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We review recent theoretical and experimental advances toward understanding the effects of nuclear spins in confined nanostructures. These systems, which include quantum dots, defect centers, and molecular magnets, are particularly…

Mesoscale and Nanoscale Physics · Physics 2009-09-15 W. A. Coish , J. Baugh

One of the key challenges in spectroscopy is inhomogeneous broadening that masks the homogeneous spectral lineshape and the underlying coherent dynamics. A variety of techniques including four-wave mixing and spectral hole-burning are used…

We demonstrate methods to locally control the spin rotation of moving electrons in a GaAs channel. The Larmor frequency of optically-injected spins is modulated when the spins are dragged through a region of spin-polarized nuclei created at…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 M. E. Nowakowski , G. D. Fuchs , S. Mack , N. Samarth , D. D. Awschalom

Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…

Chemical Physics · Physics 2026-04-22 Matthias Diez , Johannes K. Krondorfer , Albert Hirtenfelder , Andreas W. Hauser

We report a comparison of the $1/T_1$ spin lattice relaxation rates (SLR) for $^9Li$ and $^8Li$ in Pt and SrTiO$_{3}$, in order to differentiate between magnetic and electric quadrupolar relaxation mechanisms. In Pt, the ratio of the…

We theoretically and numerically investigate the spin fluctuations induced in a thermal atomic ensemble by an external fluctuating uniaxial magnetic field, in the context of a standard spin noise spectroscopy (SNS) experiment. We show that…

Quantum Physics · Physics 2023-10-05 J. Delpy , S. Liu , P. Neveu , C. Roussy , Th. Jolicoeur , F. Bretenaker , F. Goldfarb

We investigate in detail, using both analytical and numerical tools, the decoherence of electron spins in quantum dots (QDs) coupled to a bath of nuclear spins in magnetic fields or with various initial bath polarizations, focusing on the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Wenxian Zhang , V. V. Dobrovitski , K. A. Al-Hassanieh , E. Dagotto , B. N. Harmon

Optical spin pumping of color centers in diamond is presently attracting broad interest as a platform for dynamic nuclear polarization at room temperature, but the mechanisms involved in the generation and transport of polarization within…

We demonstrate that CPMG and XYXY decoupling sequences with non-ideal $\pi$ pulses can reduce dipolar interactions between spins of the same species in solids. Our simulations of pulsed electron spin resonance (ESR) experiments show that…

Mesoscale and Nanoscale Physics · Physics 2018-07-16 Evan S. Petersen , A. M. Tyryshkin , K. M. Itoh , Joel W. Ager , H. Riemann , N. V. Abrosimov , P. Becker , H. -J. Pohl , M. L. W. Thewalt , S. A. Lyon

Doping dependence of the spin fluctuations and the electron correlations in the effective five-band Hubbard model for iron pnictides is investigated using the fluctuation-exchange approximation. For a moderate hole doping, we find a…

Superconductivity · Physics 2010-07-21 Hiroaki Ikeda , Ryotaro Arita , Jan Kuneš

At the magnetic fields of common NMR instruments, electron Zeeman frequencies are too high for efficient electron-nuclear dipolar cross-relaxation to occur in solution. The rate of that process fades with the electron Zeeman frequency as…

Quantum Physics · Physics 2021-04-22 Maria Grazia Concilio , Murari Soundararajan , Lucio Frydman , Ilya Kuprov

Spin relaxation of a single electron in a weakly coupled double quantum dot is calculated numerically. The phonon assisted spin flip is allowed by the presence of the linear and cubic spin-orbit couplings and nuclear spins. The rate is…

Mesoscale and Nanoscale Physics · Physics 2014-09-02 Martin Raith , Thomas Pangerl , Peter Stano , Jaroslav Fabian

As the number of spins in an ensemble is reduced, the statistical uctuations in its polarization eventually exceed the mean thermal polarization. This transition has now been surpassed in a number of recent nuclear magnetic resonance…

Mesoscale and Nanoscale Physics · Physics 2014-08-26 B. E. Herzog , D. Cadeddu , F. Xue , P. Peddibhotla , M. Poggio

The spin dynamics of positively (X$^{+}$) and negatively (X$^{-}$) charged excitons in InP/In$_{0.48}$Ga$_{0.52}$P quantum dots subject to a magnetic field is studied. We find that a characteristic feature of the system under study is the…

Mesoscale and Nanoscale Physics · Physics 2019-12-18 S. V. Nekrasov , I. A. Akimov , Yu. G. Kusrayev , D. R. Yakovlev , M. Bayer

Hyperpolarized nanoparticles (NPs) offer high polarization levels with room temperature relaxation times exceeding half an hour. In this work, we demonstrate that the achievable hyperpolarization enhancement and relaxation (decay) time at…

Nuclear spin-lattice relaxation in one-dimensional Heisenberg ferrimagnets is studied by means of a modified spin-wave theory. Calculating beyond the first-order mechanism, where a nuclear spin directly interacts with spin waves through the…

Strongly Correlated Electrons · Physics 2015-06-25 Shoji Yamamoto , Hiromitsu Hori

A sensitivity increase of two orders of magnitude in proton (1H) and carbon (13C) spins via dynamic nuclear polarization (DNP) has been accomplished recently using a compact benchtop DNP polarizer operating at 1 T and 77 K. However the DNP…

Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Ramin M. Abolfath , Anna Trojnar , Bahman Roostaei , Thomas Brabec , Pawel Hawrylak

Motivated by a recent proposal by O. P. Sushkov and co-workers to search for a P,T-violating Schiff moment of the $^{207}$Pb nucleus in a ferroelectric solid, we have carried out a high-field nuclear magnetic resonance study of the…

Other Condensed Matter · Physics 2013-01-15 L. -S. Bouchard , A. O. Sushkov , D. Budker , J. J. Ford , A. S. Lipton

We present dynamic nuclear polarization (DNP) in the simplest pseudospin quantum Hall ferromagnet (QHF) of an InSb two-dimensional electron gas with a large g factor using tilted magnetic fields. The DNP-induced amplitude change of a…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 H. W. Liu , K. F. Yang , T. D. Mishima , M. B. Santos , Y. Hirayama
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