English

Ferrimagnetism from triple-q order in Na$_2$Co$_2$TeO$_6$

Strongly Correlated Electrons 2025-02-21 v2 Statistical Mechanics

Abstract

The candidate Kitaev magnet Na2_2Co2_2TeO6_6 exhibits a characteristic ferrimagnetic response at low temperatures, with a finite residual magnetization that changes sign at a compensation point located at around half the ordering temperature. We argue that the behavior can be naturally understood to arise in this material as a consequence of a noncollinear triple-q\mathbf{q} magnetic ground state. Using large-scale classical Monte Carlo simulations, we study the finite-temperature response of the pertinent honeycomb Heisenberg-Kitaev-Γ\Gamma-Γ\Gamma' model in weak training fields. Our model features all symmetry-allowed nearest-neighbor exchange interactions, as well as sublattice-dependent next-nearest-neighbor interactions, consistent with the reported crystal structure of the material. We also consider a six-spin ring exchange perturbation, which allows us to tune between the two different magnetic long-range orders that have been suggested for this material in the literature, namely, a collinear single-q\mathbf{q} zigzag state and a noncollinear triple-q\mathbf{q} state. We demonstrate that the experimentally-observed ferrimagnetic response of Na2_2Co2_2TeO6_6 can be well described within our modeling if the magnetic ground state features noncollinear triple-q\mathbf{q} order. The observation of a compensation point, where the residual magnetization reverses sign, suggests a sublattice gg-factor anisotropy, with a larger out-of-plane gg-factor on the sublattice with stronger antiferromagnetic intrasublattice exchange. By contrast, a classical Heisenberg-Kitaev-Γ\Gamma-Γ\Gamma'-type model with collinear zigzag ground state is insufficient even in principle to describe the observed behavior. Our results illustrate the unconventional physics of noncollinear magnetic long-range orders hosted by frustrated magnets with bond-dependent interactions.

Keywords

Cite

@article{arxiv.2409.12234,
  title  = {Ferrimagnetism from triple-q order in Na$_2$Co$_2$TeO$_6$},
  author = {Niccolò Francini and Lukas Janssen},
  journal= {arXiv preprint arXiv:2409.12234},
  year   = {2025}
}

Comments

12 pages, 6 figures; v2:published version