Related papers: Phonon-Mediated Third-Harmonic Generation in Diamo…
The addition of a weak oscillating field modifying strongly dressed spins enhances and enriches the system quantum dynamics. Through low-order harmonic mixing the bichromatic driving generates additional rectified static field acting on the…
The implementation of polaritonic materials into nanoscale devices requires selective tuning of parameters to realize desired spectral or thermal responses. One robust material is {\alpha}-MoO3, which as an orthorhombic crystal boasts three…
High-harmonic generation by a laser-driven solid slab is simulated using time-dependent density functional theory. Multiple harmonic plateaus up to very high harmonic orders are observed already at surprisingly low field strengths. The full…
Second and third harmonic signals have been usually generated by using nonlinear crystals, but that method suffers from the low efficiency in small thicknesses. Metamaterials can be used to generate harmonic signals in small thicknesses.…
Aluminum nitride and silicon nitride have recently emerged as important nonlinear optical materials in integrated photonics respectively for their quadratic and cubic optical nonlinearity. A composite aluminum nitride and silicon nitride…
Surface plasmon resonances, the coherent oscillation of free electrons, can concentrate incident field into small volumes much smaller than the incident wavelength. The intense fields at these \textit{hot spots} enhance the light-matter…
In a previous study, we have discovered that nonlinear processes can be enhanced several orders of magnitude due to the path interference effects which are introduced by Fano resonances. Emergence of this phenomenon has been demonstrated…
The Raman effect -- inelastic scattering of light by lattice vibrations (phonons) -- produces an optical response closely tied to a material's crystal structure. Here we show that resonant optical excitation of IR and Raman phonons gives…
Dielectric metasurfaces have shown prominent applications in nonlinear optics due to strong field enhancement and low dissipation losses at the nanoscale. Chalcogenide glasses are one of the promising materials for the observation of…
We explore the outcomes of detailed microscopic models by calculating second- and third-harmonic generation from thin film surfaces with discontinuous free-electron densities. These circumstances can occur in structures consisting of a…
In this work, we investigate the generation of second harmonic light by gold nanorods and demonstrate that the collected nonlinear intensity depends upon a phase interplay between different modes available in the nanostructure. By recording…
The emergence of strong-field nanoplasmonics brings extreme laser field-matter interaction into the realm of nanoscale science, unveiling exciting new physics. Highly nonlinear interaction is enabled by tightly confined electric fields in…
We experimentally demonstrate efficient third harmonic generation from an indium tin oxide (ITO) nanofilm (lambda/42 thick) on a glass substrate for a pump wavelength of 1.4 um. A conversion efficiency of 3.3x10^-6 is achieved by exploiting…
The light scattering properties of superconducting (Tc=3.8 K) heavily boron doped nanocrystalline diamond has been investigated by Raman spectroscopy using visible excitations. Fano type interference of the zone-center phonon line and the…
Third-harmonic generation can be realized via both $\chi^{(3)}$ and cascaded $\chi^{(2)}$ nonlinear processes in a triply-resonant microcavity. It is still unknown how these processes interfere with each other and the optimization of the…
Nonlinear optical frequency conversion, where optical fields interact with a nonlinear medium to generate new frequencies, is a key phenomenon in modern photonic systems. However, a major challenge with these techniques lies in the…
Chiral properties have seen increasing use in recent years, leading to the emerging fields of chiral quantum optics, plasmonics, and phononics. While these fields have achieved manipulation of the chirality of light and lattice vibrations,…
High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…
We study the enhancement of third harmonic generation in indium tin oxide nanolayers coupled to Tamm plasmon polaritons (TPPs). The TPPs are excited at the interface between a thin gold mirror and a silicon dioxide/silicon nitride…
Acoustic vibrations at the nanoscale (GHz-THz frequencies) and their interactions with electrons, photons and other excitations are the heart of an emerging field in physics: nanophononics. The design of ultrahigh frequency acoustic-phonon…