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Most of the searches for Kitaev materials deal with $4d/5d$ magnets with spin-orbit-coupled ${J=1/2}$ local moments such as iridates and $\alpha$-RuCl$_3$. Here we propose the monoclinic YbCl$_3$ with a Yb$^{3+}$ honeycomb lattice for the…

Strongly Correlated Electrons · Physics 2020-07-22 Jie Xing , Erxi Feng , Yaohua Liu , Eve Emmanouilidou , Chaowei Hu , Jinyu Liu , David Graf , Arthur P. Ramirez , Gang Chen , Huibo Cao , Ni Ni

We present comprehensive electron spin resonance (ESR) studies of in-plane oriented single crystals of $\alpha$-RuCl$_3$, a quasi-two-dimensional material with honeycomb structure, focusing on its high-field spin dynamics. The measurements…

The delafossite structure of NaYbS2 contains a planar spin-1/2 triangular lattice of Yb3+ ions and features a possible realisation of a quantum spin-liquid state. We investigated the Yb3+ spin dynamics by Electron Spin Resonance (ESR) in…

Strongly Correlated Electrons · Physics 2019-03-11 Jörg Sichelschmidt , Philipp Schlender , Burkhard Schmidt , Michael Baenitz , Thomas Doert

We report magnetic and thermodynamic properties of single crystal $\alpha$-RuCl$_3$, in which the Ru$^{3+}$ ($4d^5$) ion is in its low spin state and forms a honeycomb lattice. Two features are observed in both magnetic susceptibility and…

Strongly Correlated Electrons · Physics 2015-04-27 J. A. Sears , M. Songvilay , K. W. Plumb , J. P. Clancy , Y. Qiu , Y. Zhao , D. Parshall , Young-June Kim

We report a muon spin rotation/relaxation ($\mu$SR) study of single-crystalline samples of the $\alpha$-RuCl$_3$ honeycomb magnet, which is presumed to be a model compound for the Kitaev-Heisenberg interaction. It is inferred from magnetic…

Lattice and spin excitations have been studied by Raman scattering in hexagonal YbMnO3 single crystals. The temperature dependences of the phonon modes show that the E2 mode at 256 cm-1 related to the displacement of Mn and O ions in a-b…

Strongly Correlated Electrons · Physics 2012-11-12 J. Liu , C. Toulouse , P. Rovillain , M. Cazayous , Y. Gallais , M. -A. Measson , S. W. Cheong , N. Lee , A. Sacuto

We have measured the spin susceptibility of the underdoped high temperature superconductor, YBa2Cu4O8 by Gd^{3+} electron spin resonance in single crystals and aligned powders at several magnetic fields between 3 and 15.4 T. At low…

We present high-field electron spin resonance (ESR) studies of the honeycomb-lattice material $\alpha$-RuCl$_3$, a prime candidate to exhibit Kitaev physics. Two modes of antiferromagnetic resonance were detected in the zigzag ordered…

We present detailed ESR investigations on single crystals of the low-dimensional quantum magnet TiOCl. The anisotropy of the g-factor indicates a stable orbital configuration below room temperature, and allows to estimate the energy of the…

A series of electron spin resonance (ESR) experiments were performed on a single crystal of the heavy fermion metal YbIr2Si2 to map out the anisotropy of the ESR-intensity I_ESR which is governed by the microwave field component of the…

Strongly Correlated Electrons · Physics 2010-03-29 T. Gruner , J. Wykhoff , J. Sichelschmidt , C. Krellner , C. Geibel , F. Steglich

Using quantum chemistry calculations we shed fresh light on the electronic structure and magnetic properties of RuCl3, a proposed realization of the honeycomb Kitaev spin model. It is found that the nearest-neighbor Kitaev exchange K is…

Strongly Correlated Electrons · Physics 2017-01-19 Ravi Yadav , Nikolay A. Bogdanov , Vamshi M. Katukuri , Satoshi Nishimoto , Jeroen van den Brink , Liviu Hozoi

We study the correlated quantum magnet, YbCl$_3$, with neutron scattering, magnetic susceptibility, and heat capacity measurements. The crystal field Hamiltonian is determined through simultaneous refinements of the inelastic neutron…

Hexagonal alpha-Ru trichloride single crystals exhibit a strong magnetic anisotropy and we show that upon applying fields up to 14 T in the honeycomb plane the successive magnetic order at T1 = 14 K and T2 = 8 K could be completely…

Strongly Correlated Electrons · Physics 2015-06-02 M. Majumder , M. Schmidt , H. Rosner , A. A. Tsirlin , H. Yasuoka , M. Baenitz

A theory of spin relaxation in graphene including intrinsic, Bychkov-Rashba, and ripple spin-orbit coupling is presented. We find from spin relaxation data by Tombros et al. [Nature 448, 571 (2007).] that intrinsic spin-orbit coupling…

Strongly Correlated Electrons · Physics 2015-03-13 F. Simon , F. Muranyi , B. Dora

Fine details of the excitation spectrum of the two-dimensional spin-gap magnet PHCC are revealed by electron spin resonance investigations. The values of anisotropy parameters and the orientations of the anisotropy axes are determined by…

Strongly Correlated Electrons · Physics 2012-02-23 V. N. Glazkov , T. S. Yankova , J. Sichelschmidt , D. Hüvonen , A. Zheludev

YbOCl is a representative member of the van der Waals layered honeycomb rare-earth chalcohalide REChX (RE = rare earth, Ch = O, S, Se, and Te, and X = F, Cl, Br, and I) family reported recently. Its spin ground state remains to be explored…

Strongly Correlated Electrons · Physics 2024-09-13 Zheng Zhang , Yanzhen Cai , Jinlong Jiao , Jing Kang , Dehong Yu , Bertrand Roessli , Anmin Zhang , Jianting Ji , Feng Jin , Jie Ma , Qingming Zhang

Here, we study YbI$_3$, a quasi-2D layered material with Yb atoms arranged on an ideal honeycomb network of edge-sharing YbI$_6$ octahedra, analogous to the low-temperature phase of $\alpha-$RuCl$_3$. High quality single crystals of YbI$_3$…

We report on the experimental results of magnetic susceptibility, specific heat, electron spin resonance (ESR), and high-field magnetization measurements on a polycrystalline sample of the spin-$1/2$ distorted honeycomb-lattice…

We report a comprehensive high-field/high-frequency electron spin resonance (ESR) study on single crystals of the van der Waals magnet CrCl$_3$. This material, although being known for quite a while, has received recent significant…

Materials Science · Physics 2020-06-09 J. Zeisner , K. Mehlawat , A. Alfonsov , M. Roslova , T. Doert , A. Isaeva , B. Büchner , V. Kataev

The interplay between spin-orbit coupling, anisotropic magnetic interaction, frustration-induced quantum fluctuations and spin correlations can lead to novel quantum states with exotic excitations in rare-earth-based quantum magnets.…

Strongly Correlated Electrons · Physics 2023-08-31 J. Khatua , Q. P. Ding , M. S. Ramachandra Rao , K. Y. Choi , A. Zorko , Y. Furukawa , P. Khuntia
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