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We report the observation of optical second harmonic generation (SHG) in single-layer indium selenide (InSe). We measure a second harmonic signal of $>10^3$ $\textrm{cts/s}$ under nonresonant excitation using a home-built confocal…

Recently, natural van der Waals heterostructures of (MnBi2Te4)m(Bi2Te3)n have been theoretically predicted and experimentally shown to host tunable magnetic properties and topologically nontrivial surface states. In this work, we…

It is of fundamental importance but challenging to simultaneously identify atomic and magnetic configurations of two-dimensional van der Waals materials. In this work, we show that the nonreciprocal second-harmonic generation (SHG) can be a…

Materials Science · Physics 2020-07-15 Wenshen Song , Ruixiang Fei , Li Yang

The interplay of magnetism and topology is a key research subject in condensed matter physics and material science, which offers great opportunities to explore emerging new physics, like the quantum anomalous Hall (QAH) effect, axion…

Materials Science · Physics 2019-06-18 Jiaheng Li , Yang Li , Shiqiao Du , Zun Wang , Bing-Lin Gu , Shou-Cheng Zhang , Ke He , Wenhui Duan , Yong Xu

Van der Waals stacking presents new opportunities for nonlinear optics with its remarkable tunability and scalability. However, the fundamental role of interlayer interactions in modifying the overall nonlinear optical susceptibilities…

Materials Science · Physics 2026-03-11 Kanchan Shaikh , Taejun Yoo , Zeyuan Zhu , Qiuyang Li , Amalya C. Johnson , Hui Deng , Fang Liu , Yuki Kobayashi

As a sister compound and isostructural of MnBi2Te4, the high quality MnSb2Te4 single crystals are grown via solid-state reaction where prolonged annealing and narrow temperature window play critical roles on account of its thermal…

Materials Science · Physics 2021-04-05 Hao Li , Yaoxin Li , Yu-Kun Lian , Weiwei Xie , Ling Chen , Jinsong Zhang , Yang Wu , Shoushan Fan

MnBi$_2$Te$_4$ is an antiferromagnetic topological insulator which stimulates intense interests due to the exotic quantum phenomena and promising device applications. Surface structure is a determinant factor to understand the novel…

The van der Waals compound, MnBi$_2$Te$_4$, is the first intrinsic magnetic topological insulator, providing a materials platform for exploring exotic quantum phenomena such as the axion insulator state and the quantum anomalous Hall…

The magnetic topological insulator, MnBi$_2$Te$_4$, shows metallic behavior at zero magnetic fields (antiferromagnetic phase, AFM) in thin film transport, which coincides with gapless surface states observed by angle-resolved photoemission…

Materials Science · Physics 2023-03-27 Hengxin Tan , Binghai Yan

Crystal growth of MnBi$_{2}$Te$_{4}$ has delivered the first experimental corroboration of the 3D antiferromagnetic topological insulator state. Our present results confirm that the synthesis of MnBi$_{2}$Te$_{4}$ can be scaled-up and…

Manipulating the interlayer magnetic coupling in van der Waals magnetic materials and heterostructures is the key to tailoring their magnetic and electronic properties for various electronic applications and fundamental studies in condensed…

Materials Science · Physics 2020-08-19 Zhe Li , Jiaheng Li , Ke He , Xiangang Wan , Wenhui Duan , Yong Xu

Utilizing an interplay between band topology and intrinsic magnetism, the two-dimensional van der Waals (vdW) system MnBi_2Te_4 provides an ideal platform for realizing exotic quantum phenomena and offers great opportunities in the emerging…

Heterostructures composed of the intrinsic magnetic topological insulator MnBi$_2$Te$_4$ and its non-magnetic counterpart Bi$_2$Te$_3$ host distinct surface electronic band structures depending on the stacking order and exposed termination.…

Exotic quantum phenomena have been demonstrated in recently discovered intrinsic magnetic topological insulator MnBi2Te4. At its two-dimensional limit, quantum anomalous Hall (QAH) effect and axion insulator state are observed in odd and…

Materials Science · Physics 2020-06-24 Yonghao Yuan , Xintong Wang , Hao Li , Jiaheng Li , Yu Ji , Zhenqi Hao , Yang Wu , Ke He , Yayu Wang , Yong Xu , Wenhui Duan , Wei Li , Qi-Kun Xue

High-order harmonic generation (HHG) in solids - the frequency up-conversion of an optical signal - is governed by symmetries. At terahertz (THz) frequencies, HHG is a key technology to access high frequency spectral windows that are…

The interplay between nontrivial band topology and layered antiferromagnetism in MnBi2Te4 has opened up a new avenue for exploring topological phases of matter. Representative examples include the quantum anomalous Hall effect and axion…

The antiferromagnetic topological insulator has attracted lots of attention recently, as its intrinsic magnetism and topological property makes it a potential material to realize the quantum anomalous Hall effect (QAHE) at relative high…

Strongly Correlated Electrons · Physics 2020-11-04 Fei Jiao , Jingfeng Wang , Xianyu Wang , Meixia Chang , Lingbo Cai , Shu Zhu , Di Zhang , Qing Lu , Cao Wang , Shugang Tan , Yunlong Li , Jiayuan Hu , Qiang Jing , Bo Liu , Dong Qian

The intricate interplay between nontrivial topology and magnetism in two-dimensional (2D) materials has led to the emergence of many novel phenomena and functionalities. An outstanding example is the quantum anomalous Hall (QAH) effect,…

Mesoscale and Nanoscale Physics · Physics 2020-01-24 Chang Liu , Yongchao Wang , Hao Li , Yang Wu , Yaoxin Li , Jiaheng Li , Ke He , Yong Xu , Jinsong Zhang , Yayu Wang