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Related papers: Entanglement-enhanced dual-comb spectroscopy

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Optical frequency combs, named for their comb-like peaks in the spectrum, are essential for various sensing applications. As the technology develops, its performance has reached the standard quantum limit dictated by the quantum…

Quantum Physics · Physics 2026-05-25 Haowei Shi , Quntao Zhuang

Laser spectroscopy and interferometry have provided an unparalleled view into the fundamental nature of matter and the universe through ultra-precise measurements of atomic transition frequencies and gravitational waves. Optical frequency…

Ultraviolet spectroscopy provides unique insights into the structure of matter with applications ranging from fundamental tests to photochemistry in the earth's atmosphere and astronomical observations from space telescopes. At longer…

Optics · Physics 2024-03-08 Bingxin Xu , Zaijun Chen , Theodor W. Hänsch , Nathalie Picqué

We report a direct demonstration of quantum-enhanced sensing in the Fourier domain by comparing single- and two-photon interference in a fiber-based interferometer under strictly identical noise conditions. The simultaneous acquisition of…

Optical frequency combs have emerged as a cornerstone for a wide range of areas, including spectroscopy, ranging, optical clocks, time and frequency transfer, waveform synthesis, and communications. However, quantum mechanical fluctuations…

Quantum Physics · Physics 2024-12-30 Abdulkarim Hariri , Shuai Liu , Haowei Shi , Quntao Zhuang , Xudong Fan , Zheshen Zhang

Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…

Chemical Physics · Physics 2026-04-21 Yuta Fujihashi , Ozora Iso , Ryosuke Shimizu , Akihito Ishizaki

Dual-comb interferometry is a measurement technique that uses two laser frequency combs to retrieve complex spectra in a line-by-line basis. This technique can be implemented with electro-optic frequency combs, offering intrinsic mutual…

Optics · Physics 2016-09-21 Vicente Duran , Peter A. Andrekson , Victor Torres-Company

Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…

Quantum interferometry methods exploit quantum resources, such as photonic entanglement, to enhance phase estimation beyond classical limits. Nonlinear optics has served as a workhorse for the generation of entangled photon pairs, ensuring…

Quantum Physics · Physics 2025-08-04 Romain Dalidet , Anthony Martin , Grégory Sauder , Laurent Labonté , Sébastien Tanzilli

Dual-comb spectroscopy is emerging as one of the most appealing applications of mid-infrared frequency combs for high-resolution molecular spectroscopy, as it leverages on the unique coherence properties of frequency combs combined with the…

Quantum-correlated interferometer is a newly emerging tool in quantum technology that offers classical-limit-breaking phase sensitivity. But to date, there exists a configurational bottleneck for its practicability due to the low…

Atomic Physics · Physics 2025-01-10 Wei Du , Shuhe Wu , Dong Zhang , Jun Chen , Yiquan Yang , Peiyu Yang , Jinxian Guo , Guzhi Bao , Weiping Zhang

The optical frequency comb has made a significant impact in precision spectroscopy and on our ability to probe atomic, molecular and, recently, nuclear transitions to further our understanding of their fundamental properties and how their…

Optics · Physics 2026-02-17 John J. McCauley , DylanP. Tooley , R. Jason Jones

With the advent of laser frequency combs, coherent light sources that offer equally-spaced sharp lines over a broad spectral bandwidth have become available. One decade after revolutionizing optical frequency metrology, frequency combs hold…

The femtosecond laser frequency comb has enabled the 21st century revolution in optical synthesis and metrology. A particularly compelling technique that relies on the broadband coherence of two laser frequency combs is dual-comb…

Optics · Physics 2023-07-19 Vicente Duran , Santiago Tainta , Victor Torres-Company

Dual-comb spectroscopy allows for the rapid, multiplexed acquisition of high-resolution spectra without the need for moving parts or low-resolution dispersive optics. This method of broadband spectroscopy is most often accomplished via…

In recent years, distributed quantum sensing has gained interest for a range of applications requiring networks of sensors, from global-scale clock synchronization to high energy physics. In particular, a network of entangled sensors can…

Frequency combs are multimode photonic systems that underlie countless precision sensing and metrology applications. Since their invention over two decades ago, numerous efforts have pushed frequency combs to broader bandwidths and more…

Quantum Physics · Physics 2025-11-18 Sahil Pontula , Debasmita Banerjee , Marin Soljacic , Yannick Salamin

Improvements to dual-comb interferometers will benefit precision spectroscopy and sensing, distance metrology, tomography, telecommunications etc. A specific requirement of such interferometers is to enforce mutual coherence between the two…

Optics · Physics 2018-08-10 Zaijun Chen , Ming Yan , Theodor W. Hänsch , Nathalie Picqué

Spectroscopy has attracted much attention in molecular detection, biomolecular identification, and chemical analysis for providing accurate measurement. However, it is almost unable to distinguish different sources with overlapped…

Instrumentation and Detectors · Physics 2020-05-12 Ting Qing , Shupeng Li , Yijie Fang , Xiaohu Tang , Lihan Wang , Meihui Cao , Xinyu Li , Shilong Pan

We demonstrate single-photon time-domain interference in a new realm. We observe interferences in the photon counting statistics with two separate mode-locked femtosecond lasers of slightly different repetition frequencies, each emitting a…

Optics · Physics 2020-12-01 Nathalie Picqué , Theodor W. Hänsch
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