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Quantum technologies would benefit from the development of high performance quantum defects acting as single-photon emitters or spin-photon interface. Finding such a quantum defect in silicon is especially appealing in view of its favorable…

Materials Science · Physics 2024-05-09 Yihuang Xiong , Jiongzhi Zheng , Shay McBride , Xueyue Zhang , Sinéad M. Griffin , Geoffroy Hautier

Spin defects in wide-band gap semiconductors are promising systems for the realization of quantum bits, or qubits, in solid-state environments. To date, defect qubits have only been realized in materials with strong covalent bonds. Here, we…

Materials Science · Physics 2016-02-03 Hosung Seo , Marco Govoni , Giulia Galli

Quantum sensing with solid-state spin defects has transformed nanoscale metrology, offering sub-wavelength spatial resolution with exceptional sensitivity to multiple signal types. Maximizing these advantages requires minimizing both the…

A prerequisite for exploiting spins for quantum data storage and processing is long spin coherence times. Phosphorus dopants in silicon (Si:P) have been favoured as hosts for such spins because of measured electron spin coherence times (T2)…

Clock transitions (CTs) in spin systems, which occur at avoided level crossings, enhance quantum coherence lifetimes T$_2$ because the transition becomes immune to the decohering effects of magnetic field fluctuations to first order. We…

Materials Science · Physics 2025-02-06 Brendan C. Sheehan , Guanchu Chen , Jonathan R. Friedman

Single electron spins coupled to multiple nuclear spins provide promising multi-qubit registers for quantum sensing and quantum networks. The obtainable level of control is determined by how well the electron spin can be selectively coupled…

We demonstrate optical spin polarization of the neutrally-charged silicon-vacancy defect in diamond ($\mathrm{SiV^{0}}$), an $S=1$ defect which emits with a zero-phonon line at 946 nm. The spin polarization is found to be most efficient…

Optically active spin defects in solids are promising platforms for quantum technologies. Here, we present a first-principles framework to investigate intersystem crossing processes, which represent crucial steps in the optical…

Solid-state spin defects, such as color centers in diamond, are among the most promising candidates for scalable and integrated quantum technologies. In particular, the good optical properties of silicon-vacancy centers in diamond combined…

Quantum Physics · Physics 2024-09-20 Marco Klotz , Andreas Tangemann , Alexander Kubanek

In this paper, we study the electron spin decoherence of single defects in silicon carbide (SiC) nuclear spin bath. We find that, although the natural abundance of $^{29}\rm{Si}$ ($p_{\rm{Si}}=4.7\%$) is about 4 times larger than that of…

Mesoscale and Nanoscale Physics · Physics 2015-01-09 Li-Ping Yang , Christian Burk , Mattias Widmann , Sang-Yun Lee , Jörg Wrachtrup , Nan Zhao

The negatively-charged silicon-vacancy (SiV$^-$) color center in diamond has recently emerged as a promising system for quantum photonics. Its symmetry-protected optical transitions enable creation of indistinguishable emitter arrays and…

One of the biggest challenges to implement quantum protocols and quantum information processing (QIP) is achieving long coherence times, usually requiring systems at ultra-low temperatures. The nitrogen-vacancy (NV) center in diamond is a…

Arrays of identical and individually addressable qubits lay the foundation for the creation of scalable quantum hardware such as quantum processors and repeaters. Silicon vacancy centers in diamond (SiV) offer excellent physical properties…

Spin-orbit effects, inherent to electrons confined in quantum dots at a silicon heterointerface, provide a means to control electron spin qubits without the added complexity of on-chip, nanofabricated micromagnets or nearby coplanar…

Mesoscale and Nanoscale Physics · Physics 2022-02-04 Ryan M. Jock , N. Tobias Jacobson , Martin Rudolph , Daniel R. Ward , Malcolm S. Carroll , Dwight R. Luhman

The negatively charged nitrogen-vacancy defect ($N-V^-$ center) in diamond is an important atomic-scale structure that can be used as a qubit in quantum computing and as a marker in biomedical applications. Its usefulness relies on the…

Materials Science · Physics 2015-05-13 Adam Gali , Erik Janzén , Péter Deák , Georg Kresse , Efthimios Kaxiras

An obstacle for spin-based quantum sensors is magnetic noise due to proximal spins. However, such a spin cluster surrounding the sensor can become an asset, if it can be controlled. Here, we polarize and readout a cluster of three nitrogen…

Quantum Physics · Physics 2016-09-07 Helena S. Knowles , Dhiren M. Kara , Mete Atatüre

Coupled spin chains are promising candidates for 'wiring up' qubits in solid-state quantum computing (QC). In particular, two nitrogen-vacancy centers in diamond can be connected by a chain of implanted nitrogen impurities; when driven by a…

Quantum Physics · Physics 2013-03-07 Yuting Ping , Brendon W. Lovett , Simon C. Benjamin , Erik M. Gauger

Quantum computation provides great speedup over its classical counterpart for certain problems. One of the key challenges for quantum computation is to realize precise control of the quantum system in the presence of noise. Control of the…

Quantum Physics · Physics 2015-11-30 Xing Rong , Jianpei Geng , Fazhan Shi , Ying Liu , Kebiao Xu , Wenchao Ma , Fei Kong , Zhen Jiang , Yang Wu , Jiangfeng Du

We consider entangling operations in a single nitrogen-vacancy (NV) center in diamond where the hyperfine-coupled nuclear spin qubits are addressed with radio-frequency (rf) pulses conditioned on the state of the central electron spin.…

Quantum Physics · Physics 2025-08-25 Regina Finsterhoelzl , Guido Burkard

Optically addressable spin defects in silicon carbide (SiC) are an emerging platform for quantum information processing. Lending themselves to modern semiconductor nanofabrication, they promise scalable high-efficiency spin-photon…

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