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Hydrogen as the cleanest energy carrier is a promising alternative renewable resource to fossil fuels. There is an ever-increasing interest in exploring efficient and cost-effective approaches of hydrogen production. Recent experiments have…

Materials Science · Physics 2023-08-29 Zheng Shu , Yongqing Cai

Two-dimensional transition metal-dichalcogenides are emerging as efficient and cost-effective electrocatalysts for hydrogen evolution reaction (HER). However, only the edge sites of their trigonal prismatic phase show HER-electrocatalytic…

X-ray absorption spectroscopy (XAS) and electron energy-loss spectroscopy (EELS) produce detailed information about oxidation state, bonding, and coordination, making them essential for quantitative studies of redox and structure in…

Materials Science · Physics 2026-01-19 Brian Lee , Linna Qiao , Samuel Gleason , Guangwen Zhou , Xiaohui Qu , Judith Yang , Jim Ciston , Deyu Lu

Mitigating the climate crisis requires a rapid transition towards lower-carbon energy. Catalyst materials play a crucial role in the electrochemical reactions involved in numerous industrial processes key to this transition, such as…

Machine Learning · Computer Science 2024-03-12 Alexandre Duval , Victor Schmidt , Santiago Miret , Yoshua Bengio , Alex Hernández-García , David Rolnick

Two-dimensional materials supported by single atom catalysis (SACs) are foreseen to replace platinum for large-scale industrial scalability of sustainable hydrogen generation. Here, a series of metal (Al, Sc, Ti, V, Cr, Mn, Fe, Ni, Cu, Zn)…

Materials Science · Physics 2022-11-04 M. V. Jyothirmai , D. Roshini , B. Moses Abraham , Jayant K. Singh

Surface modification of TiO2 with single-atom catalysts (SACs) is an effective strategy for enhancing photocatalytic efficiency. However, thorough characterization of SACs at the atomic scale remains challenging. X-ray absorption…

Materials Science · Physics 2025-11-12 Yingying Li , David Morris , Peng Zhang

High overpotentials, particularly an issue of common anode materials, hamper the process of water electrolysis for clean energy generation. Thanks to immense research efforts up to date oxygen evolution electrocatalysts based on…

We used density functional theory to computationally design a Zr organometallic catalyst for selectively oxidizing substrates using molecular oxygen as oxidant without coreductant. Each selective oxidation cycle involves four general steps:…

Chemical Physics · Physics 2016-01-01 Bo Yang , Thomas A. Manz

Increasing anthropogenic carbon dioxide (CO$_2$) emissions have led to rising global temperatures and climate change. Using earth-abundant metal-oxide catalysts such as Cu$_2$O for reducing CO$_2$ through RWGS reaction seems lucrative. In…

The complexity of the topological and combinatorial configuration space of MXenes can give rise to gigantic design challenges that cannot be addressed through traditional experimental or routine theoretical approaches. To this end, we…

Materials Science · Physics 2022-12-13 B. Moses Abraham , Priyanka Sinha , Prosun Halder , Jayant K. Singh

In the last several years, there has been a wealth of studies to clarify the role of thin layers of electrocatalysts on semiconducting photoelectrodes to the efficiency of the oxygen evolution reaction (OER). It has been shown that the…

The water gas shift reaction (WGS) is important and widely applied in the production of H2. Cu modified perovskites are promising catalysts for WGS reactions in hydrogen generation. However, the structure-dependent stability and reaction…

The oxygen evolution reaction (OER) is considered a key reaction for electrochemical energy conversion but slow kinetics hamper application in electrolyzers, metal-air batteries and other applications that rely on sustainable protons from…

Materials Science · Physics 2020-10-15 Denis Antipin , Marcel Risch

Transforming CO$_2$ into methanol represents a crucial step towards closing the carbon cycle, with thermoreduction technology nearing industrial application. However, obtaining high methanol yields and ensuring the stability of…

Chemical Physics · Physics 2025-07-08 Prajwal Pisal , Ondrej Krejci , Patrick Rinke

The discovery and optimization of high-performance materials is the basis for advancing energy conversion technologies. To understand composition-property relationships, all available data sources should be leveraged: experimental results,…

Materials Science · Physics 2025-03-03 Lei Zhang , Markus Stricker

Improving the stability of electrocatalysts for the oxygen evolution reaction (OER) through materials design has received less attention than improving their catalytic activity. We explored the effect of Mn addition to a cobalt oxide for…

Materials Science · Physics 2022-02-23 Javier Villalobos , Dulce M. Morales , Denis Antipin , Götz Schuck , Ronny Golnak , Jie Xiao , Marcel Risch

The high-throughput scalable production of cheap, efficient and durable electrocatalysts that work well at high current densities demanded by industry is a great challenge for the large-scale implementation of electrochemical technologies.…

Applied Physics · Physics 2020-08-26 Chi Zhang , Yuting Luo , Junyang Tan , Fengning Yang , Zhiyuan Zhang , Liusi Yang , Hui-Ming Cheng , Bilu Liu

Catalysis has entered everyday life through a number of technological processes relying on different catalytic systems. The increasing demand for such systems requires rationalization of the use of their expensive components, like noble…

Materials Science · Physics 2019-10-29 A. S. Dobrota , I. A. Pašti , A. Z. Jovanović , B. Johansson , N. V. Skorodumova

Identifying and controlling active sites in electrocatalysis remains a grand challenge due to restructuring of catalysts in the complex chemical environments during operation. Inactive precatalysts can transform into active catalysts under…

The precise identification of neurotransmitters is essential for comprehending cerebral function, detecting neurological conditions, and formulating successful therapeutic approaches. The present work investigates the electrochemical…

Materials Science · Physics 2025-11-07 Aravindan Santhan , Kuo Yuan Hwa , Slava V. Rotkin , Cheng-Han Wang , Chun-Wei Ou
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