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We study the response of materials with nanoscale pores containing sodium chloride solutions, to cycles of relative humidity (RH). Compared to pure fluids, we show that these sorption isotherms display much wider hysteresis, with a shape…

Soft Condensed Matter · Physics 2025-11-03 Hugo Bellezza , Marine Poizat , Olivier Vincent

The calculation of the solvation properties of a single water molecule in liquid water is carried out in two ways. In the first, the water molecule is placed in a cavity and the solvent is treated as a dielectric continuum. This model is…

chem-ph · Physics 2008-02-03 Steven W. Rick , B. J. Berne

Evaporation from a porous medium partially saturated with saline water, causes the salinity (salt concentration) to increase near the top of the porous medium as water leaves while salt stays behind. As the density of the water increases…

Fluid Dynamics · Physics 2025-01-23 C. Bringedal , S. Kiemle , C. J. van Duijn , R. Helmig

Short-range correlations in electrolyte solutions lead to oscillatory profiles of water polarization and ionic concentration at electrode-electrolyte interfaces. The recently developed density-potential-polarization functional theory…

Chemical Physics · Physics 2026-03-23 Mengke Zhang , Jun Huang

Treating water as a linearly responding dielectric continuum on molecular length scales allows very simple estimates of solvation structure and thermodynamics for charged and polar solutes. While this approach can successfully account for…

Statistical Mechanics · Physics 2021-07-07 Stephen J. Cox , Kranthi K. Mandadapu , Phillip L. Geissler

Supercapacitors have been attracting significant attention as promising energy storage devices. However, the voltage window limitation associated with electrolyte solutions has hindered the improvement of their capacitance. To address this…

Chemical Physics · Physics 2023-06-27 Weihang Gao , Teng Zhao , Shian Dong , Xingyi Huang , Zhenli Xu

Solvation effect might have a tremendous influence on chemical reactions. However, precise quantum chemistry calculations are most often done either in vacuum neglecting the role of the solvent or using continuum solvent model ignoring its…

Chemical Physics · Physics 2020-07-14 Guillaume Jeanmairet , Maximilien Levesque , Daniel Borgis

It is well-known that the swelling behavior of ionic nanogels depends on their cross-link density, however it is unclear how different topologies should affect the response of the polyelectrolyte network. Here we perform Monte Carlo…

Soft Condensed Matter · Physics 2016-03-23 Leandro G. Rizzi , Yan Levin

We present results of molecular dynamics simulations of strong, flexible polyelectrolyte chains in solution with added salt. The effect of added salt on the polyelectrolyte chain structure is fully treated for the first time as a function…

Soft Condensed Matter · Physics 2008-02-03 Mark J. Stevens , Steve Plimpton

We consider an electrolyte solution confined by semipermeable membranes in contact with a salt-free solvent. Membranes are uncharged, but since small counter-ions leak-out into infinite salt-free reservoirs, we observe a distance-dependent…

Soft Condensed Matter · Physics 2014-08-19 Salim R. Maduar , Olga I. Vinogradova

The recently discovered ferroelectric nematic liquid crystals have been reported to exhibit very large dielectric permittivity values. Here, we report a systematic investigation of the dielectric behavior of a prototypical ferroelectric…

Soft Condensed Matter · Physics 2024-02-05 Aitor Erkoreka , Josu Martinez-Perdiguero , Richard J. Mandle , Alenka Mertelj , Nerea Sebastián

Recent experiments show that the relative dielectric constant $\epsilon$ of water confined to a film of nanometric thickness reaches a strikingly low value of 2.1, barely above the bulk's 1.8 value for the purely electronic response. We…

Mesoscale and Nanoscale Physics · Physics 2025-10-13 Jon Zubeltzu , Fernando Bresme , Matthew Dawber , Marivi Fernandez-Serra , Emilio Artacho

The response of a suspension under a variety of static or alternating external fields strongly depends on the equilibrium electric double layer that surrounds the colloidal particles in the suspension. The theoretical models for salt-free…

Soft Condensed Matter · Physics 2022-02-11 Jun-Sik Sin , Kwang-Il Kim , Kuk-Chol Ri , Dok-Yong Ju , Nam-Hyok Kim , Chung-Sik Sin

In this work we give the analysis of the low frequency dielectric response of selected kaolinitic clays at different water content ranging from dry, over plastic to liquid limit. For all samples investigated, depending on the moisture…

Soft Condensed Matter · Physics 2016-08-31 Dean Korosak , Janja Kramer , Renata Jecl , Bruno Cvikl , Miran Veselic

The dissolution of NaCl in water is one of the most common everyday processes, yet it remains poorly understood at the molecular level. Here we report the results of an extensive density functional theory study in which the initial stages…

Chemical Physics · Physics 2013-12-18 Jiří Klimeš , David R. Bowler , Angelos Michaelides

Wetting of a charged substrate by an electrolyte solution is investigated by means of classical density functional theory applied to a lattice model. Within the present model the pure, i.e., salt-free solvent, for which all interactions are…

Soft Condensed Matter · Physics 2013-06-06 Ingrid Ibagon , Markus Bier , S. Dietrich

Many theoretical studies were devoted in the past to ion-specific effects, trying to interpret a large body of experimental evidence, such as surface tension at air/water interfaces and force measurements between charged objects. Although…

Soft Condensed Matter · Physics 2014-04-22 Dan Ben-Yaakov , David Andelman , Rudi Podgornik

Poly(vinyl alcohol)/Poly(vinylidene fluoride) blends at mass ratio 3:1 with Nano - Graphene Platelet fillers constitute mechanically and thermally stable systems, which are used for developing piezoelectric devices. Blends host a fraction…

Chemical Physics · Physics 2025-05-07 Eirini Kolonelou , Anthony N. Papathanassiou

We study water between parallel metal walls under applied electric field accounting for the image effect at $T=298$ K. The electric field due to the surface charges serves to attract and orient nearby water molecules, while it tends to a…

Soft Condensed Matter · Physics 2015-07-24 Kyohei Takae , Akira Onuki

Dielectric permittivity of supercooled volume water has been measured in the range of temperatures from $-20\,^{\circ}$C to $-60\,^{\circ}$C at the frequencies $7.6$~GHz and $9.7$~GHz. The measurements have been made using microwave…

Soft Condensed Matter · Physics 2020-05-15 G. S. Bordonskiy , A. A. Gurulev , A. O. Orlov
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