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Intrinsic ferromagnetism is a crucial ingredient to realize quantum anomalous Hall effect in quasi two dimensional materials, thus the search of intrinsic ferromagnetic topological materials is one of the most concerned issues in the field…

Second harmonic generation has been applied to study lattice, electronic and magnetic proprieties in atomically thin materials. However, inversion symmetry breaking is usually required for the materials to generate a large signal. In this…

Materials Science · Physics 2022-05-12 Zhuoliang Ni , Nan Huang , Amanda V. Haglund , David G. Mandrus , Liang Wu

We report a new member of topological insulator (TI) family i.e., Mn$_2$Sb$_2$Te$_5$, which belongs to MnSb$_2$Te$_4$ family and is a sister compound of Mn$_2$Bi$_2$Te$_5$. An antiferromagnetic layer of (MnTe)$_2$ has been inserted between…

Materials Science · Physics 2023-10-17 Ankush Saxena , V. P. S. Awana

The atomically thin MnBi2Te4 crystal is a novel magnetic topological insulator, exhibiting exotic quantum physics. Here we report a systematic investigation of ultrafast carrier dynamics and coherent interlayer phonons in few-layer MnBi2Te4…

The magnetic properties of the van der Waals magnetic topological insulators MnBi$_2$Te$_4$ and MnBi$_4$Te$_7$ are investigated by magneto-transport measurements. We evidence that the relative strength of the inter-layer exchange coupling J…

Second harmonic generation (SHG) is a powerful optical tool for identifying non-centrosymmetric crystalline structures. Here, we analyze SHG in multilayer graphenes (MLG), with a focus on its dependence on the stacking order, encapsulation…

Mesoscale and Nanoscale Physics · Physics 2026-03-25 Patrick Johansen Sarsfield , Takaaki V. Joya , Takuto Kawakami , Mikito Koshino , Vladimir Fal'ko

The magnetic van der Waals crystals (MnX2Te4)m(X2Te3)n (X = Sb, Bi) have drawn significant attention due to their rich topological properties and the tenability by external magnetic field. In this work, we report on the discovery of…

Symmetries, quantum geometries and electronic correlations are among the most important ingredients of condensed matters, and lead to nontrivial phenomena in experiments, for example, non-reciprocal charge transport. Here we report the…

Mesoscale and Nanoscale Physics · Physics 2022-10-25 Zhaowei Zhang , Naizhou Wang , Ning Cao , Aifeng Wang , Xiaoyuan Zhou , Kenji Watanabe , Takashi Taniguchi , Binghai Yan , Wei-bo Gao

Layered NbOX$_2$ ($X=\mathrm{Cl,\,Br,\,I}$), a member of the van der Waals ferroelectric family, exhibits intrinsic ferroelectricity and pronounced nonlinear optical responses, making it a promising candidate for integrated nanophotonics…

This joint experimental and theoretical study of the structural, vibrational and electrical properties of rhombohedral SnSb2Te4 at high pressure unveils the internal mechanisms of its compression. The equation of state and the internal…

Intrinsic magnetic topological insulators (MTIs) MnBi2Te4 and MnBi2Te4/(Bi2Te3)n are expected to realize the high-temperature quantum anomalous Hall effect (QAHE) and dissipationless electrical transport. Extensive efforts have been made on…

MnBi$_2$Te$_4$ is a promising representative of intrinsic antiferromagnetic topological insulators, which could enable rare quantum mechanical effects like the quantum anomalous Hall effect. Especially at low temperatures, numerous studies…

Strongly Correlated Electrons · Physics 2022-11-11 M. Köpf , S. H. Lee , Z. Q. Mao , C. A. Kuntscher

Nonreciprocal devices that allow the light propagation in only one direction are indispensable in photonic circuits and emerging quantum technologies. Contemporary optical isolators and circulators, however, require large size or strong…

Materials Science · Physics 2021-10-12 Shingo Toyoda , Manfred Fiebig , Taka-hisa Arima , Yoshinori Tokura , Naoki Ogawa

When thinned down to just a few atomic layers, the layered magnetic topological insulator MnBi2Te4 offers an exceptional platform for exploring a wide range of topological phenomena. In this work, we overcome longstanding challenges in…

Being the first intrinsic antiferromagnetic(AFM) topological insulator(TI), MnBi2Te4 is argued to be a topological axion state in its even-layer form due to the antiparallel magnetization between the top and bottom layers. Here we combine…

Single-crystal X-ray diffraction and nonlinear optical measurements, especially second- and third-harmonic generation (SHG/THG) are comprehensively investigated for the van der Waals layered material AgScP2S6 with a non-centrosymmetric P31c…

The interplay between band topology and magnetic order could generate a variety of time-reversal-breaking gapped topological phases with exotic topological quantization phenomena, such as quantum anomalous Hall (QAH) insulators and axion…

Mesoscale and Nanoscale Physics · Physics 2020-09-30 Yue Li , Yadong Jiang , Jinlong Zhang , Zhaochen Liu , Zhongqin Yang , Jing Wang

Three-dimensional (3D) compensated MnBi2Te4 is antiferromagnetic, but undergoes a spin-flop transition at intermediate fields, resulting in a canted phase before saturation. In this work, we experimentally show that the anomalous Hall…

The intrinsic magnetic layered topological insulator MnBi2Te4 with nontrivial topological properties and magnetic order has become a promising system for exploring exotic quantum phenomena such as quantum anomalous Hall effect. However, the…

The layered magnetic topological insulator MnBi$_2$Te$_4$ is a promising platform to realize the quantum anomalous Hall effect because its layers possess intrinsic ferromagnetism. However, it is not well understood why the high-spin $d^5$…

Computational Physics · Physics 2020-05-27 Jing Li , J. Y. Ni , X. Y. Li , H. -J. Koo , M. -H. Whangbo , J. S. Feng , H. J. Xiang