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We report an observation of extremely long-lived spin states in systems of dipolar-coupled nuclear spins in solids. The 'suspended echo' experiment uses a simple stimulated echo pulse sequence and creates non-equilibrium states which live…

Mesoscale and Nanoscale Physics · Physics 2013-06-17 A. Turanov , A. K. Khitrin

Dissolution dynamical nuclear polarization has been applied in various fields, including chemistry, biology, and medical science. To expand the scope of these applications, the nuclear singlet state, which is decoherence-free against…

We report observation of long-lived spin-singlet states in a 13C-1H spin pair at zero magnetic field. In 13C-labeled formic acid, we observe spin-singlet lifetimes as long as 37 seconds, about a factor of three longer than the T1 lifetime…

We measure the lifetime of long-lived nuclear spin singlet states as a function of the strength of the RF spin-locking field and present a simple theoretical model that agrees well with our measurements, including the low-RF-power regime.…

Chemical Physics · Physics 2015-03-19 Stephen J. DeVience , Ronald L. Walsworth , Matthew S. Rosen

Long-lived states (LLS) involving pairs of magnetically inequivalent but chemically equivalent proton spins in aliphatic (CH$_2$)$_n$ chains can be excited by simultaneous application of weak selective radio-frequency (RF) fields at n…

Chemical Physics · Physics 2022-11-09 Anna Sonnefeld , Geoffrey Bodenhausen , Kirill Sheberstov

A solution with hyperpolarized nuclear spins encoded into a long-lived state has been utilized for sensing chemical phenomena. In a conventional way, nuclear spins are hyperpolarized at very low temperatures. In this work, we demonstrate…

The nuclear spin singlet order involving coupled pairs of spins-1/2 may be used to store nuclear spin hyperpolarization in a room temperature liquid for a time much longer than the spin-lattice relaxation time $T_1$. There both are…

Quantum Physics · Physics 2021-06-02 Y. Yang , L. Zhou , Q. Chen

The coherent high-fidelity generation of nuclear spins in long-lived singlet states which may find application as quantum memory or sensor represents a considerable experimental challenge. Here we propose a dissipative scheme that achieves…

Quantum Physics · Physics 2017-06-28 Q. Chen , I. Schwarz , M. B. Plenio

Coupled pairs of nuclear spins-1/2 support one singlet state and three triplet states. Transitions between the singlet state and one of the triplet states may be driven by an oscillating low-frequency magnetic field, in the presence of…

Quantum Physics · Physics 2021-10-27 Laurynas Dagys , Christian Bengs , Malcolm H. Levitt

We introduce a broadly applicable technique to create nuclear spin singlet states in organic molecules and other many-atom systems. We employ a novel pulse sequence to produce a spin-lock induced crossing (SLIC) of the spin singlet and…

Quantum Physics · Physics 2013-10-30 Stephen J. DeVience , Ronald L. Walsworth , Matthew S. Rosen

We analyze the symmetry properties of the dipolar Hamiltonian as the main relaxation mechanism responsible for the observed NMR spectra of long lived states in methyl groups. Long lived states exhibit relaxation times that are considerably…

Quantum Physics · Physics 2017-04-18 Razieh Annabestani , David Cory

It is shown that long-lived states (LLS) involving pairs of methylene protons in nuclear magnetic resonance (NMR) can be readily excited in common molecules that contain two or more neighboring CH$_2$ groups. Accessing such LLS does not…

Chemical Physics · Physics 2022-07-19 Anna Sonnefeld , Aiky Razanahoera , Geoffrey Bodenhausen , Kirill Sheberstov

Dynamical polarization of nuclear spin ensembles is of central importance for magnetic resonance studies, precision sensing and for applications in quantum information theory. Here we propose a scheme to generate long-lived singlet pairs in…

Quantum Physics · Physics 2017-04-06 Johannes N. Greiner , D. D. Bhaktavatsala Rao , Jörg Wrachtrup

The possibility of appearance of spin polarized states in nuclear matter is studied within the framework of a Fermi liquid theory with Skyrme effective forces in a wide range of isospin asymmetries and densities. There are a few possible…

Nuclear Theory · Physics 2007-05-23 A. A. Isayev

We study systems of coupled spin-gapped and gapless Luttinger liquids. First, we establish the existence of a sliding Luttinger liquid phase for a system of weakly coupled parallel quantum wires, with and without disorder. It is shown that…

Strongly Correlated Electrons · Physics 2009-11-07 Ranjan Mukhopadhyay , C. L. Kane , T. C. Lubensky

Algorithmic cooling methods manipulate an open quantum system in order to lower its temperature below that of the environment. We show that significant cooling is achieved on an ensemble of spin-pair systems by exploiting the long-lived…

It is shown that under changing density or temperature a nucleon Fermi superfluid can undergo a phase transition to an anisotropic superfluid state, characterized by nonvanishing gaps in pairing channels with singlet-singlet (SS) and…

Nuclear Theory · Physics 2009-11-07 A. A. Isayev , G. Röpke

We show how to use polar molecules in an optical lattice to engineer quantum spin models with arbitrary spin S >= 1/2 and with interactions featuring a direction-dependent spin anisotropy. This is achieved by encoding the effective spin…

In quantum mechanical many-body systems, long-range and anisotropic interactions promote rich spatial structure and can lead to quantum frustration, giving rise to a wealth of complex, strongly correlated quantum phases. Long-range…

We study theoretically the formation of the nuclear-spin polaron state in semiconductor nanosystems within the Lindblad equation approach. To this end, we derive a general Lindblad equation for the density operator that complies with the…

Mesoscale and Nanoscale Physics · Physics 2022-06-01 Iris Kleinjohann , Andreas Fischer , Mikhail M. Glazov , Frithjof B. Anders
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