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Recently, Tao and Mo (TM) derived a meta-generalized gradient approximation functional based on a model exchange-correlation hole. In this work, the performance of this functional is assessed on standard test sets, using the…

Chemical Physics · Physics 2017-01-04 Yuxiang Mo , Guocai Tian , Roberto Car , Viktor N. Staroverov , Gustavo E. Scuseria , Jianmin Tao

The Normalized Transformer, or nGPT (arXiv:2410.01131) achieves impressive training speedups and does not require weight decay or learning rate warmup. However, despite having hyperparameters that explicitly scale with model size, we…

Machine Learning · Computer Science 2026-05-04 Boris Shigida , Boris Hanin , Andrey Gromov

The accuracy of applying density functional theory to noncovalent interactions is hindered by errors arising from low-density regions of interaction-induced change in the density gradient, error compensation between correlation and exchange…

Chemical Physics · Physics 2014-10-22 Marcin Modrzejewski , Grzegorz Chałasiński , Małgorzata M. Szczęśniak

The $\text{Cu}_7\text{P}\text{S}_6$ compound has garnered significant attention due to its potential in thermoelectric applications. In this study, we introduce a neuroevolution potential (NEP), trained on a dataset generated from ab initio…

Materials Science · Physics 2024-11-19 Junlan Liu , Qian Yin , Mengshu He , Jun Zhou

The newly developed machine learning (ML) empirical pseudopotential (EP) method overcomes the poor transferability of the traditional EP method with the help of ML techniques while preserving its formal simplicity and computational…

Materials Science · Physics 2025-11-20 Sungmo Kang , Rokyeon Kim , Seungwu Han , Young-Woo Son

We formulate a spin-polarized van Leeuwen and Baerends (vLB) correction to the local density approximation (LDA) exchange potential [Phys. Rev. A 49, 2421 (1994)] that enforces the ionization potential (IP) theorem following Stein et al.…

Materials Science · Physics 2016-03-09 Prashant Singh , Manoj K. Harbola , M. Hemanadhan , Abhijit Mookerjee , D. D. Johnson

We propose a short- and long-range corrected (SLC) hybrid scheme employing 100% Hartree-Fock (HF) exchange at both zero and infinite interelectronic distances, wherein three SLC hybrid density functionals with the D3 dispersion corrections…

Chemical Physics · Physics 2016-11-23 Chih-Wei Wang , Kerwin Hui , Jeng-Da Chai

Experimental studies of the oxygen reduction reaction (ORR) at nitrogen doped graphene electrodes have reported a remarkably low overpotential, on the order of 0.5 V, similar to Pt based electrodes. Theoretical calculations using density…

Pseudopotential locality errors have hampered the applications of the diffusion Monte Carlo (DMC) method in materials containing transition metals, in particular oxides. We have developed locality error free effective core potentials,…

Machine learned potentials (MLPs) have been widely employed in molecular dynamics (MD) simulations to study thermal transport. However, literature results indicate that MLPs generally underestimate the lattice thermal conductivity (LTC) of…

Materials Science · Physics 2024-09-12 Xiguang Wu , Wenjiang Zhou , Haikuang Dong , Penghua Ying , Yanzhou Wang , Bai Song , Zheyong Fan , Shiyun Xiong

Ultrafast laser experiments yield increasingly reliable data on warm dense matter, but their interpretation requires theoretical models. We employ an efficient density functional neutral-pseudoatom hypernetted-chain (NPA-HNC) model with…

Materials Science · Physics 2016-12-02 Louis Harbour , M. W. Chandre Dharma-wardana , Dennis D. Klug , Laurent J. Lewis

Realistic prediction of the superconducting transition temperature (Tc) for PdH is a long-standing challenge, because it depends on robust calculations of the electron and phonon band structures to obtain the electron-phonon scattering…

Materials Science · Physics 2022-08-08 Samaneh Sadat Setayandeh , Tim Gould , Toktam Morshedloo , Evan Gray

Context. The study of pre-stellar cores (PSCs) suffers from a lack of undepleted species to trace the gas physical properties in their very dense inner parts. Aims. We want to carry out detailed modelling of N2H+ and N2D+ cuts across the…

Astrophysics · Physics 2009-11-13 Laurent Pagani , Aurore Bacmann , Sylvie Cabrit , Charlotte Vastel

We have calculated the ground state electronic structure of He under pressure from 0 to 1500 GPa using both all-electron full-potential and pseudopotential methods based on the density functional theory (DFT). We find that throughout this…

Materials Science · Physics 2012-01-10 W. Xiao , Z. X. Tian , W. T. Geng

Artificial neural network potentials (NNPs) have emerged as effective tools for understanding atomic interactions at the atomic scale in various phenomena. Recently, we developed highly transferable NNPs for {\alpha}-iron and…

Materials Science · Physics 2023-12-01 Shihao Zhang , Fanshun Meng , Rong Fu , Shigenobu Ogata

New interatomic potentials describing defects, plasticity and high temperature phase transitions for Ti are presented. Fitting the martensitic hcp-bcc phase transformation temperature requires an efficient and accurate method to determine…

Materials Science · Physics 2016-12-12 M. I. Mendelev , T. L. Underwood , G. J. Ackland

First-principles calculations rely heavily on pseudopotentials, yet their impact on accuracy is hardly addressed. In this work, we show that most pseudopotentials to date introduce errors, which manifest themselves as errors of atomic…

Materials Science · Physics 2025-11-19 Kuiyu Ye , Jiale Shen , Haitao Liu , Yuanchang Li , S. B. Zhang

We present a systematic study that clarifies validity and limitation of current hybrid functionals in density functional theory for structural and electronic properties of various semiconductors and insulators. The three hybrid functionals,…

Materials Science · Physics 2015-03-19 Yu-ichiro Matsushita , Kazuma Nakamura , Atsushi Oshiyama

We discuss low-energy and collider constraints on the effective couplings characterizing non-standard charged current interactions. A direct comparison of low-energy and LHC probes can be performed within an effective theory framework, when…

High Energy Physics - Phenomenology · Physics 2015-06-11 Vincenzo Cirigliano , Martín González-Alonso , Michael L. Graesser

The Heyd-Scuseria-Ernzerhof (HSE) hybrid functional has become a widely used tool for theoretical calculations of point defects in semiconductors. It generally offers a satisfactory qualitative description of defect properties, including…