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In a recent inelastic neutron scattering experiment in the pseudogap state of the high temperature superconductor $\mathrm{YBa_{2}Cu_{3}O_{6.6}}$ an unusual `vertical' dispersion of the spin excitations with a large in-plane anisotropy was…

Superconductivity · Physics 2015-03-20 Chen-Hsuan Hsu , Zhiqiang Wang , Sudip Chakravarty

Using a combination of density functional theory (DFT) and spin-wave theory methods, we investigate the magnetic interactions and spin excitations in semiconducting VI$_3$. Exchange parameters of monolayer, bilayer, and bulk forms are…

Materials Science · Physics 2021-09-24 Elijah Gordon , V. V. Mkhitaryan , Haijun Zhao , Y. Lee , Liqin Ke

We derive the microscopic spin Hamiltonian for rhombohedral CrI$_3$ using extensive first-principles density functional theory (DFT) calculations which incorporate spin-orbit coupling and Hubbard U. Our calculations indicate a dominant…

Inelastic neutron scattering measurements have been performed to investigate the spin waves of the quasi-one-dimensional antiferromagnetic ladder compound BaFe$_2$S$_3$, where a superconducting transition was observed under pressure [H.…

Spin wave dispersion in the metallic antiferromagnet Mn$_3$Pt was investigated just above the order-order transition temperature by using the inelastic neutron scattering technique. The spin wave dispersion at $T = 400$ K along [100], [110]…

Materials Science · Physics 2017-07-06 Soshi Ibuka , Tetsuya Yokoo , Shinichi Itoh , Kazuya Kamazawa , Mitsutaka Nakamura , Motoharu Imai

CrSBr is an air-stable 2D van der Waals semiconducting magnet with great technological promise, but its atomic-scale magnetic interactions -- crucial information for high-frequency switching -- are poorly understood. We present an…

Materials Science · Physics 2022-07-18 A. Scheie , M. Ziebel , D. G. Chica , Y. J. Bae , Xiaoping Wang , A. I. Kolesnikov , Xiaoyang Zhu , X. Roy

The tetrameric Ni(II) spin cluster Ni4Mo12 has been studied by INS. The data were analyzed extensively in terms of a very general spin Hamiltonian, which includes antiferromagnetic Heisenberg interactions, biquadratic 2-spin and 3-spin…

Mesoscale and Nanoscale Physics · Physics 2010-06-11 J. Nehrkorn , M. Höck , M. Brüger , H. Mutka , J. Schnack , O. Waldmann

Magnetic van der Waals (vdW) materials have opened new frontiers for realizing novel many-body phenomena. Recently NiPS3 has received intense interest since it hosts an excitonic quasiparticle whose properties appear to be intimately linked…

Strongly Correlated Electrons · Physics 2024-04-29 W. He , Y. Shen , K. Wohlfeld , J. Sears , J. Li , J. Pelliciari , M. Walicki , S. Johnston , E. Baldini , V. Bisogni , M. Mitrano , M. P. M. Dean

We report an inelastic neutron scattering study of magnetic excitations in a quantum paramagnet driven into a magnetically ordered state by chemical substitution, namely Ni(Cl$_{1-x}$Br$_x$)$_2$$\cdot$4SC(NH$_2$)$_2$ with $x=0.21(2)$. The…

Strongly Correlated Electrons · Physics 2018-12-13 A. Mannig , K. Yu. Povarov , J. Ollivier , A. Zheludev

Kitaev interactions underlying a quantum spin liquid have been long sought, but experimental data from which their strengths can be determined directly is still lacking. Here, by carrying out inelastic neutron scattering measurements on…

Single crystal inelastic neutron scattering is used to study spin wave excitations in the fully polarized state of the frustrated quantum ferro-antiferromagnet BaCdVO(PO$_4$)$_2$. The data analysis is based on a Heisenberg spin Hamiltonian…

Strongly Correlated Electrons · Physics 2021-04-07 V. K. Bhartiya , S. Hayashida , K. Yu. Povarov , Z. Yan , Y. Qiu , S. Raymond , A. Zheludev

Strong quantum fluctuations and unconventional spin dynamics are well established in the spin-1/2 triangular lattice Heisenberg antiferromagnet. However, their survival in the spin-1 case remains an open question. We investigate the spin…

Exchange interactions up to fourth nearest neighbor are shown within a classical local-moment Heisenberg approach to be important to model inelastic neutron scattering data on the fcc kagome antiferromagnet IrMn$_3$. Spin wave frequencies…

Strongly Correlated Electrons · Physics 2021-08-04 M. D. LeBlanc , A. A. Aczel , G. E. Granroth , B. W. Southern , J. -Q. Yan , S. E. Nagler , J. P. Whitehead , M. L. Plumer

We report a neutron scattering study of the spin-1/2 alternating bond antiferromagnet Cu(NO_3)_2. 2.5D_2O for 0.06<k_BT/J_1<1.5. For k_BT/J_1 << 1 the excitation spectrum is dominated by a coherent singlet-triplet mode centered at…

Strongly Correlated Electrons · Physics 2009-10-31 Guangyong Xu , C. Broholm , Daniel H. Reich , M. A. Adams

We propose a new scheme for numerically computing collective-mode spectra for large-size systems, using a reformulation of the Random Phase Approximation. In this study, we apply this method to investigate the spectrum and nature of the…

Materials Science · Physics 2009-11-07 Mona Berciu , R. N. Bhatt

The idea of embedding and transmitting information within the fluctuations of the magnetic moments of spins (spin waves) has been recently proposed and experimentally tested. The coherence of spin waves, which describes how well defined…

The spin excitation continuum, expected to dominate the low-energy fluctuation spectrum in the Haldane spin chain around the Brillouin zone center, q=0, is directly observed by inelastic magnetic neutron scattering in the S=1 quasi-1D…

Strongly Correlated Electrons · Physics 2010-07-28 I. A. Zaliznyak , S. -H. Lee , S. V. Petrov

We develop a description of spin waves in a $3D$ quantum $XY$ antiferromagnet (AFM) in terms of macroscopic variables, magnetization and N\'eel vector densities. We consider a layered AFM with spins located on the honeycomb lattice. In the…

Materials Science · Physics 2023-04-04 Ankang Liu , Alexander M. Finkel'stein

We investigate magnetic excitations in the $S=1$ easy-plan-type triangular antiferromagnets CsFeCl$_{3}$ and RbFeCl$_{3}$ through a combination of inelastic neutron scattering measurements and spin-wave theory calculations based on an…

Strongly Correlated Electrons · Physics 2021-09-17 L. Stoppel , S. Hayashida , Z. Yan , A. Podlesnyak , A. Zheludev

The two-dimensional van der Waals (vdW) materials MPS_3(M = Mn, Fe, Co, Ni) display antiferromagnetic ordering of the magnetic moments at the transition metal ions. The possibility to exfoliate thin layers that preserve the magnetic order…

Materials Science · Physics 2024-08-28 Mohammad Amirabbasi , Peter Kratzer