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We present an alternative approach to pump-probe spectroscopy for measuring fast charge dynamics with an atomic force microscope (AFM). Our approach is based on coherent multifrequency lock-in measurement of the intermodulation between a…

Mesoscale and Nanoscale Physics · Physics 2019-01-30 Riccardo Borgani , David B. Haviland

The quantum dynamics of vibrational polaritonic states arising from the interaction of a bistable molecule with the quantized mode of a Fabry-Perot microcavity is investigated using an asymmetric double-well potential as a simplified…

Chemical Physics · Physics 2024-01-11 Loïse Attal , Florent Calvo , Cyril Falvo , Pascal Parneix

We consider the final stage of double ionization of $\rm O_2$ molecules by short linearly polarized laser pulses. The saddles of the effective adiabatic potential energy close to which simultaneous escape of electrons from a molecule takes…

Atomic Physics · Physics 2007-05-23 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt

We simulate vibrational strong (VSC) and ultrastrong coupling (V-USC) for liquid water with classical molecular dynamics simulations. When the cavity modes are resonantly coupled to the O-H stretch mode of liquid water, the infrared…

Chemical Physics · Physics 2020-07-21 Tao E. Li , Joseph E. Subotnik , Abraham Nitzan

We study a fermionic two-band model with the interband transition resonantly coupled to a cavity. This model was recently proposed to explain cavity-enhanced charge transport, but a thorough characterization of the closed system, in…

Computational Physics · Physics 2024-01-08 Sebastian Stumper , Junichi Okamoto

In this work, we present a field-theoretic model of strongly coupled photonic molecules composed of interacting dielectric cavities in a closed, perfect-electric-conductor domain. Within this setting, we treat the resulting inter-mode…

Optics · Physics 2025-12-17 Kevin C. Smith , Austin G. Nixon , David J. Masiello

For decades, scientists have studied the intricate charge migration dynamics, where after ionization a localized charge distribution ("hole") migrates across the molecule on a femtosecond timescale. This has the potential for controlling…

Chemical Physics · Physics 2026-03-12 Imam S. Wahyutama , Madhumita Rano , Henrik R. Larsson

We present a hybrid method for the simulation of colloidal systems, that combines molecular dynamics (MD) with the Lattice-Boltzmann (LB) scheme. The LB method is used as a model for the solvent in order to take into account the…

Soft Condensed Matter · Physics 2009-11-11 Apratim Chatterji , Juergen Horbach

We demonstrate parametric coupling between two modes of a silicon nitride membrane. We achieve the coupling by applying an oscillating voltage to a sharp metal tip that approaches the membrane surface to within a few 100 nm. When the…

We employ ultrafast pump-probe spectroscopy to directly monitor electron tunneling between discrete orbital states in a pair of spatially separated quantum dots. Immediately after excitation, several peaks are observed in the pump-probe…

Nonstationary pump-probe interaction between short laser pulses propagating in a resonant optically dense coherent medium is considered. A special attention is paid to the case, where the density of two-level particles is high enough that a…

Quantum Physics · Physics 2007-05-23 V. S. Egorov , V. N. Lebedev , I. B. Mekhov , P. V. Moroshkin , I. A. Chekhonin , S. N. Bagayev

A novel technique for measuring plasma conditions using monochromatic pump-broadband probe laser interactions has been experimentally demonstrated. Originally proposed in [J. Ludwig et al., Phys. Plasmas \textbf{26}, 113108 (2019)], this…

We have demonstrated that near complete coherence can be achieved in a four level double lambda-like systems using a train of ultra-short optical pulses. The effect of the Doppler broadening has been analyzed and a scheme has been proposed…

Optics · Physics 2014-01-16 Pawan Kumar , Amarendra K. Sarma

We propose a method for achieving highly efficient transfer between the vibrational states in a diatomic molecule. The process is mediated by strong laser pulses and can be understood in terms of light-induced potentials. In addition to…

Quantum Physics · Physics 2009-11-06 M. Rodriguez , K. -A. Suominen , B. M. Garraway

We report on a theoretical investigation concerning the polaronic effect on the transport properties of a charge carrier in the one-dimensional molecular chain. Our technique is based on the Feynman's path integral approach. Analytical…

Mesoscale and Nanoscale Physics · Physics 2015-12-10 Sikarin Yoo-Kong , Watchara Liewrian

The adiabatic charge pumping of a non-equilibrium state of spinless fermions in a one-dimensional lattice is investigated, with an emphasis placed on its usefulness in revealing many-body interaction effects on interband coherence. For a…

Mesoscale and Nanoscale Physics · Physics 2019-10-14 Sen Mu , Da-Jian Zhang , Longwen Zhou , Jiangbin Gong

Femtosecond optical pump-probe technique is used to study charge carrier dynamics in few-layer MoS2 samples fabricated by mechanical exfoliation. An ultrafast pump pulse excites carriers and differential reflection of a probe pulse tuned to…

Mesoscale and Nanoscale Physics · Physics 2011-11-01 Rui Wang , Brian A. Ruzicka , Nardeep Kumar , Matthew Z. Bellus , Hsin-Ying Chiu , Hui Zhao

We study the electrophoretic flow of suspensions of charged colloids with a mesoscopic method that allows to model generic experimental conditions. We show that for highly charged colloids their electrophoretic mobility increases…

Soft Condensed Matter · Physics 2015-05-28 Giovanni Giupponi , Ignacio Pagonabarraga

We study the mobility of a charged colloidal particle in a constant homogeneous electric field by means of computer simulations. The simulation method combines a lattice Boltzmann scheme for the fluid with standard Langevin dynamics for the…

Soft Condensed Matter · Physics 2007-06-20 Vladimir Lobaskin , Burkhard Duenweg , Christian Holm

We utilize near-infrared pump and mid-infrared probe spectroscopy to investigate the ultrafast electronic response of pressurized VO$_2$. Distinct pump-probe signals and a pumping threshold behavior are observed even in the pressure-induced…

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