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Recent experiments have observed that the chemical and photophysical properties of molecules can be modified inside an optical Fabry-Perot microcavity under collective vibrational strong coupling (VSC) conditions, and such modification is…
We analyse the equilibrium behaviour and non-equilibrium dynamics of sparse Boolean networks with self-interactions that evolve according to synchronous Glauber dynamics. Equilibrium analysis is achieved via a novel application of the…
In computational chemistry of molecular materials, strong static correlation effects appear when electronic states, often involving the ground state, become quasi-degenerate, as occurs, for example, in bond-breaking processes. Such…
Recent experiments suggest that vibrational strong coupling (VSC) may significantly modify ground-state chemical reactions and their rates even without external pumping. The intrinsic mechanism of this "vacuum-field catalysis" remains…
The central topic of this letter is to show that light-matter hybridization not only gives rise to novel dynamic responses but can also modify intermolecular interactions and induce new structural order. Using the van der Waals (vdW) system…
We describe vacuum fluctuations and photon-field correlations in interacting quantum mechanical light-matter systems, by generalizing the application of mixed quantum-classical dynamics techniques. We employ the multi-trajectory…
In this paper we consider a system of identical three two-level atoms interacting at resonance with a single-mode of the quantized field in a lossless cavity. The initial cavity field is prepared in the coherent state while the atoms are…
Recent experiments have shown contradictory effects of strong light-matter coupling on exciton-exciton annihilation (EEA) in organic molecular systems. In this work, we perform numerical simulations of polariton dynamics and reveal the role…
Molecular polaritons have become an emerging platform for remotely controlling molecular properties through strong light-matter interactions. Herein, a semiclassical approach is developed for describing molecular polaritons by…
Calibrating the role of entanglement in quantum algorithms is a crucial task in the development of quantum computing. Most existing studies have primarily focused on how the static properties of entanglement-such as its magnitude and…
Many-body phenomena in quantum materials emerge from the interplay among a broad continuum of electronic states, and controlling these interactions is critical for engineering novel phases. One promising approach exploits fluctuations of…
We consider a generalized double Jaynes-Cummings model consisting of two isolated two-level atoms, each contained in a lossless cavity, with the cavities interacting with each other through a controlled photon hopping mechanism. The…
When the interaction between a molecular system and confined light modes in an optical or plasmonic cavity is strong enough to overcome the dissipative process, hybrid light-matter states (polaritons) become the fundamental excitations in…
Placing an atom and a molecule in a cavity opens the door to initialize molecular dynamics by exciting a level of the atom. This approach enlarges the range of choosing the light source to trigger molecular dynamics substantially. The…
As pioneering experiments have shown, strong vibrational coupling between molecular vibrations and light modes in an optical cavity can significantly alter molecular properties and even affect chemical reactivity. However, the current…
Transition metal complexes for photochemical applications often feature a high density of electron-vibrational states characterized by nonadiabatic and spin-orbit couplings. Overall, the dynamics after photoexcitation is shaped by rapid…
Quantum correlations are interesting resources for modern quantum technologies such as quantum information processing, quantum communication, quantum teleportation, and quantum computation tasks. However, engineering these quantum states…
The interaction of atoms and molecules with quantum light as realized in cavities has become a highly topical and fast growing field of research. This interaction leads to the formation of hybrid light-matter states giving rise to new…
We show that long-distance steady-state quantum correlations (entanglement) between pairs of cavity-atom systems in an array of lossy and driven coupled resonators can be established and controlled. The maximal of entanglement for any pair…
In this paper, we study the interaction between a moving $\Lambda$-type three-level atom and a single-mode cavity field in the presence of intensity-dependent atom-field coupling. After obtaining the state vector of the entire system…