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We explore the magnetic properties of isolated a-b planes of trinuclear organometallic crystals, Mo3S7(dmit)3, in which an interplay of strong electronic correlations and spin molecular-orbital coupling (SMOC) occurs. The magnetic…

Strongly Correlated Electrons · Physics 2018-11-01 J. Merino , A. C. Jacko , A. L. Khosla , A. Ralko , B. J. Powell

For the first time, magnetization of high-Tc samples with different crystalline structure and its isothermal relaxation is studied at very weak constant fields (H <= 0.1 Oe) for temperatures close to the critical ones. Essential influence…

Superconductivity · Physics 2009-11-11 V. P. Timofeev , A. N. Omelyanchouk

Muon spin rotation measurements have been performed on a powder sample of a-RuCl3, a layered material which previously has been proposed to be a quantum magnet on a honeycomb lattice close to a quantum spin liquid ground state. Our data…

Strongly Correlated Electrons · Physics 2016-07-20 F. Lang , P. J. Baker , A. A. Haghighirad , Y. Li , D. Prabhakaran , R. Valenti , S. J. Blundell

The electron paramagnetic resonance investigations of the magnetically concentrated crystal of KYb(MoO4)2 have been performed. The main value of g-factors along principal local axes was determinate. The two nonequivalent Yb3+ centers were…

Materials Science · Physics 2007-05-23 K. G. Dergachev , M. I. Kobets , E. N. Khatsko

Single crystals of the Kitaev spin-liquid candidate $\alpha$-RuCl$_3$ have been studied to determine low-temperature bulk properties, structure and the magnetic ground state. Refinements of x-ray diffraction data show that the low…

Strongly Correlated Electrons · Physics 2016-04-27 H. B. Cao , A. Banerjee , J. -Q. Yan , C. A. Bridges , M. D. Lumsden , D. G. Mandrus , D. A. Tennant , B. C. Chakoumakos , S. E. Nagler

Magnetic properties of high-quality Al-free nonsuperconducting GdBa_2Cu_3O_{6+y} single crystals grown by flux method have been studied. The magnetic anisotropy below the N\'eel temperature T_N~2.3K corresponds to the direction of Gd^{3+}…

Materials Science · Physics 2016-08-31 V. N. Narozhnyi , D. Eckert , G. Fuchs , V. Nekvasil , K. -H. Müller

We report results of magnetization, specific-heat and muon-spin relaxation measurements on single crystals of disorder-free Yb$^{3+}$ triangular lattice Yb(BaBO$_3$)$_3$. The magnetization experiments show anisotropic magnetic properties…

Strongly Correlated Electrons · Physics 2022-07-27 C. Y. Jiang , Y. X. Yang , Y. X. Gao , Z. T. Wan , Z. H. Zhu , T. Shiroka , C. S. Chen , Q. Wu , X. Li , J. C. Jiao , K. W. Chen , Y. Bao , Z. M. Tian , L. Shu

Quantum magnets based on honeycomb lattices with low-coordination number offer a viable ground to realize exotic emergent quantum excitations and phenomena arising from the interplay between competing magnetic interactions, spin…

Strongly Correlated Electrons · Physics 2024-11-14 J. Khatua , M. Gomilsek , Kwang-Yong Choi , P. Khuntia

Magnetic properties of a mixed spin-1/2 and spin-1 Ising model on honeycomb lattice are exactly investigated within the framework of generalized star-triangle mapping transformation. The particular attention is focused on the effect of…

Statistical Mechanics · Physics 2009-11-10 Jozef Strecka , Michal Jascur

Single crystals of a honeycomb lattice antiferromagnet, Tb$_2$Ir$_3$Ga$_9$ were synthesized, and the physical properties have been studied. From magnetometry, a long-range antiferromagnetic ordering at $\approx$12.5 K with highly…

Mesoscale and Nanoscale Physics · Physics 2019-11-27 Mojammel A. Khan , Qiang Zhang , Jin-Ke Bao , Randy S. Fishman , Antia S. Botana , Y. Choi , G. Fabbris , D. Haskel , John Singleton , John F. Mitchell

Mott insulators with strong spin-orbit coupling have been proposed to host unconventional magnetic states, including the Kitaev quantum spin liquid. The 4$d$ system $\alpha$-RuCl$_3$ has recently come into view as a candidate Kitaev system,…

The crystal growth and the structural, transport and magnetic properties of the magnetically frustrated YbMn$_2$Sb$_2$ single crystals are reported. The crystals show a trigonal symmetry (space group $P\bar{3}m1$), where corrugated…

Atomic Physics · Physics 2020-04-27 J. Munevar , F. R. Arantes , L. Mendonça-Ferreira , M. A. Avila , R. A. Ribeiro

The layered honeycomb magnet alpha-RuCl3 has been proposed as a candidate to realize a Kitaev spin model with strongly frustrated, bond-dependent, anisotropic interactions between spin-orbit entangled jeff=1/2 Ru4+ magnetic moments. Here we…

Strongly Correlated Electrons · Physics 2015-12-16 R. D. Johnson , S. Williams , A. A. Haghighirad , J. Singleton , V. Zapf , P. Manuel , I. I. Mazin , Y. Li , H. O. Jeschke , R. Valenti , R. Coldea

Single crystal neutron diffraction, inelastic neutron scattering, bulk magnetization measurements, and first-principles calculations are used to investigate the magnetic properties of the honeycomb lattice $\rm Tb_2Ir_3Ga_9$. While the…

Kitaev materials often order magnetically at low temperatures due to the presence of non-Kitaev interactions. Torque magnetometry is a very sensitive technique for probing the magnetic anisotropy, which is critical in understanding the…

Strongly Correlated Electrons · Physics 2024-12-17 John S. Pearce , David A. S. Kaib , Zeyu Ma , Danrui Ni , R. J. Cava , Roser Valenti , Radu Coldea , Amalia I. Coldea

We report inelastic neutron scattering measurements on Na2IrO3, a candidate for the Kitaev spin model on the honeycomb lattice. We observe spin-wave excitations below 5 meV with a dispersion that can be accounted for by including…

The honeycomb compound $\alpha$-RuCl$_3$ is widely discussed as a proximate Kitaev spin-liquid material. This scenario builds on spin-orbit entangled $j = 1/2$ moments arising for a $t_{2g}^5$ electron configuration with strong spin-orbit…

Strongly Correlated Electrons · Physics 2020-10-21 P. Warzanowski , N. Borgwardt , K. Hopfer , T. C. Koethe , P. Becker , V. Tsurkan , A Loidl , M. Hermanns , P. H. M. van Loosdrecht , M. Grüninger

The layered compound $\alpha$-RuCl$_3$ is composed of a honeycomb lattice of magnetic Ru$^{3+}$ ions with the $4d^5$ electronic state. We have investigated the magnetic properties of $\alpha$-RuCl$_3$ via magnetization and specific heat…

Strongly Correlated Electrons · Physics 2015-06-24 Yumi Kubota , Hidekazu Tanaka , Toshio Ono , Yasuo Narumi , Koichi Kindo

We report magnetization and neutron diffraction studies on crystal and magnetic structures of Ir- and Rh-substituted honeycomb lattice $\alpha$-RuCl$_3$. The iridium or rhodium atoms are distributed at the Ru site with little structural…

Materials Science · Physics 2023-10-05 Zachary Morgan , Iris Ye , Colin L. Sarkis , Xiaoping Wang , Stephen Nagler , Jiaqiang Yan

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…