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We investigate ionization at a solid-water interface in applied electric field. We attach an electrode to a dielectric film bearing silanol or carboxyl groups with an areal density $\Gamma_0$, where the degree of dissociation $\alpha$ is…

Soft Condensed Matter · Physics 2016-09-29 Ryuichi Okamoto , Akira Onuki

Solid-state electrolytes, by enabling lithium metal anodes, may significantly increase the energy density of current lithium-ion batteries. However, similar to their liquid counterparts, these hard and stiff electrolytes can still be…

Chemical Physics · Physics 2024-10-04 Rajeev Gopal , Longan Wu , Youngju Lee , Jinzhao Guo , Peng Bai

We introduce an adhesion parameter that enables rapid screening for materials interfaces with high adhesion. This parameter is obtained by density functional theory calculations of individual single-material slabs rather than slabs…

The optical properties of a V4O7 single crystal have been investigated from the high temperature metallic phase down to the low temperature antiferromagnetic insulating one. The temperature dependent behavior of the optical conductivity…

Strongly Correlated Electrons · Physics 2015-06-22 I. Lo Vecchio , M. Autore , F. D'Apuzzo , F. Giorgianni , A. Perucchi , U. Schade , V. N. Andreev , V. A. Klimov , S. Lupi

We report a method to precisely control the atomic defects at grain boundaries (GBs) of monolayer MoS2 by vapor-liquid-solid (VLS) growth using sodium molybdate liquid alloys, which serve as growth catalysts to guide the formations of the…

Graphite is a ubiquitous electrode material with particular promise for use in e.g., energy storage and desalination devices, but very little is known about the properties of the graphite-electrolyte double layer at technologically relevant…

Materials Science · Physics 2021-09-03 Aaron R. Finney , Ian J. McPherson , Patrick R. Unwin , Matteo Salvalaglio

We report an electron-beam based method for the nanoscale patterning of the poly(ethylene oxide)/LiClO$_{4}$ polymer electrolyte. We use the patterned polymer electrolyte as a high capacitance gate dielectric in single nanowire transistors…

Mesoscale and Nanoscale Physics · Physics 2014-04-09 D. J. Carrad , A. M. Burke , R. W. Lyttleton , H. J. Joyce , H. H. Tan , C. Jagadish , K. Storm , H. Linke , L. Samuelson , A. P. Micolich

We demonstrate the realization of (laterally) optically bounded colloidal structures on a liquid-liquid interface of an emulsion droplet. We use DNA tethers to graft the particles to the droplet surface, effectively confining them to a…

Soft Condensed Matter · Physics 2017-03-27 Alessio Caciagli , Darshana Joshi , Jurij Kotar , Erika Eiser

This work presents a scalable method to produce robust all-solid electric double layer capacitors (EDLCs), compatible with roll-to-roll processes and structural laminate composite fabrication. It consists in sandwiching and pressing an…

This study investigates optical and electrical properties of thin melanin films self-organized grown from water solutions of eumelanin extracted from edible plants. The melanin films exhibit the characteristics of a transparent low…

Organic semiconductors are usually not thought to show outstanding performance in highly-integrated, sub 100 nm transistors. Consequently, single-crystalline materials such as SWCNTs, MoS2 or inorganic semiconductors are the material of…

Applied Physics · Physics 2019-10-02 Jakob Lenz , Fabio del Giudice , Fabian R. Geisenhof , Felix Winterer , R. Thomas Weitz

Graphene based THz modulators are promising due to the conical band structure and high carrier mobility of graphene. Here, we tune the Fermi level of graphene via electrical gating with the help of ionic liquid to control the THz…

We study the electrode polarization behaviour of different Na-Ca-phosphosilicate glasses by measuring the differential capacitance between blocking Pt electrodes. At low applied dc bias voltages, we detect a linear capacitance regime with…

Disordered Systems and Neural Networks · Physics 2009-11-11 C. R. Mariappan , T. P. Heins , B. Roling

Vertical heterostructures combining different layered materials offer novel opportunities for applications and fundamental studies of collective behavior driven by inter-layer Coulomb coupling. Here we report heterostructures comprising a…

Mesoscale and Nanoscale Physics · Physics 2015-01-09 A. Gamucci , D. Spirito , M. Carrega , B. Karmakar , A. Lombardo , M. Bruna , A. C. Ferrari , L. N. Pfeiffer , K. W. West , Marco Polini , V. Pellegrini

Transport measurements made on films of thallium-oxide (n-type semiconductor) are presented and discussed. The focus in this work is on the strongly-localized regime where charge transport is by variable-range-hopping. It is demonstrated…

Mesoscale and Nanoscale Physics · Physics 2013-08-12 Z. Ovadyahu

Highly-efficient water splitting based on solar energy is one of the most attractive research focuses in the energy field. Searching for more candidate photocatalysts that can work under visible-light irradiation are highly demanded.…

Materials Science · Physics 2024-09-17 Yun-Lai Zhu , Jun-Hui Yuan , Ya-Qian Song , Sheng Wang , Kan-Hao Xue , Ming Xu , Xiao-Min Cheng , Xiang-Shui Miao

This work presents conclusive observations about the long lasting topic of eumelanins' electronic vs. ionic conduction, allowing to access unprecedented conductivity of this mammal pigment. Key strengths of the study include, the easy…

Interfacial thermal transport between electrodes and polymer electrolytes can play a crucial role in the thermal management of solid-state lithium-ion batteries (SLIBs). Modifying the electrode surface with functional molecules can…

Mesoscale and Nanoscale Physics · Physics 2021-07-22 Siyu Tian , Dezhao Huang , Zhihao Xu , Shiwen Wu , Tengfei Luo , Guoping Xiong

Ballistic electrons in solids can have mean free paths far larger than the smallest features patterned by lithography. This has allowed development and study of solid-state electron-optical devices such as beam splitters and quantum point…

Mesoscale and Nanoscale Physics · Physics 2017-05-24 Arthur W. Barnard , Alex Hughes , Aaron L. Sharpe , Kenji Watanabe , Takashi Taniguchi , David Goldhaber-Gordon

Under pressure, metals exhibit increasingly shorter interatomic distances. Intuitively, this response is expected to be accompanied by an increase in the widths of the valence and conduction bands and hence a more pronounced…

Materials Science · Physics 2017-10-16 Y. Ma , M. I. Eremets , A. R. Oganov , Y. Xie , I. Trojan , S. Medvedev , A. O. Lyakhov , M. Valle , V. Prakapenka
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