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We use molecular dynamics simulations to test integral equation theory predictions for the structure of fluids of spherical particles with eight different piecewise-constant pair interaction forms comprising a hard core and a combination of…

Soft Condensed Matter · Physics 2015-05-01 Kyle B. Hollingshead , Thomas M. Truskett

Liquid state entropy formulas based on configurational probability distributions are examined for Lennard-Jones fluids across a range temperatures and densities. These formulas are based on expansions of the entropy in series of $n$-body…

Statistical Mechanics · Physics 2023-12-19 Yang Huang , Michael Widom

Using the first seven known virial coefficients and forcing it to possess two branch-point singularities, a new equation of state for the hard-sphere fluid is proposed. This equation of state predicts accurate values of the higher virial…

Soft Condensed Matter · Physics 2009-06-26 Andrés Santos , Mariano López de Haro

We propose an improved effective-medium theory to obtain the concentration dependence of the viscosity of particle suspensions at arbitrary volume fractions. Our methodology can be applied, in principle, to any particle shape as long as the…

Soft Condensed Matter · Physics 2010-06-01 I. Santamaria-Holek , Carlos I. Mendoza

We derive the Ornstein-Zernike equation for molecular crystals of axially symmetric particles and apply the Percus-Yevick approximation to this system. The one-particle orientational distribution function has a nontrivial dependence on the…

Statistical Mechanics · Physics 2016-08-31 Michael Ricker , Rolf Schilling

The excess entropy of restricted primitive model electrolytes is calculated using a potential based approach through the symmetric Poisson-Boltzmann and the modified Poisson-Boltzmann theories. The theories are utilized in conjunction with…

Statistical Mechanics · Physics 2025-04-01 S. Lamperski , L. B. Bhuiyan , C. W. Outhwaite , R. Gorniak

We consider the effect of intermolecular interactions on the optimal size-distribution of $N$ hard spheres that occupy a fixed total volume. When we minimize the free-energy of this system, within the Percus-Yevick approximation, we find…

Soft Condensed Matter · Physics 2009-10-31 Junfang Zhang , Ronald Blaak , Emmanuel Trizac , Jose A. Cuesta , Daan Frenkel

We propose a new method to compute the free energy or enthalpy of fluids or disordered solids by computer simulation . The main idea is to construct a reference system by freezing one representative configuration, and then carry out a…

Computational Physics · Physics 2011-03-16 Friederike Schmid , Tanja Schilling

The hard sphere repulsion among ions can be considered in the Poisson-Nernst-Planck (PNP) equations by combining the fundamental measure theory (FMT). To reduce the nonlocal computational complexity in 3D simulation of biological systems, a…

Chemical Physics · Physics 2016-03-23 Yu Qiao , Benzhuo Lu , Minxin Chen

An iterative Monte Carlo inversion method for the calculation of particle pair potentials from given particle pair correlations is proposed in this paper. The new method, which is best referred to as Iterative Ornstein-Zernike Inversion,…

Soft Condensed Matter · Physics 2018-04-13 Marco Heinen

I first calculate the charged spherical Renyi entropy by a numerical method that does not require knowledge of any eigenvalue degeneracies, and applies to all odd dimensions. An image method is used to relate the full sphere values to those…

High Energy Physics - Theory · Physics 2016-01-26 J. S. Dowker

We compare two calculations of the particle density in the superfluid phase of the classical XY model with a chemical potential $\mu$ in 1+1 dimensions.The first relies on exact blocking formulas from the Tensor Renormalization Group (TRG)…

Statistical Mechanics · Physics 2016-01-26 Li-Ping Yang , Yuzhi Liu , Haiyuan Zou , Z. Y. Xie , Y. Meurice

Integral equation of pure liquids, combined with a new "scaling approximation" based on a corresponding states treatment of pair correlation functions, is used to evaluate approximate structure factors for colloidal fluids constituted of…

A closed virial equation-of-state for the low density fluid phase of hard disks is obtained from the known virial coefficients. The equation exhibits 6-figure accuracy for the thermodynamic (MD) pressure up to the reduced number density ~…

Statistical Mechanics · Physics 2010-08-24 Anthony Beris , Leslie V. Woodcock

Confined fluids display complex behavior due to layering and local packing. Here, we disentangle these effects by confining a hard-sphere fluid to the surface of a cylinder, such the circumference extends only over a few particle diameters.…

Soft Condensed Matter · Physics 2020-04-23 Charlotte F. Petersen , Lukas Schrack , Thomas Franosch

A simple result for the pressure of a hard sphere fluid that was developed many years ago by Rennert is extended in a straightforward manner by adding the terms that are of the same form as the Rennert's formula. The resulting expression is…

Soft Condensed Matter · Physics 2013-12-13 D. Henderson

In this work, a one-dimensional model of crystalline solids based on the Dirac comb limit of the Kronig-Penney model is considered. From the wave functions of the valence electrons, we calculate a statistical measure of complexity and the…

Adaptation and Self-Organizing Systems · Physics 2015-06-04 Jaime Sanudo , Ricardo Lopez-Ruiz

We construct a density functional theory (DFT) for the sticky hard sphere (SHS) fluid which, like Rosenfeld's fundamental measure theory (FMT) for the hard sphere fluid [Phys. Rev. Lett. {\bf 63}, 980 (1989)], is based on a set of weighted…

Soft Condensed Matter · Physics 2015-05-20 Hendrik Hansen-Goos , J. S. Wettlaufer

By using the Rosenfeld density functional we determine the number density profiles of both components of binary hard-sphere fluids close to a planar hard wall as well as the corresponding excess coverage and surface tension. The comparison…

Soft Condensed Matter · Physics 2009-10-31 R. Roth , S. Dietrich

The direct correlation function and the (static) structure factor for a seven-dimensional hard-sphere fluid are considered. Analytical results for these quantities are derived within the Percus-Yevick theory

Statistical Mechanics · Physics 2007-05-23 Miguel Robles , Mariano Lopez de Haro , Andres Santos