English

Robust triple-q magnetic order with trainable spin vorticity in Na$_2$Co$_2$TeO$_6$

Strongly Correlated Electrons 2025-09-24 v1

Abstract

Recent studies suggest that the candidate Kitaev magnet Na2_2Co2_2TeO6_6 possesses novel triple-q\mathbf{q} magnetic order instead of conventional single-q\mathbf{q} zigzag order. Here we present dedicated experiments in search for distinct properties expected of the triple-q\mathbf{q} order, namely, insensitivity of the magnetic domains to weak C3C_3 symmetry-breaking fields and fictitious magnetic fields generated by the spin vorticity. In structurally pristine single crystals, we show that C3C_3 symmetry-breaking in-plane uniaxial strains do not affect the order's magnetic neutron diffraction signals. We further show that c\mathbf{c}-axis propagating light exhibits large Faraday rotations in the ordered state due to the spin vorticity, the sign of which can be trained via the system's ferrimagnetic moment. These results are in favor of the triple-q\mathbf{q} order in Na2_2Co2_2TeO6_6 and reveal its unique emerging behavior.

Keywords

Cite

@article{arxiv.2501.07843,
  title  = {Robust triple-q magnetic order with trainable spin vorticity in Na$_2$Co$_2$TeO$_6$},
  author = {Xianghong Jin and Mengqiao Geng and Fabio Orlandi and Dmitry Khalyavin and Pascal Manuel and Yang Liu and Yuan Li},
  journal= {arXiv preprint arXiv:2501.07843},
  year   = {2025}
}

Comments

4 pages, 4 figures, plus Supplemental Material