Related papers: Intercombination line frequencies in $^{171}$Yb va…
We report absolute optical frequencies of electronic transitions from the $X\, ^2\Pi_{3/2},v''=0,J''=3/2$ rovibronic ground state to the 12 lowest levels of the $A\, ^2\Sigma^+,v'=0$ vibronic state in $^{16}$OH, as well as to the 16 lowest…
We perform high resolution spectroscopy on $^{176}$Lu$^+$ including the $^1S_0\leftrightarrow{^3}D_1$ and $^1S_0\leftrightarrow{^3}D_2$ clock transitions. Hyperfine structures and optical frequencies relative to the $^1S_0$ ground state of…
A sharp resonance line that appears in three-photon transitions between the $^{1}S_{0}$ and $^{3}P_{0}$ states of alkaline earth and Yb atoms is proposed as an optical frequency standard. This proposal permits the use of the even isotopes,…
We stabilise a microwave oscillator at 9.6 GHz to an optical clock laser at 344 THz by using a fibre-based femtosecond laser frequency comb as a transfer oscillator. With a second frequency comb we measure independently the instability of…
We present a 100 MHz repetition rate Yb-fiber-laser-pumped synchronously pumped optical parametric oscillator (SPOPO) delivering tunable frequency combs covering almost the entire visible spectral range. By intracavity doubling both the…
Optical clocks have extremely attractive applications in many fields, including time-frequency metrology, validation of fundamental physical principles, and relativistic geodesy. The 467 nm octupole transition in 171Yb+ ion exhibits…
We have performed for the first time direct laser spectroscopy of the 1S0-3P0 optical clock transition at 265.6 nm in fermionic isotopes of neutral mercury laser-cooled in a magneto-optical trap. Spectroscopy is performed by measuring the…
Broadband precision spectroscopy is indispensable for providing high fidelity molecular parameters for spectroscopic databases. We have recently shown that mechanical Fourier transform spectrometers based on optical frequency combs can…
We report on the first coherent excitation of the highly forbidden $^2S_{1/2}\rightarrow{}^2F_{7/2}$ electric octupole (E3) transition in a single trapped ${}^{172}$Yb$^+$ ion, an isotope without nuclear spin. Using the transition in…
The wide span and high density of lines in its rovibrational spectrum render hydrogen cyanide a useful spectroscopic media for referencing absolute frequencies of lasers in optical communication and dimensional metrology. We determined, for…
Over a two-year duration, we have compared the frequency of the 199Hg+ 5d106s 2S 1/2 (F=0)<-> 5d9 6s2 2D 5/2 (F=2) electric-quadrupole transition at 282 nm with the frequency of the ground-state hyperfine splitting in neutral 133Cs. These…
We report a direct measurement of the 0-1 R(0) vibrational transition frequency in ground-state hydrogen deuteride (HD) using infrared-ultraviolet double resonance spectroscopy in a molecular beam. Ground-state molecules are vibrationally…
We report on the measurement of the isotope shifts of the $3d^74s \,\, a \, {}^5\!F_5 - 3d^74p \,\, z \, {}^5\!G^o_6$ Fe~I line at 358~nm between all four stable isotopes ${}^{54}$Fe, ${}^{56}$Fe, ${}^{57}$Fe and ${}^{58}$Fe, as well as the…
Accurate measurements of different transition frequencies between atomic levels of the electronic and hyperfine structure over time are used to investigate temporal variations of the fine structure constant $\alpha$ and the…
Spin squeezing can improve atomic precision measurements beyond the standard quantum limit (SQL), and unitary spin squeezing is essential for improving atomic clocks. We report substantial and nearly unitary spin squeezing in $^{171}$Yb, an…
In 2003 we have measured the absolute frequency of the $(1S, F=1, m_F=\pm 1) \leftrightarrow (2S, F'=1, m_F'=\pm 1)$ two-photon transition in atomic hydrogen. We observed a variation of $(-29\pm 57)$ Hz over a 44 months interval separating…
Solid-state electronic spins are extensively studied in quantum information science, as their large magnetic moments offer fast operations for computing and communication, and high sensitivity for sensing. However, electronic spins are more…
We have measured the absolute frequency of the optical lattice clock based on $^{87}$Sr at PTB with an uncertainty of $3.9\times 10^{-16}$ using two caesium fountain clocks. This is close to the accuracy of today's best realizations of the…
We radically simplify coherently averaged dual-comb spectroscopy by introducing a real-time self-correction system: a radio frequency system-on-chip computes each incoming dual-comb interferogram's phase, frequency, and arrival time;…
A data acquisition system is described that is designed to stabilize cooling and probe rates to maximize detection sensitivity and minimize possible systematic errors due to correlations between drifting experimental conditions and varying…