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As a candidate Kitaev material, Na$_2$Co$_2$TeO$_6$ exhibits intriguing magnetism on a honeycomb lattice that is believed to be $C_3$-symmetric. Here we report a neutron diffraction study of high quality single crystals under $a$-axis…

Strongly Correlated Electrons · Physics 2023-06-06 Weiliang Yao , Yang Zhao , Yiming Qiu , Christian Balz , J. Ross Stewart , Jeffrey W. Lynn , Yuan Li

We report magnetometry data obtained on twin-free single crystals of Na3Co2SbO6, which is considered a candidate material for realizing the Kitaev honeycomb model for quantum spin liquids. Contrary to a common belief that such materials can…

We have synthesized single crystals of Na$_3$Co$_2$SbO$_6$ and characterized the structure and magnetic order by measuring anisotropic magnetic properties, heat capacity, x-ray and neutron single crystal diffraction. Magnetic properties and…

Strongly Correlated Electrons · Physics 2019-07-17 J. -Q. Yan , S. Okamoto , Y. Wu , Q. Zheng , H. D. Zhou , H. B. Cao , M. A. McGuire

We report a rich anisotropic magnetic phase diagram of Na$_3$Co$_2$SbO$_6$, a previously proposed cobaltate Kitaev candidate, based on field- and temperature-dependent magnetization, specific heat, and magnetocaloric effect studies. At low…

Cobalt-based quantum magnets forming layered honeycomb arrangements have attracted much attention recently, as they are considered as a potential platform for materials with exotic Kitaev spin exchange. Amongst the discussed candidate…

Strongly Correlated Electrons · Physics 2026-05-28 Abdul Basit , Richard A. Mole , Alex J. Brown , Jiatu Liu , Chris D. Ling , Stephan Rachel

Recent experimental studies of the spin-1 honeycomb antiferromagnet Na$_3$Ni$_2$BiO$_6$ have revealed a pronounced one-third magnetization plateau under applied magnetic fields, highlighting the presence of strong magnetic frustration and…

Strongly Correlated Electrons · Physics 2026-02-05 Amanda A. Konieczna , P. Peter Stavropoulos , Roser Valentí

The Kitaev honeycomb model has received significant attention for its exactly solvable quantum spin liquid ground states and fractionalized excitations. For realizing the model, layered cobalt oxides have been considered a promising…

Strongly Correlated Electrons · Physics 2025-01-27 Yuchen Gu , Xianghong Jin , Yuan Li

Recent studies suggest that the candidate Kitaev magnet Na$_2$Co$_2$TeO$_6$ possesses novel triple-$\mathbf{q}$ magnetic order instead of conventional single-$\mathbf{q}$ zigzag order. Here we present dedicated experiments in search for…

Strongly Correlated Electrons · Physics 2025-09-24 Xianghong Jin , Mengqiao Geng , Fabio Orlandi , Dmitry Khalyavin , Pascal Manuel , Yang Liu , Yuan Li

BaCo$_2$(AsO$_4$)$_2$ (BCAO), a honeycomb cobaltate, is considered a promising candidate for materials displaying the Kitaev quantum spin liquid state. This assumption is based on the distinctive characteristics of Co$^{2+}$ ions (3$d^7$)…

Strongly Correlated Electrons · Physics 2024-08-02 Sangyun Lee , Shengzhi Zhang , S. M. Thomas , L. Pressley , C. A. Bridges , Eun Sang Choi , Vivien S. Zapf , Stephen M. Winter , Minseong Lee

Recent theoretical studies have suggested that the low-energy Hamiltonian of honeycomb cobaltate systems could be dominated by anisotropic Kitaev interactions. Motivated by the theory, a honeycomb layered material Na$_{2}$Co$_{2}$TeO$_{6}$…

Strongly Correlated Electrons · Physics 2023-08-14 Emilie Dufault , Faranak Bahrami , Alenna Streeter , Xiaohan Yao , Enrique Gonzalez , Qiang Zhang , Fazel Tafti

The Kitaev candidate material Na$_2$Co$_2$TeO$_6$ is proposed to be proximate to a quantum spin liquid state but a suitable spin model and the nature of its ground states are still under debate. Our high-frequency/high-field electron spin…

Strongly Correlated Electrons · Physics 2025-09-08 Luca Bischof , Jan Arneth , Raju Kalaivanan , Raman Sankar , Kwang-Yong Choi , Rüdiger Klingeler

The honeycomb magnet Na$_3$Co$_2$SbO$_6$ recently emerged as a promising candidate for realizing Kitaev quantum spin liquid with relatively low levels of structural disorder. While the precise spin Hamiltonian remains controversial, the…

Strongly Correlated Electrons · Physics 2025-07-16 Rongsheng Li , Liyu Shi , Yuchen Gu , Yue Chen , Xintong Li , Qiong Wu , Shuxiang Xu , Dong Wu , Yuan Li , Fa Wang , Tao Dong , Nanlin Wang

Li3Co2SbO6 is prepared by molten salt ion exchange and its structure refined by the Rietveld method confirming the honeycomb-type Co/Sb ordering of its Na precursor. Monoclinic rather than trigonal symmetry of Na3Co2SbO6 is directly…

We present magnetization and dilatometry measurements on the honeycomb cobaltate Na$_3$Co$_2$SbO$_6$ and map out its detailed field-temperature phase diagram down to sub-Kelvin temperatures. Our data for in-plane magnetic fields show a…

We present a comprehensive study of single crystals of Na2Co2TeO6, a putative Kitaev honeycomb magnet, focusing on its low-temperature phase behaviors. A new thermal phase transition is identified at 31.0 K, below which the system develops…

Strongly Correlated Electrons · Physics 2021-05-26 Wenjie Chen , Xintong Li , Zhenhai Hu , Ze Hu , Li Yue , Ronny Sutarto , Feizhou He , Kazuki Iida , Kazuya Kamazawa , Weiqiang Yu , Xi Lin , Yuan Li

The search for Kitaev's quantum spin liquid (KQSL) state in real materials has recently expanded with the prediction that honeycomb lattices of divalent, high-spin cobalt ions could host the dominant bond-dependent exchange interactions…

The synthesis, structure, and basic magnetic properties of Na2Co2TeO6 and Na3Co2SbO6 are reported. The crystal structures were determined by neutron powder diffraction. Na2Co2TeO6 has a two-layer hexagonal structure (space group P6322)…

Materials Science · Physics 2022-04-26 L. Viciu , Q. Huang , E. Morosan , H. W. Zandbergen , N. I. Greenbaum , T. McQueen , R. J. Cava

The identification of quantum spin liquid phases in Kitaev candidate materials remains a major experimental challenge. Since most Kitaev candidates develop antiferromagnetic (AFM) order at low temperatures, currently there are great…

The magnetic orders in Na$_2$IrO$_3$ and $\alpha-$RuCl$_3$, honeycomb systems with strong spin-orbit coupling and correlations, have been recently described by models with the dominant Kitaev interactions. In this work we discuss how the…

Strongly Correlated Electrons · Physics 2017-02-10 Yuriy Sizyuk , Peter Woelfle , Natalia B. Perkins

Layered {\alpha}-RuCl3 is a promising material to potentially realize the long-sought Kitaev quantum spin liquid with fractionalized excitations. While evidence of this exotic state has been reported under a modest in-plane magnetic field,…

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