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Van der Waals materials provide a versatile toolbox for the emergence of new quantum phenomena and the fabrication of functional heterostructures. Among them, the trihalide VI3 stands out for its unique magnetic and structural landscape.…

Materials Science · Physics 2024-02-07 A. De Vita , R. Sant , V. Polewczyk , G. van der Laan , N. B. Brookes , T. Kong , R. J. Cava , G. Rossi , G. Vinai , G. Panaccione

We grew high-quality single crystals of the 5f electron van der Waals compound UI$_3$ and investigated them by measurements of specific heat and magnetization as functions of temperature and magnetic field. UI$_3$ behaves as an…

Changes in the spin configuration of atomically-thin, magnetic van-der-Waals multilayers can cause drastic modifications in their opto-electronic properties. Conversely, the opto-electronic response of these systems provides information…

Mesoscale and Nanoscale Physics · Physics 2020-05-28 Zhe Wang , Marco Gibertini , Dumitru Dumcenco , Takashi Taniguchi , Kenji Watanabe , Enrico Giannini , Alberto F. Morpurgo

A comprehensive study of magnetocrystalline anisotropy of a layered van-der-Waals ferromagnet VI3 was performed. We measured angular dependences of the torque and magnetization with respect to the direction of the applied magnetic field…

Interest in van der Waals materials often stems from a desire to miniaturise existing technologies by exploiting their intrinsic layered structure to create near atomically-thin components that do not suffer from surface defects. One…

Mesoscale and Nanoscale Physics · Physics 2022-08-22 A. J. Healey , S. Rahman , S. C. Scholten , I. O. Robertson , G. J. Abrahams , N. Dontschuk , B. Liu , L. C. L. Hollenberg , Y. Lu , J. -P. Tetienne

VBr$_3$ is a van der Waals antiferromagnet below the N\'eel temperature of 26.5 K with a saturation moment of 1.2 mB/f.u. above the metamagnetic transitions detected in the in-plane and out-of-plane directions. To reveal the AFM structure…

The magnetic moment in van der Waals (vdW) materials containing 3d transition metals originates from unpaired d-electron spins and their interaction with surrounding ligands. The interplay between exchange interactions and magnetic…

We report a comprehensive investigation of the lattice and magnetic structure in van der Waals antiferromagnet VBr3, characterized by a BiI3-type structure at room temperature. Neutron diffraction experiments were performed on both…

Strongly Correlated Electrons · Physics 2024-08-06 Yimeng Gu , Yiqing Hao , Zeyu Kao , Yiqing Gu , Feiyang Liu , Shiyi Zheng , Huibo Cao , Lunhua He , Jun Zhao

Layered van der Waals ferromagnets are promising candidates for designing new spintronic devices. Here we investigated the critical properties and magnetocaloric effect connected with ferromagnetic transition in layered van der Waals VI$_3$…

Materials Science · Physics 2020-01-15 Yu Liu , Milinda Abeykoon , C. Petrovic

CrCl3 is a layered insulator that undergoes a crystallographic phase transition below room temperature and orders antiferromagnetically at low temperature. Weak van der Waals bonding between the layers and ferromagnetic in-plane magnetic…

The discovery of ordered magnetism in two-dimensional van der Waals materials at the monolayer limit challenges the Mermin-Wagner theorem, which forbids spontaneous breaking of continuous symmetries in two dimensions at finite temperatures.…

The theoretical description of quantum phase transition, induced by the external magnetic field, into antiferromagnetic state in the van Vleck - singlet - magnet with a single-ion anisotropy of "easy-plane" type and ion spin S=1 is…

Statistical Mechanics · Physics 2009-11-13 V. M. Kalita , I. M. Ivanova , V. M. Loktev

Since their first observation in 2017, atomically thin van der Waals (vdW) magnets have attracted significant fundamental, and application-driven attention. However, their low ordering temperatures, $T_c$, sensitivity to atmospheric…

Single crystals of EuNiGe$_3$ crystallizing in the non-centrosymmetric BaNiSn$_3$-type structure have been grown using In flux, enabling us to explore the anisotropic magnetic properties which was not possible with previously reported…

Strongly Correlated Electrons · Physics 2014-02-04 Arvind Maurya , P. Bonville , A. Thamizhavel , S. K. Dhar

We report a comprehensive high-field/high-frequency electron spin resonance (ESR) study on single crystals of the van der Waals magnet CrCl$_3$. This material, although being known for quite a while, has received recent significant…

Materials Science · Physics 2020-06-09 J. Zeisner , K. Mehlawat , A. Alfonsov , M. Roslova , T. Doert , A. Isaeva , B. Büchner , V. Kataev

Van der Waals magnet VI$_3$ demonstrates intriguing magnetic properties that render it great for use in various applications. However, its microscopic magnetic structure has not been determined yet. Here, we report neutron diffraction and…

Strongly Correlated Electrons · Physics 2021-08-19 Yiqing Hao , Yiqing Gu , Yimeng Gu , Erxi Feng , Huibo Cao , Songxue Chi , Hua Wu , Jun Zhao

Single crystalline samples of the van der Waals antiferromagnet CrPS4 were studied by measurements of specific heat and comprehensive anisotropic temperature- and magnetic field-dependent magnetization. In addition, measurements of the heat…

Materials Science · Physics 2021-06-09 Sergey L. Bud'ko , Elena Gati , Tyler J. Slade , Paul C. Canfield

Evolution of magnetism in single crystals of the van der Waals compound VI3 in external pressure up to 7.3 GPa studied by measuring magnetization and ac magnetic susceptibility is reported. Four magnetic phase transitions, at T1 = 54.5 K,…

The existence of the V3+ ion orbital moment is the open issue of the nature of magnetism in the van der Waals ferromagnet VI3. The huge magnetocrystalline anisotropy in conjunction with the significantly reduced ordered magnetic moment…

Materials Science · Physics 2023-03-06 David Hovancik , Cinthia Piamonteze , Jiri Pospisil , Karel Carva , Vladimir Sechovsky

The van der Waals material CrSBr stands out as a promising two-dimensional magnet. Especially, its high magnetic ordering temperature and versatile magneto-transport properties make CrSBr an important candidate for new devices in the…

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