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Large area epitaxy of two-dimensional (2D) layered materials with high material quality is a crucial step in realizing novel device applications based on 2D materials. In this work, we report high-quality, crystalline, large-area gallium…

Nanorods grow in two modes through physical vapor deposition (PVD). In mode I, monolayer surface steps dictate the diameter of nanorods. In mode II, multiple-layer surface steps dictate the diameter, which is the smallest possible under…

Materials Science · Physics 2018-05-09 Feng Du , Hanchen Huang

Assembling different two-dimensional (2D) crystals, covering a very broad range of properties, into van der Waals (vdW) heterostructures enables the unprecedented possibilities for combining the best of different ingredients in one…

Materials Science · Physics 2017-05-17 Jia-Bin Qiao , Yue Gong , Wei-Jie Zuo , Yi-Cong Wei , Dong-Lin Ma , Hong Yang , Ning Yang , Kai-Yao Qiao , Jin-An Shi , Lin Gu , Lin He

Two-dimensional (2D) semiconducting transition-metal dichalcogenides (TMDCs) are an exciting platform for new excitonic physics and next-generation electronics, creating a strong demand to understand their growth, doping, and…

Shaping low-dimensional crystals into precise geometries with low disorder is an outstanding challenge. Here, we present a method to grow single crystals of arbitrary geometry within van der Waals (vdW) materials. By injecting molten…

Two-dimensional (2D) transition metal dichalcogenides (TMDs), especially MoS2 and WS2 recently attract extensive attentions due to their rich physics and great potential applications. Superior to graphene, MS2 (M = Mo/W) monolayers have a…

Materials Science · Physics 2013-12-06 Chunxiao Cong , Jingzhi Shang , Xing Wu , Bingchen Cao , Namphung Peimyoo , Caiyu Qiu , Litao Sun , Ting Yu

Hexagonal Si2Te2 monolayers (ML-Si2Te2) were predicted to show strain-dependent band-crossover between semiconducting and room-temperature quantum spin Hall phases. However, investigations on this artificial two-dimensional (2D) material…

The ability of different materials to display self-limiting growth has recently attracted enormous attention due to the importance of nanoscale materials in applications for catalysis, energy conversion, (opto)electronics, etc. Here, we…

Monolayer MoTe2 exhibits a variety of derivative structural phases and associated novel electronic properties that enable a wealth of potential applications in future electronic and optoelectronic devices. However, a comprehensive study…

Materials Science · Physics 2024-07-22 Zemin Pan , Tao Jian , Hui Zhang , Xiaoyu Lin , Chao Zhu , Jinghao Deng , Zhengbo Cheng , Chuansheng Liu , Chendong Zhang

We have combined the benefits of two catalytic growth phenomena to form nanostructures of transition metal trichalcogenides (TMTs), materials that are challenging to grow in a nanostructured form by conventional techniques, as required to…

Controlling the interconnection of neighboring seeds (nanoflakes) to full coverage of the textured substrate is the main challenge for the large-scale conformal growth of atomic-thick transition metal dichalcogenides by chemical vapor…

Layered van der Waals (vdW) materials grown by physical vapor deposition techniques are generally assumed to have a weak interaction with the substrate during growth. This leads to films with relatively small domains that are usually…

Materials Science · Physics 2021-03-25 Theresa P. Ginley , Stephanie Law

Palladium diselenide (PdSe$_2$), a new type of two-dimensional noble metal dihalides (NMDCs), has received widespread attention for its excellent electrical and optoelectronic properties. Herein, high-quality continuous centimeter-scale…

Materials Science · Physics 2021-09-07 MingYang Wei , Jie Lian , Yu Zhang , ChenLin Wang , Yueming Wang , Zhen Xu

Near-field optical microscopy can be used as a viable route to understand the nanoscale material properties below the diffraction limit. On the other hand, atomically thin two-dimensional (2D) transition metal dichalcogenides (TMDs) are the…

The growth of crystals confined in porous or cellular materials is ubiquitous in Nature and industry. Confinement affects the formation of biominerals in living organisms, of minerals in the Earth's crust and of salt crystals damaging…

Materials Science · Physics 2022-11-30 Felix Kohler , Olivier Pierre-Louis , Dag Kristian Dysthe

Monolayers of transition metal dichalcogenides (TMDCs) are atomically thin direct-gap semiconductors with potential applications in nanoelectronics, optoelectronics, and electrochemical sensing. Recent theoretical and experimental efforts…

Mesoscale and Nanoscale Physics · Physics 2013-02-26 Sanfeng Wu , Chunming Huang , Grant Aivazian , Jason S Ross , David H Cobden , Xiaodong Xu

Applying time-dependent photoemission we unravel the graphene growth process on a metallic surface by chemical vapor deposition (CVD). Graphene CVD growth is in stark contrast to the standard growth process of two--dimensional films because…

Materials Science · Physics 2015-05-13 Alexander Grüneis , Kurt Kummer , Denis V. Vyalikh

Layered metal dichalcogenide materials are a family of semiconductors with a wide range of energy band gaps and properties, and potential to open up new areas of physics and technology applications. However, obtaining high crystal quality…

The growth of single-layer MoS2 with chemical vapor deposition is an established method that can produce large-area and high quality samples. In this article, we investigate the geometrical and optical properties of hundreds of individual…

Mesoscale and Nanoscale Physics · Physics 2017-04-07 Foad Ghasemi , Riccardo Frisenda , Dumitru Dumcenco , Andras Kis , David Perez de Lara , Andres Castellanos-Gomez

Real-time monitoring is essential for understanding and eventually precise controlling of the growth of two dimensional transition-metal dichalcogenides (2D TMDCs). However, it is very challenging to carry out such kind of studies on…

Materials Science · Physics 2018-11-02 C. B. López-Posadas , Yaxu Wei , Wanfu Shen , Daniel Kahr , Michael Hohage , Lidong Sun