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Related papers: Isotopic effects in molecular attosecond photoelec…

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Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

Chemical Physics · Physics 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

Characterizing time delays in molecular photoionization as a function of the ejected electron emission direction relative to the orientation of the molecule and the light polarization axis pro-vides unprecedented insights into the…

In this paper we present a mathematical analysis of the photoelectric effect for one-electron atoms in the framework of non-relativistic QED. We treat photo-ionization as a scattering process where in the remote past an atom in its ground…

Mathematical Physics · Physics 2015-05-14 Marcel Griesemer , Heribert Zenk

The photoelectron momentum shifts along the laser propagation are investigated by the time-dependent perturbation theory for diatomic molecules, such as H$_2^+$, N$_2$ and O$_2$. Such longitudinal momentum shifts characterize the photon…

Optics · Physics 2016-06-08 Di Lao , Pei-Lun He , Feng He

Resonant two-photon ionization in a system consisting of two spatially well-separated atoms is studied. Due to two-center electron-electron correlations, the ionization may also proceed through photo-excitation of both atoms with subsequent…

Atomic Physics · Physics 2015-05-27 C. Müller , A. B. Voitkiv

The photodissociation of the HD+ molecular ion in intense short- pulsed linearly polarized laser fields is studied using a time- dependent wave-packet approach where molecular rotation is fully included. We show that applying a coherent…

chem-ph · Physics 2019-04-04 Eric Charron , Annick Giusti-Suzor , Frederick Mies

When an atom or molecule absorbs a high-energy photon, an electron is emitted with a well-defined energy and a highly-symmetric angular distribution, ruled by energy quantization and parity conservation. These rules seemingly break down…

Formulas to describe the photoabsorption and the photon scattering by a plasma or a liquid metal are derived in a unified manner with each other. It is shown how the nuclear motion, the free-electron motion and the core-electron behaviour…

Materials Science · Physics 2009-10-31 Junzo Chihara

Ionization of matter by energetic radiation generally causes complex secondary reactions which are hard to decipher. Using large helium nanodroplets irradiated by XUV photons, we show that the full chain of processes ensuing primary…

Atomic and Molecular Clusters · Physics 2023-07-26 L. Ben Ltaief , K. Sishodia , S. Mandal , S. De , S. R. Krishnan , C. Medina , N. Pal , R. Richter , T. Fennel , M. Mudrich

The nature of light-induced structures in attosecond transient absorption spectroscopy of molecular systems is investigated theoretically. It is shown how nuclear dynamics affect these structures. We find that a theoretical three-surface…

Atomic Physics · Physics 2015-08-19 Jens E. Bækhøj , Lars Bojer Madsen

Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…

Chemical Physics · Physics 2016-07-27 Markus Kowalewski , Kochise Bennett , Jérémy R. Rouxel , Shaul Mukamel

We explore the novel capabilities offered by attosecond extreme ultraviolet and x-ray pulses that can be now generated by free-electron lasers and high-harmonics generation sources for probing photon-induced electron dynamics in molecules.…

Quantum Physics · Physics 2023-02-15 Marvin Reuner , Daria Popova-Gorelova

A hidden local symmetry formalism with a two-photon counterterm approach is performed based on the relativistic continuum quantum many-body theory. The underlying electromagnetic under-screening as well as screening effects between the…

Nuclear Theory · Physics 2007-05-23 Ji-sheng Chen

Modifications of photoionization arising from resonant electron-electron correlations between neighbouring atoms in an atomic sample are studied. The sample contains atomic species A and B, with the ionization potential of A being smaller…

Atomic Physics · Physics 2015-06-04 B. Najjari , C. Müller , A. B. Voitkiv

We investigate ionization of neon atoms by an isolated attosecond pump pulse in the presence of two coherent extreme ultraviolet or x-ray probe fields. The probe fields are tuned to a core-valence transition in the residual ion and induce…

Atomic Physics · Physics 2016-03-30 Jhih-An You , Nina Rohringer , Jan Marcus Dahlström

Isotopic effects in spectator fragmentations following heavy-ion collisions at relativistic energies are investigated using data from recent exclusive experiments with SIS beams at GSI. Reactions of 12C on 112,124Sn at incident energies 300…

Nuclear Experiment · Physics 2008-11-26 W. Trautmann

Reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) is a powerful photoelectron spectroscopy, offering direct access to internal dynamics of the target. It is being increasingly applied to molecular…

Chemical Physics · Physics 2023-04-10 Serguei Patchkovskii , Jakub Benda , Dominik Ertel , David Busto

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

We study photoproduction off nuclei based on a self consistent and covariant many body approach for the pion and isobar propagation in infinite nuclear matter. For the first time the t-channel exchange of an in-medium pion is evaluated in…

Nuclear Theory · Physics 2009-08-21 F. Riek , M. F. M. Lutz , C. L. Korpa

Using first principle approaches, we investigate the effects of isotope substitution on the inelastic features in the hydrogen molecular junction. We observe thatlocal heating and inelastic current have significant isotope-substitution…

Mesoscale and Nanoscale Physics · Physics 2009-04-06 Yu-Chang Chen