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The density and orientational relaxation of bulk water can be separately studied by depolarized light scattering (DLS) and dielectric spectroscopy (DS), respectively. Here we ask the question of what are the leading collective modes…

Soft Condensed Matter · Physics 2014-02-26 Daniel R. Martin , Daniele Fioretto , Dmitry V. Matyushov

Most organic and inorganic surfaces (e.g., glass, nucleic acids or lipid membranes) become charged in aqueous solutions. The resulting ionic distribution induces effective interactions between the charged surfaces. Stacks of like-charged…

The magnitude of the relative permittivity of the ferroelectric nematic phase (NF) is under a lively scientific discussion since the phase was recently discovered. Dielectric spectroscopy measurements (DSM) give a huge value of relative…

Soft Condensed Matter · Physics 2024-09-05 Vojko Matko , Ewa Gorecka , Damian Pociecha , Joanna Matraszek , Nataša Vaupotič

Over the last decade, an increasing body of evidence has emerged, supporting the existence of a metastable liquid-liquid critical point in supercooled water, whereby two distinct liquid phases of different densities coexist. Analysing long…

Soft Condensed Matter · Physics 2024-08-20 Cesare Malosso , Natalia Manko , Maria Grazia Izzo , Stefano Baroni , Ali Hassanali

The present article experimentally and theoretically probes the evaporation kinetics of sessile saline droplets. Observations reveal that presence of solvated ions leads to modulated evaporation kinetics, which is further a function of…

Fluid Dynamics · Physics 2020-06-24 Abhishek Kaushal , Vivek Jaiswal , Vishwajeet Mehandia , Purbarun Dhar

The dielectric permittivity of liquid water is a fundamental property that underlies its distinctive behaviors in numerious physical, biological, and chemical processes. Within a machine learning framework, we present a unified approach to…

Soft Condensed Matter · Physics 2025-08-11 Kehan Cai , Chunyi Zhang , Xifan Wu

The electric field dielectric polarization-based separations mechanism represents a novel method for separating solutions at small length scales. An electric field gradient with a maximum strength of $\mathrm{0.4~MV/m}$ applied across a…

Chemical Physics · Physics 2023-11-29 Gaurav Anand , Samira Safaripour , Craig Snoeyink

The dielectric constant of ionic solutions is known to reduce with increasing ionic concentrations. However, the origin of this effect has not been thoroughly explored. In this paper we study two such possible sources: long-range Coulombic…

Statistical Mechanics · Physics 2022-08-04 Ram M. Adar , Tomer Markovich , Amir Levy , Henri Orland , David Andelman

We study the electric double layer near a charged soft surface by using a mean-field approach including non-uniform size effect and solvent polarization. Based on a free energy model, electrostatic potential and number densities of water…

Soft Condensed Matter · Physics 2022-02-10 Jun-Sik Sin , Nam-Hyok Kim , Chung-Sik Sin

Life on Earth depends upon the dissolution of ionic salts in water, particularly NaCl. However, an atomistic scale understanding of the process remains elusive. Simulations lend themselves conveniently to studying dissolution since they…

Chemical Physics · Physics 2022-11-09 Niamh O'Neill , Christoph Schran , Stephen J. Cox , Angelos Michaelides

We study the variation of the dielectric response of ionic aqueous solutions as function of their ionic strength. The effect of salt on the dielectric constant appears through the coupling between ions and dipolar water molecules. On a…

Soft Condensed Matter · Physics 2013-11-19 Amir Levy , David Andelman , Henri Orland

It is well known that the convection of liquid solution or melt liquid is inhibited by the magnetic field experimentally, and so that we can make the larger and better crystals at the cost of slow growth rate. We shall show here another two…

Other Condensed Matter · Physics 2007-05-23 Naohisa Ogawa , Shu-ichi Nagasawa

Landau Damping (LD) mechanism of the Localized Surface Plasmon (LSP) decay is studied for the hybrid nanoplasmonic (metal core/dielectric shell) structures. It is shown that LD in hybrid structures is strongly affected by permittivity and…

Humid hydrophobic ionic liquids, widely used as electrolytes, have narrowed electrochemical windows, because their water, absorbed on the electrode surface, gets involved in electrolysis. In this work, we performed molecular dynamics…

Applied Physics · Physics 2020-12-02 Ming Chen , Jiedu Wu , Ting Ye , Jinyu Ye , Sheng Bi , Jiawei Yan , Bingwei Mao , Guang Feng

Salt is a very common molecule in aqueous environments but the question of whether the interactions of monovalent ions Na^+ and Cl^- ,with the neutral heads of phospholipids are impactful enough to change the membrane rigidity is still a…

We study the salt-dependent conformations of dilute flexible polyelectrolytes in solution via computer simulations. Low concentrations of multivalent salt induce the known conformational collapse of individual polyelectrolyte chains, but as…

Soft Condensed Matter · Physics 2009-11-11 Pai-Yi Hsiao , Erik Luijten

The effects of ionic ordering in DNA water solutions are studied by conductivity experiments. The conductivity measurements are performed for the solutions of DNA with KCl salt in the temperature range from 28 to 70 C. Salt concentration…

Biomolecules · Quantitative Biology 2014-01-06 O. O. Liubysh , O. M. Alekseev , S. Yu. Tkachov , S. M. Perepelytsya

We re-examine the problem of the dielectric response of highly polar liquids such as water in confinement between two walls using a simple two-variable density functional theory involving number and polarisation densities. In the…

Statistical Mechanics · Physics 2023-02-08 Daniel Borgis , Damien Laage , Luc Belloni , Guillaume Jeanmairet

Understanding the pressure-dependent dielectric properties of water is crucial for a wide range of scientific and practical applications. In this study, we employ a deep neural network trained on density functional theory data to…

Materials Science · Physics 2026-03-31 Yizhi Song , Xifan Wu

The dielectric response of nano-confined fluids is crucial across technologies and biological systems, yet its calculation and interpretation from molecular simulations are often muddled by unclear boundary conditions. We re-derive the…

Soft Condensed Matter · Physics 2026-05-06 Philipp Stärk , Henrik Stooß , Philip Loche , Douwe Jan Bonthuis , Roland R. Netz , Alexander Schlaich