We investigate magnetic excitations in the S=1 easy-plan-type triangular antiferromagnets CsFeCl3 and RbFeCl3 through a combination of inelastic neutron scattering measurements and spin-wave theory calculations based on an established exchange-coupling Hamiltonian. We show that in either material the model falls short of providing an adequate description of the measured intensities and for RbFeCl3 even fails to reproduce the measured dispersion relation. The most striking discrepancy is a very anisotropic azimuthal intensity distribution in the acoustic spin-wave branches in the long-wavelength limit, which is incompatible with spin-wave theory on a fundamental level. The observed anomalies are attributed to long-range dipolar interactions.
@article{arxiv.2106.09447,
title = {Anomalous spin waves in CsFeCl$_{3}$ and RbFeCl$_{3}$},
author = {L. Stoppel and S. Hayashida and Z. Yan and A. Podlesnyak and A. Zheludev},
journal= {arXiv preprint arXiv:2106.09447},
year = {2021}
}