Ferrimagnetism from triple-q order in Na$_2$Co$_2$TeO$_6$
Abstract
The candidate Kitaev magnet NaCoTeO exhibits a characteristic ferrimagnetic response at low temperatures, with a finite residual magnetization that changes sign at a compensation point located at around half the ordering temperature. We argue that the behavior can be naturally understood to arise in this material as a consequence of a noncollinear triple- magnetic ground state. Using large-scale classical Monte Carlo simulations, we study the finite-temperature response of the pertinent honeycomb Heisenberg-Kitaev-- model in weak training fields. Our model features all symmetry-allowed nearest-neighbor exchange interactions, as well as sublattice-dependent next-nearest-neighbor interactions, consistent with the reported crystal structure of the material. We also consider a six-spin ring exchange perturbation, which allows us to tune between the two different magnetic long-range orders that have been suggested for this material in the literature, namely, a collinear single- zigzag state and a noncollinear triple- state. We demonstrate that the experimentally-observed ferrimagnetic response of NaCoTeO can be well described within our modeling if the magnetic ground state features noncollinear triple- order. The observation of a compensation point, where the residual magnetization reverses sign, suggests a sublattice -factor anisotropy, with a larger out-of-plane -factor on the sublattice with stronger antiferromagnetic intrasublattice exchange. By contrast, a classical Heisenberg-Kitaev---type model with collinear zigzag ground state is insufficient even in principle to describe the observed behavior. Our results illustrate the unconventional physics of noncollinear magnetic long-range orders hosted by frustrated magnets with bond-dependent interactions.
Cite
@article{arxiv.2409.12234,
title = {Ferrimagnetism from triple-q order in Na$_2$Co$_2$TeO$_6$},
author = {Niccolò Francini and Lukas Janssen},
journal= {arXiv preprint arXiv:2409.12234},
year = {2025}
}
Comments
12 pages, 6 figures; v2:published version