English

Room-temperature continuous-wave pumped exciton polariton condensation in a perovskite microcavity

Optics 2024-02-16 v2 Mesoscale and Nanoscale Physics Materials Science

Abstract

Microcavity exciton polaritons (polaritons) as part-light part-matter quasiparticles, garner significant attention for non-equilibrium Bose-Einstein condensation at elevated temperatures. Recently, halide perovskites have emerged as promising room-temperature polaritonic platforms thanks to their large exciton binding energies and superior optical properties. However, currently, inducing room-temperature non-equilibrium polariton condensation in perovskite microcavities requires optical pulsed excitations with high excitation densities. Herein, we demonstrate continuous-wave optically pumped polariton condensation with an exceptionally low threshold of ~0.6 W cm-2 and a narrow linewidth of ~1 meV. Polariton condensation is unambiguously demonstrated by characterizing the nonlinear behavior and coherence properties. We also identify a microscopic mechanism involving the potential landscape in the perovskite microcavity, where numerous discretized energy levels arising from the hybridization of adjacent potential minima enhance the polariton relaxation, facilitating polariton condensate formation. Our findings lay the foundation for the next-generation energy-efficient polaritonic devices operating at room temperature.

Keywords

Cite

@article{arxiv.2311.12381,
  title  = {Room-temperature continuous-wave pumped exciton polariton condensation in a perovskite microcavity},
  author = {Jiepeng Song and Sanjib Ghosh and Xinyi Deng and Qiuyu Shang and Xinfeng Liu and Yubin Wang and Xiaoyue Gao and Wenkai Yang and Xianjin Wang and Qing Zhao and Kebin Shi and Peng Gao and Qihua Xiong and Qing Zhang},
  journal= {arXiv preprint arXiv:2311.12381},
  year   = {2024}
}

Comments

16 pages, 4 figures