Related papers: Ultrafast simultaneous manipulation of multiple fe…
Light fields at THz and mid-infrared frequencies allow for the direct excitation of collective modes in condensed matter, which can be driven to large amplitudes. For example, excitation of the crystal lattice, has been shown to stimulate…
In Eu2ZnIrO6, effectively two atoms are active i.e. Ir is magnetically active, which results in complex magnetic ordering within the Ir sublattice at low temperature. On the other hand, although Eu is a van-vleck paramagnet, it is active in…
We used Raman and terahertz spectroscopies to investigate lattice and magnetic excitations and their cross-coupling in the hexagonal YMnO3 multiferroic. Two phonon modes are strongly affected by the magnetic order. Magnon excitations have…
We analyze the ``ferron" excitations in order-disorder ferroelectrics by a microscopic pseudo-spin model. We demonstrate that analogous to magnons, the quanta of spin waves in magnetic materials, ferrons carry both static and oscillating…
When ultrafast laser pulse strikes the crystal with a van Hove singularity in the phonon density of states, it can create a pair of anti-correlated in wave-vector acoustic phonons. As a result, the atomic fluctuations in either position or…
The coexistence and coupling of ferroelasticity and magnetic ordering in a single material offers a great opportunity to realize novel devices with multiple tuning knobs. Complex oxides are a particularly promising class of materials to…
Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…
We propose a theoretical framework for the detection of order parameter fluctuations in three dimensions using ultrafast coherent phonon spectroscopy. We focus our attention on long wavelength charge density fluctuations (plasmons), and…
We resolve the real-time electric field of a femtosecond third-order nonlinear optical signal in the molecular frame. The electric field emitted by the induced third-order polarization from impulsively pre-aligned gas-phase molecules at…
In bismuth ferrite (BiFeO3), antiferromagnetic and ferroelectric order coexist at room temperature, making it of particular interest for studying magnetoelectric coupling. The mutual control of magnetic and electric properties is very…
The phonon dispersion was measured at room temperature along (0,0,L) in the tetragonal phase of LaFeAsO using inelastic x-ray scattering. Spin-polarized first-principles calculations imposing various types of antiferromagnetic order are in…
The coherent nonlinear dynamics between collective excitations, such as magnons and phonons, drive emergent phenomena in quantum materials, yet their direct observation remains a central challenge. Here, using double-terahertz-pump…
We use the frozen phonon method to calculate the anharmonic potential energy surface and to model the ultrafast ferroelectric polarization reversal in LiNbO3 driven by intense pulses of THz light. Before stable switching of the polarization…
Born effective charge (BEC), a fundamental quantity in lattice dynamics and ferroelectric theory, provides a quantitative measure of linear polarization response to ionic displacements. However, it does not account for higher-order effects,…
Negative nonlinear electron-phonon coupling involving an infrared-active phonon mode can lead to an instability towards the formation of a polar lattice distortion with ferrielectric (FE) moments accompanied by an electronic charge-density…
The challenge of achieving ultrafast switching of electric polarization in ferroelectric materials remains unsolved, as there is no experimental evidence of such switching to date. In this study, we have developed an enhanced model that…
The effects of high magnetic fields applied perpendicular to the spontaneous ferroelectric polarization on single crystals of BiFeO$_3$ were investigated through magnetization, magnetostriction, and neutron diffraction measurements. The…
We identify the bosonic excitations in ferroelectrics that carry electric dipoles from the phenomenological Landau-Ginzburg-Devonshire theory. The "ferron" quasi-particles emerge from the concerted action of anharmonicity and broken…
The nonlinear dynamics of magnetization in antiferromagnets, resulting in high-frequency spin waves (high-order harmonics) as signal carriers, enable fast magnetic state switching in spintronic devices. More harmonic orders potentially…
Enabling the light-control of complex systems on ultra-short timescales gives rise to rich physics with promising applications. While crucial, the quantitative determination of both the longitudinal and shear photo-induced strains still…