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We study the dynamics of optically-induced nuclear spin polarization in a fluorine-doped ZnSe epilayer via time-resolved Kerr rotation. The nuclear polarization in the vicinity of a fluorine donor is induced by interaction with coherently…

Mesoscale and Nanoscale Physics · Physics 2016-02-24 F. Heisterkamp , E. Kirstein , A. Greilich , E. A. Zhukov , T. Kazimierczuk , D. R. Yakovlev , A. Pawlis , M. Bayer

Dynamic nuclear polarization enables the hyperpolarization of nuclear spins beyond the thermal-equilibrium Boltzmann distribution. However, it is often unclear why the experimentally measured hyperpolarization is below the theoretical…

Chemical Physics · Physics 2023-12-13 Gevin von Witte , Aaron Himmler , Sebastian Kozerke , Matthias Ernst

Thermal motion of the flux lines (FL) gives rise to fluctuating magnetic fields. These dynamic fields couple to the nuclei in the sample and relax the nuclear spins. Based on a model of harmonic fluctuations, we provide a theoretical…

Condensed Matter · Physics 2009-10-22 Lei Xing , Yia-Chung Chang

The physics of interacting nuclear spins arranged in a crystalline lattice is typically described using a thermodynamic framework: a variety of experimental studies in bulk solid-state systems have proven the concept of a spin temperature…

Mesoscale and Nanoscale Physics · Physics 2009-07-21 P. Maletinsky , M. Kroner , A. Imamoglu

We present a detailed analytical and numerical analysis of the nuclear spin dynamics in parabolic quantum wells. The shallow potential of parabolic quantum wells permits substantial modification of the electronic wave function in small…

Materials Science · Physics 2009-11-10 I. Tifrea , Michael E. Flatte

Low frequency spin fluctuation dynamics in paramagnetic spinel LiV$_2$O$_4$, a rare 3$d$-electron heavy fermion system, is investigated. A parametrized self-consistent renormalization (SCR) theory of the dominant AFM spin fluctuations is…

Strongly Correlated Electrons · Physics 2009-11-13 V. Yushankhai , T. Takimoto , P. Thalmeier

We analyze the nuclear magnetic relaxation rate $(1/T_1)_{orb}$ due to the coupling of nuclear spin to the orbital moment of itinerant electrons in metals. In the clean non--interacting case, contributions from large--distance current…

Superconductivity · Physics 2013-05-29 A. Knigavko , B. Mitrovic , K. V. Samokhin

We report achieving enhanced nuclear magnetization in a magnetic resonance force microscope experiment at 0.6 tesla and 4.2 kelvin using the dynamic nuclear polarization (DNP) effect. In our experiments a microwire coplanar waveguide…

Our measurements of $^{125}$Te NMR relaxations reveal an enhancement of electronic spin fluctuations above $\mu_0H^*\sim15$ T, leading to their divergence in the vicinity of the metamagnetic transition at $\mu_0H_m\approx35$ T, below which…

The effect of electron-nuclear spin interactions on qubit operations is investigated for a qubit represented by the spin of an electron localized in a self-assembled quantum dot. The localized electron wave function is evaluated within the…

Quantum Physics · Physics 2009-11-10 Seungwon Lee , Paul von Allmen , Fabiano Oyafuso , Gerhard Klimeck , K. Birgitta Whaley

75As NMR measurements were performed as a function of temperature and doping in (Eu1-xKx)Fe2As2 (x=0,0.38,0.5,0.7) samples. The large Eu2+ moments and their fluctuations are found to dominate the 75As NMR properties. The 75As nuclei close…

Superconductivity · Physics 2013-11-06 Tusharkanti Dey , P. Khuntia , A. V. Mahajan , Anupam , Z. Hossain

This paper proposes an effective diffusion equation method to analyze nuclear magnetic resonance (NMR) relaxation. NMR relaxation is a spin system recovery process, where the evolution of the spin system is affected by the random field due…

Chemical Physics · Physics 2021-03-31 Guoxing Lin

Not all noise in experimental measurements is unwelcome. Certain fundamental noise sources contain valuable information about the system itself -- a notable example being the inherent voltage fluctuations that exist across any resistor…

Disordered Systems and Neural Networks · Physics 2009-11-10 S. A. Crooker , D. G. Rickel , A. V. Balatsky , D. L. Smith

We report on measurements of the spin lifetime of nuclear spins strongly coupled to a micromechanical cantilever as used in magnetic resonance force microscopy. We find that the rotating-frame correlation time of the statistical nuclear…

Mesoscale and Nanoscale Physics · Physics 2008-04-04 C. L. Degen , M. Poggio , H. J. Mamin , D. Rugar

The polarisation dynamics of nuclear spins weakly coupled to an NV center is highly sensitive to the parameters of the microwave control and the nuclear Larmor frequency. What is commonly regarded as a challenge, we propose here as a…

Quantum Physics · Physics 2018-10-24 Q. Chen , Z. -Y. Wang , B. Tratzmiller , I. Schwartz , M. B. Plenio

The available theoretical approaches aiming at describing Dynamic Nuclear spin Polarization (DNP) in solutions containing molecules of biomedical interest and paramagnetic centers are not able to model the behaviour observed upon varying…

Statistical Mechanics · Physics 2014-06-06 Sonia Colombo Serra , Marta Filibian , Pietro Carretta , Alberto Rosso , Fabio Tedoldi

In dynamic nuclear polarization (DNP) experiments, the compound is driven out-of-equilibrium by microwave (MW) irradiation of the radical electron spins. Their stationary state has been recently probed via electron double resonance (ELDOR)…

Strongly Correlated Electrons · Physics 2017-02-28 Filippo Caracciolo , Marta Filibian , Pietro Carretta , Alberto Rosso , Andrea De Luca

Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…

The spin of a confined electron, when oriented originally in some direction, will lose memory of that orientation after some time. Physical mechanisms leading to this relaxation of spin memory typically involve either coupling of the…

Mesoscale and Nanoscale Physics · Physics 2013-07-24 A. C. Johnson , J. R. Petta , J. M. Taylor , A. Yacoby , M. D. Lukin , C. M. Marcus , M. P. Hanson , A. C. Gossard

We present formulas for the nuclear and electronic spin relaxation times due to the hyperfine interaction for nanostructed systems and show that the times depend on the square of the local density of electronic states at the nuclear…

Condensed Matter · Physics 2009-11-07 Ionel Tifrea , Michael E. Flatte