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Nonlinear frequency conversion by optical rectification, as well as difference- and sum-frequency generation are fundamental processes for producing electromagnetic radiation at different frequencies. Here, we demonstrate that coherently…

Hybrid dielectric metasurfaces have emerged as a promising approach to enhancing near field confinement and thus achieving high optical nonlinearity using low loss dielectrics. Additional flexibility in design and fabrication of hybrid…

Light generation through optical harmonics plays a pivotal role in photonics, driving innovations in coherent light sources, biological imaging, and spectroscopy. Traditional methods for tuning optical harmonics, including electrostatic…

Optics · Physics 2025-04-01 George Trivizas , Matthew D. Feinstein , Euclides Almeida

Improving the conversion efficiency is critical for advancing nonlinear photonic devices, enabling applications in ultrafast optics, quantum light sources, and high-resolution imaging. Herein, we present a bilayer waveguide integrated with…

Optics · Physics 2025-08-21 Xin Huang , Qi Lin , Sheng-Xuan Xia , Xiang Zhai , Gui-Dong Liu

The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…

We study the nonlinear process of second harmonic generation in photonic time-crystals, materials with refractive index that varies abruptly and periodically in time, and obtain the phase matching condition for this process. We find…

In recent years, techniques of intense THz laser have enabled us to experimentally observe nonlinear spin dynamics in antiferromagnets since the elementary excitations such as magnons reside on a THz to GHz range in antiferromagnets and THz…

Strongly Correlated Electrons · Physics 2026-04-09 Yuto Jita , Minoru Kanega , Takumi Ogawa , Shunsuke C. Furuya , Masahiro Sato

We investigate high-harmonic generation in graphene heterostructures consisting of metallic nanoribbons separated from a graphene sheet by either a few-nanometer layer of aluminum oxide or an atomic monolayer of hexagonal boron nitride. The…

Noble metals with well-defined crystallographic orientation constitute an appealing class of materials for controlling light-matter interactions on the nanoscale. Nonlinear optical processes, being particularly sensitive to anisotropy, are…

We simulate propagation of phonon-polaritons (admixtures of polar lattice vibrations and electromagnetic waves) in ferroelectric LiNbO3 with a model that consists of a spatially periodic array of harmonic oscillators coupled to THz…

Condensed Matter · Physics 2007-05-23 David W. Ward , Eric Statz , Nikolay Stoyanov , Keith A. Nelson

The active and nonlinear graphene properties are limited due to weak light matter interaction between the ultrathin graphene and the incident light. In this work, we present enhanced nonlinear effects at the low terahertz (THz) range by…

Optics · Physics 2020-06-29 Boyuan Jin , Tianjing Guo , Liang Zhu , Pai-Yen Chen , Christos Argyropoulos

Frequency conversion processes, such as second- and third-harmonic generation, are one of the most common effects in nonlinear optics which offer many opportunities for photonics, chemistry, material science, characterization, and…

Optics · Physics 2017-06-26 Alexander Krasnok , Mykhailo Tymchenko , Andrea Alu

We discuss the mechanism of coherent phonon generation by Stimulated Ionic Raman Scattering, a process different from conventional excitation with near visible optical pulses. Ionic Raman scattering is driven by anharmonic coupling between…

Superconductivity · Physics 2015-05-25 R. Mankowsky , M. Först , T. Loew , J. Porras , B. Keimer , A. Cavalleri

At levels of laser intensity below threshold for multiphoton ionization, the parametric generation of optical harmonics in gases and other isotropic media is subject to selection rules with origins in angular momentum conservation. The…

Optics · Physics 2019-06-13 David L. Andrews , Henryk Haniewicz , Enrique J. Galvez

We report observation of strong and anisotropic third harmonic generation (THG) in monolayer and multilayer ReS$_2$. The third-order nonlinear optical susceptibility of monolayer ReS$_2$, $\left| \chi^{(3)} \right|$ is on the order of…

Materials Science · Physics 2017-04-12 Qiannan Cui , Rodrigo A. Muniz , J. E. Sipe , Hui Zhao

Recent techniques have allowed transition metal dichalcogenides (TMD) monolayers to be grown and adequately characterised. Of particular interest, their nonlinear optical response presents many promising opportunities for future…

Mesoscale and Nanoscale Physics · Physics 2020-03-06 David N. Carvalho , Fabio Biancalana

Zinc Oxide is a thoroughly studied wide-bandgap semiconductor possessing excellent optical and electronic properties at room temperature. The renewed interest in this material has been generated by doping with various impurities in order to…

Materials Science · Physics 2023-04-25 Calford Otieno

Organic cavity polaritons are bosonic quasi-particles that arise from the strong interaction between organic molecular excitons and photons within microcavities. The spectral dispersion of third harmonic generation near resonance with the…

Optics · Physics 2018-10-08 Bin Liu , Michael Crescimanno , Robert J. Twieg , Kenneth D. Singer

Efficient third-order nonlinearities of the Zinc Oxide and Al-doped Zinc Oxide were studied by Third Harmonic Generation (Third Harmonic Generation) Maker fringes to establish the effect Aluminum of Aluminum doping(Al-doping) on the cubic…

Materials Science · Physics 2023-05-01 Calford Otieno

Plasmonic nanoantennas have been recently proposed to boost nonlinear optical processes. In a metal dipole nanoantenna with a dielectric nanoparticle placed in the gap, the linear field enhancement can be exploited to enhance third harmonic…

Optics · Physics 2017-04-13 Antonino Calà Lesina , Pierre Berini , Lora Ramunno