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The interaction of organic molecules and molecular aggregates with electromagnetic fields that are strongly confined inside optical cavities within nanoscale volumes, has allowed the observation of exotic quantum regimes of light-matter…

Quantum Physics · Physics 2018-01-30 Felipe Herrera , Frank C. Spano

Realizing nonlinear coupling across space can enable new scientific and technological advances, including ultrafast operation and propagation of information in IR photonic circuitry, remote triggering or catalyzing of chemical reactions,…

Optics · Physics 2019-12-13 Jiaxi Wang , Bo Xiang , Wei Xiong

We propose a robust and efficient way of controlling the optical spectra of two-dimensional materials and van der Waals heterostructures by quantum cavity embedding. The cavity light-matter coupling leads to the formation of…

Mesoscale and Nanoscale Physics · Physics 2019-06-19 Simone Latini , Enrico Ronca , Umberto de Giovannini , Hannes Hübener , Angel Rubio

Controlling light-matter based quantum systems in the strong coupling regime allows for exploring quantum simulation of many-body physics in nowadays architectures. For instance, the atom-field interaction in a cavity QED network provides…

Quantum Physics · Physics 2021-05-26 Diego Tancara , Ariel Norambuena , Rubén Peña , Guillermo Romero , Felipe Torres , Raúl Coto

Advances in nanophotonics, quantum optics, and low-dimensional materials have enabled precise control of light-matter interactions down to the nanoscale. Combining concepts from each of these fields, there is now an opportunity to create…

Chemical Physics · Physics 2019-07-11 Johannes Flick , Prineha Narang

Two-dimensional semiconductors inside optical microcavities have emerged as a versatile platform to explore new hybrid light-matter quantum states. The strong light-matter coupling leads to the formation of exciton-polaritons, which in turn…

Mesoscale and Nanoscale Physics · Physics 2021-11-05 Miguel Angel Bastarrachea-Magnani , Jannie Thomsen , Arturo Camacho-Guardian , Georg M. Bruun

Collective strong coupling between a disordered ensemble of $N$ localized molecular vibrations and a resonant optical cavity mode gives rise to 2 polariton and $N-1\gg2$ dark modes. Thus, experimental changes in thermally-activated reaction…

Quantum Physics · Physics 2022-03-14 Matthew Du , Joel Yuen-Zhou

Nonperturbative coupling between cavity photons and excitons leads to formation of hybrid light-matter excitations termed polaritons. In structures where photon absorption leads to creation of excitons with aligned permanent dipoles, the…

Mesoscale and Nanoscale Physics · Physics 2018-11-30 Emre Togan , Hyang-Tag Lim , Stefan Faelt , Werner Wegscheider , Atac Imamoglu

We study a system of interacting matter quasiparticles strongly coupled to photons inside an optomechanical cavity. The resulting normal modes of the system are represented by hybrid polaritonic quasiparticles, which acquire effective…

Quantum Gases · Physics 2017-02-27 N. Bobrovska , M. Matuszewski , T. C. H. Liew , O. Kyriienko

The effects of long-range intermolecular interactions on characteristic features of soliton bound states, consisting of localized excitons and polaritons in molecular crystals interacting with a high-intensity optical field, are…

Optics · Physics 2019-12-17 E. Nji Nde Aboringong , Alain M. Dikandé

The development of reliable ab initio methods for light-matter strong coupling is necessary for a deeper understanding of molecular polaritons. The recently developed strong coupling quantum electrodynamics Hartree-Fock model (SC-QED-HF)…

Chemical Physics · Physics 2025-02-21 Matteo Castagnola , Rosario R. Riso , Yassir El Moutaoukal , Enrico Ronca , Henrik Koch

Strong coupling of molecules to vacuum fields has been widely reported to lead to modified chemical properties such as reaction rates. However, some recent attempts to reproduce infrared strong coupling results have not been successful,…

Mesoscale and Nanoscale Physics · Physics 2024-01-03 Philip A. Thomas , Wai Jue Tan , Vasyl G. Kravets , Alexander N. Grigorenko , William L. Barnes

Controlling quantum materials with light is of fundamental and technological importance. By utilizing the strong coupling of light and matter in optical cavities (1-3), recent studies were able to modify some of their most defining features…

A quantum system composed of a molecule and an atomic ensemble, confined in a microscopic cavity, is investigated theoretically. The indirect coupling between atoms and the molecule, realized by their interaction with the cavity radiation…

Chemical Physics · Physics 2020-05-05 Tamás Szidarovszky , Gábor J. Halász , Ágnes Vibók

Cavity quantum electrodynamics advances the coherent control of a single quantum emitter with a quantized radiation field mode, typically piecewise engineered for the highest finesse and confinement in the cavity field. This enables the…

When atoms come together and bond, we call these new states molecules, and their properties determine many aspects of our daily life. Strangely enough, it is conceivable for light and molecules to bond, creating new hybrid light-matter…

Materials Science · Physics 2018-02-19 Branko Kolaric , Bjorn Maes , Koen Clays , Thomas Durt , Yves Caudano

The interaction between light and matter can give rise to novel topological states. This principle was recently exemplified in Floquet topological insulators, where \emph{classical} light was used to induce a topological electronic band…

Quantum Gases · Physics 2015-07-08 Torsten Karzig , Charles-Edouard Bardyn , Netanel Lindner , Gil Refael

The emergence of spatial and temporal coherence of light emitted from solid-state systems is a fundamental phenomenon, rooting in a plethora of microscopic processes. It is intrinsically aligned with the control of light-matter coupling,…

Over the past decade, exciton-polaritons in semiconductor microcavities have attracted a great deal of interest as a driven-dissipative quantum fluid. These systems offer themselves as a versatile platform for performing Hamiltonian…

We introduce a theory of chemical equilibrium in optical microcavities, which allows us to relate equilibrium reaction quotients in different electromagnetic environments. Our theory shows that in planar microcavities under strong coupling…

Chemical Physics · Physics 2023-05-02 Kaihong Sun , Raphael F. Ribeiro