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We theoretically designed and experimentally demonstrated a mechanism to protect a spatially segregated mixed light-matter state, known as intercavity exciton-polariton in strongly coupled optical cavities. This excitation, shared across…

The interaction of light with solids can be dramatically enhanced owing to electron-photon momentum matching. This mechanism is driven by either quantum confinement or long-range structural correlations in media with crystal-liquid duality.…

A theoretical variation between the two distinct light-matter coupling regimes, namely weak and strong coupling, becomes uniquely feasible in open optical Fabry-P\'erot microcavities with low mode volume, as discussed here. In combination…

Applied Physics · Physics 2019-12-02 Franziska Wall , Oliver Mey , Lorenz Maximilian Schneider , Arash Rahimi-Iman

In recent years, hybrid organic-inorganic metal halides have been at the forefront of materials research. Typically, the functional (e.g., optoelectronic) properties of hybrid halides are derived from the inorganic structural part, whereas…

Strong coupling of photons and materials in semiconductor nanocavity systems has been investigated because of its potentials in quantum information processing and related applications, and has been testbeds for cavity quantum…

Other Condensed Matter · Physics 2015-05-13 M. Nomura , N. Kumagai , S. Iwamoto , Y. Ota , Y. Arakawa

Lead-free metal halide perovskites are emerging as less-toxic alternatives to their lead-based counterparts. However, their applicability in optoelectronic devices is limited, and the charge transport dynamics remain poorly understood.…

Coherent light-matter interaction at the single photon and electronic qubit level promises the remarkable potential for nonclassical information processing. Against the efforts of improving the figure of merit of the cavities, here we…

Quantum Physics · Physics 2015-06-19 Yong-Chun Liu , Xingsheng Luan , Hao-Kun Li , Qihuang Gong , Chee Wei Wong , Yun-Feng Xiao

Superfluorescence, the cooperative burst of spontaneous emission from an ensemble of dipoles, arises when microscopic oscillators spontaneously synchronize their phases. Here we show that this process can be reversed in time within quantum…

We study the optical properties of coupled quantum dot-microcavity systems with elliptical cross section. First, we develop an analytic model that describes the spectrum of the cavity modes that are split due to the reduced symmetry of the…

Optical orientation of carrier spins by circularly polarized light is the basis of spin physics in semiconductors. Here, we demonstrate strong optical orientation of 85\%, approaching the ultimate limit of unity, for excitons in…

Two-dimensional semiconductors host excitons with very large oscillator strengths and binding energies due to significantly reduced carrier screening. Two-dimensional semiconductors integrated with optical cavities are emerging as a…

We introduce crystal polaritons, hybrid excitations formed when the collective excitations of a periodic quantum-emitter array strongly couple to the resonant Bloch modes of a metasurface. This realizes a cavity-QED platform in which…

Halide perovskite materials raised tremendous interest in recent years since their cheap fabrication, superior performance in both solar cell and light emitting diode (LED). Due to the existence of layered quantum well structure, quasi…

Materials Science · Physics 2021-11-23 Wei Tang , Liting Tao , Tian Zhang , Yanjun Fang , Deren Yang , Linjun Li

Advances in opto-electronics require the development of materials with novel and engineered characteristics. A class of materials that has garnered tremendous interest is metal-halide perovskites, stimulated by meteoric increases in…

We study theoretically the excitonic nonlinearity in hybrid organic-inorganic Ruddlesden-Popper perovskite thin films. The composite layered structure of these materials allows for flexible modulation of their excitonic response between the…

Mesoscale and Nanoscale Physics · Physics 2022-11-14 D. A. Baghdasaryan , E. S. Hakobyan , D. B. Hayrapetyan , I. V. Iorsh , I. A. Shelykh , V. Shahnazaryan

The discovery of lead free all-inorganic alloyed double perovskites have revolutionized photovoltaic research, showing promising light emitting efficiency and its tunability. However, detailed studies regarding optical, exciton, polaron and…

Materials Science · Physics 2021-10-26 Manjari Jain , Manish Kumar , Preeti Bhumla , Saswata Bhattacharya

Microcavity exciton polaritons (polaritons) as part-light part-matter quasiparticles, garner significant attention for non-equilibrium Bose-Einstein condensation at elevated temperatures. Recently, halide perovskites have emerged as…

Nonperturbative coupling between cavity photons and excitons leads to formation of hybrid light-matter excitations termed polaritons. In structures where photon absorption leads to creation of excitons with aligned permanent dipoles, the…

Mesoscale and Nanoscale Physics · Physics 2018-11-30 Emre Togan , Hyang-Tag Lim , Stefan Faelt , Werner Wegscheider , Atac Imamoglu

In a standard semiconductor laser, electrons and holes recombine via stimulated emission to emit coherent light, in a process that is far from thermal equilibrium. Exciton-polariton condensates -- sharing the same basic device structure as…

Cavity-polaritons in semiconductor microstructures have emerged as a promising system for exploring nonequilibrium dynamics of many-body systems. Key advances in this field, including the observation of polariton condensation,…

Mesoscale and Nanoscale Physics · Physics 2019-04-05 Aymeric Delteil , Thomas Fink , Anne Schade , Sven Höfling , Christian Schneider , Ataç Imamoğlu