Related papers: Isotopic effects in molecular attosecond photoelec…
Proton-coupled electron transfer (PCET) is the underlying mechanism governing important reactions ranging from water splitting in photosynthesis to oxygen reduction in hydrogen fuel cells. The interplay of proton and electronic charge…
Charge separation properties, that is the ability of a chromophore, or a chromophore/semiconductor interface, to separate charges upon light absorption, are crucial characteristics for an efficient photovoltaic device. Starting from this…
The Fermi transition (\Delta L=\Delta S=0 and \Delta T=1) between the nuclear isobaric analog states (IAS), induced by the charge-exchange (p,n) or (3He,t) reaction, can be considered as "elastic" scattering of proton or 3He by the…
In this work we investigate the effects of the electron-electron interaction between a molecular junction and the metallic leads in time-dependent quantum transport. We employ the recently developed embedded Kadanoff-Baym method [Phys. Rev.…
Feynman path-integral deep potential molecular dynamics (PI-DPMD) calculations have been employed to study both light (H$_2$O) and heavy water (D$_2$O) within the isothermal-isobaric ensemble. In particular, the deep neural network is…
We propose an experimental scheme for performing sensitive, high-precision laser spectroscopy studies on fast exotic isotopes. By inducing a step-wise resonant ionization of the atoms travelling inside an electric field and subsequently…
The coupling of light to electrical charge carriers in semiconductors is the foundation of many technological applications. Attosecond transient absorption spectroscopy measures simultaneously how excited electrons and the vacancies they…
Isotope effects in a multiband superconductor with a leading interband pairing channel are investigated. A relatively small electron-phonon contribution into the pair-transfer interaction can cause effects of observed magnitude. A multiband…
Directly imaging structural dynamics involving hydrogen atoms by ultrafast diffraction methods is complicated by their low scattering cross-sections. Here we demonstrate that megaelectronvolt ultrafast electron diffraction is sufficiently…
Tho-photon absorption holds potential for many practical applications. We theoretically investigate the onset of this phenomenon in a semiconductor quantum dot -- metallic nanoshell composite subjected to a resonant CW excitation.…
The ionization of an atom by a high-frequency intense laser pulse, where the energy of a single-photon is sufficient to ionize the system, is investigated from first principles. It is shown that as a consequence of an AC Stark effect in the…
Using $He@C_{60}$ as an example, we demonstrate that static potential of the fullerene core essentially alters the cross section of the two-electron ionization differential in one-electron energy $d\sigma ^{++}(\omega )/d\epsilon $. We…
This is a tutorial-style introduction to the field of molecular polaritons. We describe the basic physical principles and consequences of strong light-matter coupling common to molecular ensembles embedded in UV-visible or infrared…
We study orientation and two-center interference effects in attosecond time-resolved photoionization of the H$_2$ molecule. Time resolution of XUV ionization of H$_2$ is gained through the phase retrieval capability of attosecond angular…
Time-resolved investigations of ultrafast electronic and molecular dynamics were not possible until recently. The typical time scale of these processes is in the picosecond to attosecond realm. The tremendous technological progress in…
Isotope separation is one of the grand challenges of modern society and holds great potential for basic science, medicine, energy, and defense. We consider here a new and general approach to isotope separation. The method is based on an…
Excitons are two-particle correlated bound states that are formed due to Coulomb interaction between single-particle holes and electrons. In the solid-state, cooperative interactions with surrounding quasiparticles can strongly tailor the…
Reactions $n_{\gamma }\gamma +$ $d+$ $_{z_{2}}^{A_{2}}X\rightarrow \left( n_{\gamma }\pm 1\right) \gamma +$ $p+$ $_{z_{2}}^{A_{2}+1}X$ and especially the reaction $d+$ $_{z_{2}}^{A_{2}}X\rightarrow \gamma +$ $p+$ $% _{z_{2}}^{A_{2}+1}X$,…
Observation of charge asymmetry by comparing electron and positron, or muon and anti-muon, scattering on a hadronic target presently serves as an experimental tool to study two-photon exchange effects. In addition to two-photon exchange,…
Photoelectron interferometry with femto- and atto-second light pulses is a powerful probe of the fast electron wavepacket dynamics, albeit it has practical limitations on the energy resolution. We show that one can simultaneously obtain…