper , D. C. Yost

Recent breakthroughs in high repetition-rate extreme ultraviolet (XUV) light sources and photoelectron analyzers have led to dramatic advances in the performance of time-resolved photoemission experiments. In this perspective article, we…

Optics · Physics 2024-10-16 Thomas K. Allison , Alice Kunin , Gerd Schönhense

Generating widely tunable, continuous wave light at long wavelengths via difference frequency generation (DFG) remains challenging due to high absorption and dispersion. The relatively new platform of thin film lithium niobate enables…

Optics · Physics 2023-06-02 Valerie Yoshioka , Jicheng Jin , Qiang Lin , Bo Zhen

Supercontinuum generation by femtosecond filaments in air is investigated for different laser wavelengths ranging from ultraviolet to infrared. Particular attention is paid on the role of third-harmonic generation and temporal steepening…

Optics · Physics 2008-04-30 S. Skupin , L. Berge

A scheme for generation of monochromatic Cherenkov radiation in a thin dielectric layer is proposed. The electrons travel in vacuum parallel to a dielectric, exciting a single synchronous electromagnetic waveguide mode. The proposed scheme…

Optics · Physics 2025-09-18 Andrzej Szczepkowicz , Po-Wei Kuo , Yen-Cheh Huang

We demonstrate a novel microcavity-based photon up-conversion using second harmonic generation (SHG) from a polar nematic fluid media doped with a laser dye. The present idea is based on coherent light generation via simultaneous frequency…

Optics · Physics 2024-06-11 Daichi Okada , Hiroya Nishikawa , Fumito Araoka

We demonstrate second order optical nonlinearity in a silicon architecture through heterogeneous integration of single-crystalline gallium nitride (GaN) on silicon (100) substrates. By engineering GaN microrings for dual resonance around…

Sub-femtosecond x-ray burst is powerful tool for probing and imaging electronic and concomitant atomic motion in attosecond physics. For years, x-ray source (above 2 keV) had mainly been obtained from X-ray free electron laser (XFEL) or…

We demonstrate second order optical nonlinearity in aluminum nitride on insulator substrates. Using sputter-deposited aluminum nitride thin films we realize nanophotonic waveguides coupled to micro-ring resonators that simultaneously…

Optics · Physics 2012-06-13 W. H. P. Pernice , C. Xiong , C. Schuck , H. X. Tang

We observe a new regime of coherent XUV radiation generation in noble gases induced by femtosecond pulses at very high intensities. This XUV emission has both a reduced divergence and spectral width as compared to high-order harmonic…

Nano-resonator integrated with two-dimensional materials (e.g. transition metal dichalcogenides) have recently emerged as a promising nano-optoelectronic platform. Here we demonstrate resonatorenhanced second-harmonic generation (SHG) in…

We demonstrate that phase-matched frequency upconversion of ultrafast laser light can be extended to shorter wavelengths by using longer driving laser wavelengths. Experimentally, we show that the phase-matching cutoff for harmonic…

Optical second-harmonic generation (SHG) is a nonlinear parametric process that doubles the frequency of incoming light. Only allowed in non-centrosymmetric materials, it has been widely used in frequency modulation of lasers, surface…

Materials Science · Physics 2021-01-05 Wontaek Kim , Je Yhoung Ahn , Juseung Oh , Ji Hoon Shim , Sunmin Ryu

We report on nonlinear frequency conversion from the telecom range via second harmonic generation (SHG) and third harmonic generation (THG) in suspended gallium nitride slab photonic crystal (PhC) cavities on silicon, under continuous-wave…

Vigorous efforts to harness the topological properties of light have enabled a multitude of novel applications. Translating the applications of structured light to higher spatial and temporal resolutions mandates their controlled…

Dielectric metasurfaces have shown prominent applications in nonlinear optics due to strong field enhancement and low dissipation losses at the nanoscale. Chalcogenide glasses are one of the promising materials for the observation of…